Impact of Biomass Burning on Air Quality in Temuco City, Chile

Abstract Residential wood burning emits a complex mixture of particulate and gaseous compounds. In this article we show an in-depth chemical characterization of particulate matter evidencing the impact of biomass burning on the urban air quality in Greater Temuco, the capital city of the Araucanía R...

Full description

Saved in:
Bibliographic Details
Main Authors: Felipe Reyes, Sofía Ahumada, Francisca Rojas, Pedro Oyola, Yeanice Vásquez, Claudio Aguilera, Andres Henriquez, Ernesto Gramsch, Choong-Min Kang, Sanna Saarikoski, Kimmo Teinilä, Minna Aurela, Hilkka Timonen
Format: Article
Language:English
Published: Springer 2021-09-01
Series:Aerosol and Air Quality Research
Subjects:
Online Access:https://doi.org/10.4209/aaqr.210110
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1823862891558731776
author Felipe Reyes
Sofía Ahumada
Francisca Rojas
Pedro Oyola
Yeanice Vásquez
Claudio Aguilera
Andres Henriquez
Ernesto Gramsch
Choong-Min Kang
Sanna Saarikoski
Kimmo Teinilä
Minna Aurela
Hilkka Timonen
author_facet Felipe Reyes
Sofía Ahumada
Francisca Rojas
Pedro Oyola
Yeanice Vásquez
Claudio Aguilera
Andres Henriquez
Ernesto Gramsch
Choong-Min Kang
Sanna Saarikoski
Kimmo Teinilä
Minna Aurela
Hilkka Timonen
author_sort Felipe Reyes
collection DOAJ
description Abstract Residential wood burning emits a complex mixture of particulate and gaseous compounds. In this article we show an in-depth chemical characterization of particulate matter evidencing the impact of biomass burning on the urban air quality in Greater Temuco, the capital city of the Araucanía Region, Chile. The measurements were carried out at two sites, Las Encinas and Padre Las Casas, in spring and winter. Extremely high fine particulate matter (PM2.5) concentrations (up to 700 µg m–3) were frequently observed at both stations in the wintertime, while in spring, PM2.5 concentrations were significantly lower (campaign-average 6.4 and 8.6 µg m–3 in Las Encinas and Padre Las Casas, respectively). Chemical composition of submicron PM was dominated by organics (average 87%) followed by inorganic ions (10–30%) and a minor contribution of black carbon (< 5%). In the wintertime, atmospheric levels of biomass burning tracers, such as levoglucosan, potassium and chloride, were elevated and their diurnal profiles showed a significant concentration increase in the evening. Diurnal profiles combined with the in-depth chemical analysis clearly indicated that in the wintertime local biomass burning was the main source of air pollutants in the region. Furthermore, in winter, most of the high concentration events correlated with the periods with high surface pressure, low temperature and low wind speed. These events matched with higher temperatures at high altitude than at the surface characterizing the typical profile of a vertical inversion that prevents the dilution of air pollutants.
format Article
id doaj-art-65838e461c2d4aad8c37a101d41c61dc
institution Kabale University
issn 1680-8584
2071-1409
language English
publishDate 2021-09-01
publisher Springer
record_format Article
series Aerosol and Air Quality Research
spelling doaj-art-65838e461c2d4aad8c37a101d41c61dc2025-02-09T12:20:32ZengSpringerAerosol and Air Quality Research1680-85842071-14092021-09-01211112010.4209/aaqr.210110Impact of Biomass Burning on Air Quality in Temuco City, ChileFelipe Reyes0Sofía Ahumada1Francisca Rojas2Pedro Oyola3Yeanice Vásquez4Claudio Aguilera5Andres Henriquez6Ernesto Gramsch7Choong-Min Kang8Sanna Saarikoski9Kimmo Teinilä10Minna Aurela11Hilkka Timonen12Centro Mario Molina ChileCentro Mario Molina ChileCentro Mario Molina ChileCentro Mario Molina ChileCentro Mario Molina ChileCentro Mario Molina ChileCentro Mario Molina ChilePhysics Department, Universidad de Santiago de ChileDepartment of Environmental Health, Harvard T.H. Chan School of Public HealthAtmospheric Composition Research, Finnish Meteorological InstituteAtmospheric Composition Research, Finnish Meteorological InstituteAtmospheric Composition Research, Finnish Meteorological InstituteAtmospheric Composition Research, Finnish Meteorological InstituteAbstract Residential wood burning emits a complex mixture of particulate and gaseous compounds. In this article we show an in-depth chemical characterization of particulate matter evidencing the impact of biomass burning on the urban air quality in Greater Temuco, the capital city of the Araucanía Region, Chile. The measurements were carried out at two sites, Las Encinas and Padre Las Casas, in spring and winter. Extremely high fine particulate matter (PM2.5) concentrations (up to 700 µg m–3) were frequently observed at both stations in the wintertime, while in spring, PM2.5 concentrations were significantly lower (campaign-average 6.4 and 8.6 µg m–3 in Las Encinas and Padre Las Casas, respectively). Chemical composition of submicron PM was dominated by organics (average 87%) followed by inorganic ions (10–30%) and a minor contribution of black carbon (< 5%). In the wintertime, atmospheric levels of biomass burning tracers, such as levoglucosan, potassium and chloride, were elevated and their diurnal profiles showed a significant concentration increase in the evening. Diurnal profiles combined with the in-depth chemical analysis clearly indicated that in the wintertime local biomass burning was the main source of air pollutants in the region. Furthermore, in winter, most of the high concentration events correlated with the periods with high surface pressure, low temperature and low wind speed. These events matched with higher temperatures at high altitude than at the surface characterizing the typical profile of a vertical inversion that prevents the dilution of air pollutants.https://doi.org/10.4209/aaqr.210110Particulate matterResidential biomass burningChemical compositionElemental composition
spellingShingle Felipe Reyes
Sofía Ahumada
Francisca Rojas
Pedro Oyola
Yeanice Vásquez
Claudio Aguilera
Andres Henriquez
Ernesto Gramsch
Choong-Min Kang
Sanna Saarikoski
Kimmo Teinilä
Minna Aurela
Hilkka Timonen
Impact of Biomass Burning on Air Quality in Temuco City, Chile
Aerosol and Air Quality Research
Particulate matter
Residential biomass burning
Chemical composition
Elemental composition
title Impact of Biomass Burning on Air Quality in Temuco City, Chile
title_full Impact of Biomass Burning on Air Quality in Temuco City, Chile
title_fullStr Impact of Biomass Burning on Air Quality in Temuco City, Chile
title_full_unstemmed Impact of Biomass Burning on Air Quality in Temuco City, Chile
title_short Impact of Biomass Burning on Air Quality in Temuco City, Chile
title_sort impact of biomass burning on air quality in temuco city chile
topic Particulate matter
Residential biomass burning
Chemical composition
Elemental composition
url https://doi.org/10.4209/aaqr.210110
work_keys_str_mv AT felipereyes impactofbiomassburningonairqualityintemucocitychile
AT sofiaahumada impactofbiomassburningonairqualityintemucocitychile
AT franciscarojas impactofbiomassburningonairqualityintemucocitychile
AT pedrooyola impactofbiomassburningonairqualityintemucocitychile
AT yeanicevasquez impactofbiomassburningonairqualityintemucocitychile
AT claudioaguilera impactofbiomassburningonairqualityintemucocitychile
AT andreshenriquez impactofbiomassburningonairqualityintemucocitychile
AT ernestogramsch impactofbiomassburningonairqualityintemucocitychile
AT choongminkang impactofbiomassburningonairqualityintemucocitychile
AT sannasaarikoski impactofbiomassburningonairqualityintemucocitychile
AT kimmoteinila impactofbiomassburningonairqualityintemucocitychile
AT minnaaurela impactofbiomassburningonairqualityintemucocitychile
AT hilkkatimonen impactofbiomassburningonairqualityintemucocitychile