Interaction of SBA-15 with Dilute Acetic Acid and Ammonia

The SAXS pattern and pore volume of SBA-15 are not affected by aging SBA-15 with water, dilute acetic acid, and ammonia up for to 1 month, while the specific surface area is substantially depressed in interactions with basic solutions. The SEM images indicate pits on the side surfaces of SBA-15 part...

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Main Authors: Marta Kalbarczyk, Sebastian Skupiński, Daniel Kamiński, Marek Kosmulski
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Colloids and Interfaces
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Online Access:https://www.mdpi.com/2504-5377/9/3/39
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author Marta Kalbarczyk
Sebastian Skupiński
Daniel Kamiński
Marek Kosmulski
author_facet Marta Kalbarczyk
Sebastian Skupiński
Daniel Kamiński
Marek Kosmulski
author_sort Marta Kalbarczyk
collection DOAJ
description The SAXS pattern and pore volume of SBA-15 are not affected by aging SBA-15 with water, dilute acetic acid, and ammonia up for to 1 month, while the specific surface area is substantially depressed in interactions with basic solutions. The SEM images indicate pits on the side surfaces of SBA-15 particles in interactions with basic solutions. Aging of SBA-15 in ammonia solutions results in cavities formed by the collapse of walls between neighboring hexagonal channels in the SBA-15. This phenomenon is discussed with a special emphasis on its possible effect on the potentiometric titration curves. Especially, a standard procedure, in which the SSA measured before the titration is used to calculate the <i>σ</i><sub>0</sub>, is compared with a modified procedure, in which the SSAs measured before and after the titration are used to estimate the SSA for each data point separately.
format Article
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institution Kabale University
issn 2504-5377
language English
publishDate 2025-06-01
publisher MDPI AG
record_format Article
series Colloids and Interfaces
spelling doaj-art-63fbaa54a7f94abeade896b68257f8742025-08-20T03:26:56ZengMDPI AGColloids and Interfaces2504-53772025-06-01933910.3390/colloids9030039Interaction of SBA-15 with Dilute Acetic Acid and AmmoniaMarta Kalbarczyk0Sebastian Skupiński1Daniel Kamiński2Marek Kosmulski3Laboratory of Electrochemistry, Department of Electrical Engineering and Smart Technologies, Lublin University of Technology, Nadbystrzycka 38, 20-618 Lublin, PolandLaboratory of Electrochemistry, Department of Electrical Engineering and Smart Technologies, Lublin University of Technology, Nadbystrzycka 38, 20-618 Lublin, PolandDepartment of Organic Chemistry and Crystallography, Institute of Chemical Sciences, Faculty of Chemistry, Maria-Curie-Skłodowska University in Lublin, Pl. M Curie-Skłodowskiej 3, 20-031 Lublin, PolandLaboratory of Electrochemistry, Department of Electrical Engineering and Smart Technologies, Lublin University of Technology, Nadbystrzycka 38, 20-618 Lublin, PolandThe SAXS pattern and pore volume of SBA-15 are not affected by aging SBA-15 with water, dilute acetic acid, and ammonia up for to 1 month, while the specific surface area is substantially depressed in interactions with basic solutions. The SEM images indicate pits on the side surfaces of SBA-15 particles in interactions with basic solutions. Aging of SBA-15 in ammonia solutions results in cavities formed by the collapse of walls between neighboring hexagonal channels in the SBA-15. This phenomenon is discussed with a special emphasis on its possible effect on the potentiometric titration curves. Especially, a standard procedure, in which the SSA measured before the titration is used to calculate the <i>σ</i><sub>0</sub>, is compared with a modified procedure, in which the SSAs measured before and after the titration are used to estimate the SSA for each data point separately.https://www.mdpi.com/2504-5377/9/3/39mesoporous silicasurface chargingsurface charge density
spellingShingle Marta Kalbarczyk
Sebastian Skupiński
Daniel Kamiński
Marek Kosmulski
Interaction of SBA-15 with Dilute Acetic Acid and Ammonia
Colloids and Interfaces
mesoporous silica
surface charging
surface charge density
title Interaction of SBA-15 with Dilute Acetic Acid and Ammonia
title_full Interaction of SBA-15 with Dilute Acetic Acid and Ammonia
title_fullStr Interaction of SBA-15 with Dilute Acetic Acid and Ammonia
title_full_unstemmed Interaction of SBA-15 with Dilute Acetic Acid and Ammonia
title_short Interaction of SBA-15 with Dilute Acetic Acid and Ammonia
title_sort interaction of sba 15 with dilute acetic acid and ammonia
topic mesoporous silica
surface charging
surface charge density
url https://www.mdpi.com/2504-5377/9/3/39
work_keys_str_mv AT martakalbarczyk interactionofsba15withdiluteaceticacidandammonia
AT sebastianskupinski interactionofsba15withdiluteaceticacidandammonia
AT danielkaminski interactionofsba15withdiluteaceticacidandammonia
AT marekkosmulski interactionofsba15withdiluteaceticacidandammonia