Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter

85Kr is a noble gas radioactive nuclide with a half-life of 10.75 years, and it decays by emission of beta rays associated with weak gamma rays. Most of the 85Kr released into the atmosphere is artificially produced by neutron induced fission reactions, and it plays an important role in atmospheric...

Full description

Saved in:
Bibliographic Details
Main Author: LIANG Jianfeng, XIE Feng, DAI Yihua, SHI Quanlin, WANG Chunjie, LI Xuesong, GUAN Qingdi, JIANG Wengang, YU Gongshuo, LIU Zhichao
Format: Article
Language:English
Published: Editorial Board of Atomic Energy Science and Technology 2025-05-01
Series:Yuanzineng kexue jishu
Subjects:
Online Access:https://yznkxjs.xml-journal.net/article/doi/10.7538/yzk.2024.youxian.0643
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850270491328118784
author LIANG Jianfeng, XIE Feng, DAI Yihua, SHI Quanlin, WANG Chunjie, LI Xuesong, GUAN Qingdi, JIANG Wengang, YU Gongshuo, LIU Zhichao
author_facet LIANG Jianfeng, XIE Feng, DAI Yihua, SHI Quanlin, WANG Chunjie, LI Xuesong, GUAN Qingdi, JIANG Wengang, YU Gongshuo, LIU Zhichao
author_sort LIANG Jianfeng, XIE Feng, DAI Yihua, SHI Quanlin, WANG Chunjie, LI Xuesong, GUAN Qingdi, JIANG Wengang, YU Gongshuo, LIU Zhichao
collection DOAJ
description 85Kr is a noble gas radioactive nuclide with a half-life of 10.75 years, and it decays by emission of beta rays associated with weak gamma rays. Most of the 85Kr released into the atmosphere is artificially produced by neutron induced fission reactions, and it plays an important role in atmospheric environmental monitoring, detection of clandestine production of fissile materials, and verification of atmospheric transport model. Low-level detection of 85Kr is therefore required. Internal gas proportional counter (IGPC) is one of the primary techniques to measure 85Kr. However, studies about anti-coincidence measurement based on IGPC mostly focused on the measurement of 37Ar, and few studies about 85Kr were reported. In this paper, an anti-cosmic ray IGPC system was established to improve the detection sensitivity of 85Kr. A quasi-4π well-type plastic scintillator surrounding the inner IGPC was used as an anti-coincidence detector to actively shield the background arising from cosmic rays. Compared with the non-anticoincidence spectrum, the background count rate of the anti-coincidence spectrum decreases from 3.64 s−1 to 0.182 s−1. The activity concentration of 85Kr was measured using length compensation method, and the detection efficiency of the system was calibrated to be 95.8%. The minimum detectable activity of 85Kr of about 7 mBq was achieved within 24 hours, which effectively improves the measurement sensitivity of 85Kr.
format Article
id doaj-art-633efb593c2d491e83630b6d437cc2b4
institution OA Journals
issn 1000-6931
language English
publishDate 2025-05-01
publisher Editorial Board of Atomic Energy Science and Technology
record_format Article
series Yuanzineng kexue jishu
spelling doaj-art-633efb593c2d491e83630b6d437cc2b42025-08-20T01:52:38ZengEditorial Board of Atomic Energy Science and TechnologyYuanzineng kexue jishu1000-69312025-05-015951120112510.7538/yzk.2024.youxian.0643 Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter LIANG Jianfeng, XIE Feng, DAI Yihua, SHI Quanlin, WANG Chunjie, LI Xuesong, GUAN Qingdi, JIANG Wengang, YU Gongshuo, LIU Zhichao0Northwest Institute of Nuclear Technology, Xi’an 710024, China85Kr is a noble gas radioactive nuclide with a half-life of 10.75 years, and it decays by emission of beta rays associated with weak gamma rays. Most of the 85Kr released into the atmosphere is artificially produced by neutron induced fission reactions, and it plays an important role in atmospheric environmental monitoring, detection of clandestine production of fissile materials, and verification of atmospheric transport model. Low-level detection of 85Kr is therefore required. Internal gas proportional counter (IGPC) is one of the primary techniques to measure 85Kr. However, studies about anti-coincidence measurement based on IGPC mostly focused on the measurement of 37Ar, and few studies about 85Kr were reported. In this paper, an anti-cosmic ray IGPC system was established to improve the detection sensitivity of 85Kr. A quasi-4π well-type plastic scintillator surrounding the inner IGPC was used as an anti-coincidence detector to actively shield the background arising from cosmic rays. Compared with the non-anticoincidence spectrum, the background count rate of the anti-coincidence spectrum decreases from 3.64 s−1 to 0.182 s−1. The activity concentration of 85Kr was measured using length compensation method, and the detection efficiency of the system was calibrated to be 95.8%. The minimum detectable activity of 85Kr of about 7 mBq was achieved within 24 hours, which effectively improves the measurement sensitivity of 85Kr.https://yznkxjs.xml-journal.net/article/doi/10.7538/yzk.2024.youxian.064385krinternal gas proportional counteranti-cosmic raylow-level activity measurement
spellingShingle LIANG Jianfeng, XIE Feng, DAI Yihua, SHI Quanlin, WANG Chunjie, LI Xuesong, GUAN Qingdi, JIANG Wengang, YU Gongshuo, LIU Zhichao
Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter
Yuanzineng kexue jishu
85kr
internal gas proportional counter
anti-cosmic ray
low-level activity measurement
title Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter
title_full Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter
title_fullStr Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter
title_full_unstemmed Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter
title_short Radioactivity Measurement of 85Kr by Using Anti-cosmic Ray Internal Gas Proportional Counter
title_sort radioactivity measurement of 85kr by using anti cosmic ray internal gas proportional counter
topic 85kr
internal gas proportional counter
anti-cosmic ray
low-level activity measurement
url https://yznkxjs.xml-journal.net/article/doi/10.7538/yzk.2024.youxian.0643
work_keys_str_mv AT liangjianfengxiefengdaiyihuashiquanlinwangchunjielixuesongguanqingdijiangwengangyugongshuoliuzhichao radioactivitymeasurementof85krbyusinganticosmicrayinternalgasproportionalcounter