Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement

Abstract Fast Mobility Particle Sizer (FMPS) size distribution measurements with different inversion matrices were compared with the Scanning Mobility Particle Sizer (SMPS) for ambient aerosols sampled from a background location in Riverside, CA in this study. The FMPS-compact matrix showed the best...

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Main Authors: Yue Lin, Liem Pham, Xiaoliang Wang, Roya Bahreini, Heejung S. Jung
Format: Article
Language:English
Published: Springer 2021-01-01
Series:Aerosol and Air Quality Research
Subjects:
Online Access:https://doi.org/10.4209/aaqr.200525
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author Yue Lin
Liem Pham
Xiaoliang Wang
Roya Bahreini
Heejung S. Jung
author_facet Yue Lin
Liem Pham
Xiaoliang Wang
Roya Bahreini
Heejung S. Jung
author_sort Yue Lin
collection DOAJ
description Abstract Fast Mobility Particle Sizer (FMPS) size distribution measurements with different inversion matrices were compared with the Scanning Mobility Particle Sizer (SMPS) for ambient aerosols sampled from a background location in Riverside, CA in this study. The FMPS-compact matrix showed the best agreement with SMPS for particle concentration in the size ranges of 9–359 nm and 9–100 nm (for ultrafine particles). The FMPS-compact matrix also showed the best agreement with the SMPS for mode diameter. All FMPS inversion matrices showed size-dependent discrepancies compared with the SMPS. Measurement of the non-volatile fraction of ambient aerosol downstream of a catalytic stripper showed that the FMPS-compact matrix agreed best with the SMPS with the FMPS over SMPS linear regression slope of 0.99–1.00 for particle concentrations. This is likely due to the restructuring of soot during the removal of volatile coating. This study showed that the soot and compact matrices are insufficient for ambient aerosol measurement. Challenges remain for FMPS measurements when particle morphologies are not known a priori or when they are different from near spherical shape or aggregate structure.
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series Aerosol and Air Quality Research
spelling doaj-art-61db6ccbbc5b4044bc475687dc9f330c2025-08-20T02:48:27ZengSpringerAerosol and Air Quality Research1680-85842071-14092021-01-0121411210.4209/aaqr.200525Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol MeasurementYue Lin0Liem Pham1Xiaoliang Wang2Roya Bahreini3Heejung S. Jung4Department of Mechanical Engineering, University of California RiversideDepartment of Mechanical Engineering, University of California RiversideDesert Research InstituteDepartment of Environmental Science, University of California RiversideDepartment of Mechanical Engineering, University of California RiversideAbstract Fast Mobility Particle Sizer (FMPS) size distribution measurements with different inversion matrices were compared with the Scanning Mobility Particle Sizer (SMPS) for ambient aerosols sampled from a background location in Riverside, CA in this study. The FMPS-compact matrix showed the best agreement with SMPS for particle concentration in the size ranges of 9–359 nm and 9–100 nm (for ultrafine particles). The FMPS-compact matrix also showed the best agreement with the SMPS for mode diameter. All FMPS inversion matrices showed size-dependent discrepancies compared with the SMPS. Measurement of the non-volatile fraction of ambient aerosol downstream of a catalytic stripper showed that the FMPS-compact matrix agreed best with the SMPS with the FMPS over SMPS linear regression slope of 0.99–1.00 for particle concentrations. This is likely due to the restructuring of soot during the removal of volatile coating. This study showed that the soot and compact matrices are insufficient for ambient aerosol measurement. Challenges remain for FMPS measurements when particle morphologies are not known a priori or when they are different from near spherical shape or aggregate structure.https://doi.org/10.4209/aaqr.200525Particle size distributionInversion matrixAmbient particlesFractal dimensionFast Mobility Particle Sizer
spellingShingle Yue Lin
Liem Pham
Xiaoliang Wang
Roya Bahreini
Heejung S. Jung
Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement
Aerosol and Air Quality Research
Particle size distribution
Inversion matrix
Ambient particles
Fractal dimension
Fast Mobility Particle Sizer
title Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement
title_full Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement
title_fullStr Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement
title_full_unstemmed Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement
title_short Evaluation of Fast Mobility Particle Sizer (FMPS) for Ambient Aerosol Measurement
title_sort evaluation of fast mobility particle sizer fmps for ambient aerosol measurement
topic Particle size distribution
Inversion matrix
Ambient particles
Fractal dimension
Fast Mobility Particle Sizer
url https://doi.org/10.4209/aaqr.200525
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AT xiaoliangwang evaluationoffastmobilityparticlesizerfmpsforambientaerosolmeasurement
AT royabahreini evaluationoffastmobilityparticlesizerfmpsforambientaerosolmeasurement
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