Nuclear Magnetic Resonance Studies of Coordination Compounds

The applicability of donor and metal atom nmr to coordination chemistry is briefly reviewed. The following structural studies are discussed: (1) the use of 31P resonances for the determination of molecular geometry of complexes [RuCl2(QP)], [Fe(NCS)2(QP)] and [W(CO)3(QP)] (QP = [o-Ph2P•C6H4]3P); (2...

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Main Author: L.M. Venanzi
Format: Article
Language:deu
Published: Swiss Chemical Society 1976-04-01
Series:CHIMIA
Online Access:https://www.chimia.ch/chimia/article/view/9307
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author L.M. Venanzi
author_facet L.M. Venanzi
author_sort L.M. Venanzi
collection DOAJ
description The applicability of donor and metal atom nmr to coordination chemistry is briefly reviewed. The following structural studies are discussed: (1) the use of 31P resonances for the determination of molecular geometry of complexes [RuCl2(QP)], [Fe(NCS)2(QP)] and [W(CO)3(QP)] (QP = [o-Ph2P•C6H4]3P); (2) the use of 13C resonances for the formulation of the carbon moiety C8H11•OCH3 coordinated to a palladium atom and (3) the use of 14N to establish the nature of the donor atom in a number of thiocyanato-complexes. It is further shown that proton-noise decoupled 31P spectra can be conveniently used to obtain activation parameters for ligand exchange in complexes [Ni{P(OR)3}4]. A possible interpretation of changes in 1|J105Pt-15N| parameters, in platinum complexes containing primary amines, in terms of selective hybridization at the platinum atom is presented. Finally, possible future developments in nmr studies of coordination compounds are briefly outlined.
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spelling doaj-art-60a5a22f508d4faabaabd9918588ecb12025-08-20T02:29:54ZdeuSwiss Chemical SocietyCHIMIA0009-42932673-24241976-04-0130410.2533/chimia.1976.227Nuclear Magnetic Resonance Studies of Coordination CompoundsL.M. Venanzi0Laboratorium für Anorganische Chemie, Eidgenössische Technische Hochschule, Zürich, Switzerland The applicability of donor and metal atom nmr to coordination chemistry is briefly reviewed. The following structural studies are discussed: (1) the use of 31P resonances for the determination of molecular geometry of complexes [RuCl2(QP)], [Fe(NCS)2(QP)] and [W(CO)3(QP)] (QP = [o-Ph2P•C6H4]3P); (2) the use of 13C resonances for the formulation of the carbon moiety C8H11•OCH3 coordinated to a palladium atom and (3) the use of 14N to establish the nature of the donor atom in a number of thiocyanato-complexes. It is further shown that proton-noise decoupled 31P spectra can be conveniently used to obtain activation parameters for ligand exchange in complexes [Ni{P(OR)3}4]. A possible interpretation of changes in 1|J105Pt-15N| parameters, in platinum complexes containing primary amines, in terms of selective hybridization at the platinum atom is presented. Finally, possible future developments in nmr studies of coordination compounds are briefly outlined. https://www.chimia.ch/chimia/article/view/9307
spellingShingle L.M. Venanzi
Nuclear Magnetic Resonance Studies of Coordination Compounds
CHIMIA
title Nuclear Magnetic Resonance Studies of Coordination Compounds
title_full Nuclear Magnetic Resonance Studies of Coordination Compounds
title_fullStr Nuclear Magnetic Resonance Studies of Coordination Compounds
title_full_unstemmed Nuclear Magnetic Resonance Studies of Coordination Compounds
title_short Nuclear Magnetic Resonance Studies of Coordination Compounds
title_sort nuclear magnetic resonance studies of coordination compounds
url https://www.chimia.ch/chimia/article/view/9307
work_keys_str_mv AT lmvenanzi nuclearmagneticresonancestudiesofcoordinationcompounds