Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions

Electrosorptive removal of uranium from aqueous solutions has emerged as an auspicious approach for mitigating radioactive pollution, with carbon-based materials serving as pivotal electrode components due to their exceptional conductivity, tunable surface chemistry, and structural versatility. This...

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Main Authors: Ling Tang, Tao Wei, Yanfeng Wei, Yin Yu, Haipeng Zhang
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-08-01
Series:Frontiers in Materials
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fmats.2025.1639589/full
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author Ling Tang
Tao Wei
Yanfeng Wei
Yin Yu
Haipeng Zhang
author_facet Ling Tang
Tao Wei
Yanfeng Wei
Yin Yu
Haipeng Zhang
author_sort Ling Tang
collection DOAJ
description Electrosorptive removal of uranium from aqueous solutions has emerged as an auspicious approach for mitigating radioactive pollution, with carbon-based materials serving as pivotal electrode components due to their exceptional conductivity, tunable surface chemistry, and structural versatility. This review thoroughly examines recent progress in carbon-based capacitive deionization (CDI) electrodes for U(VI) removal and systematically assesses critical modification approaches, including heteroatom doping, surface functional group modification, and metal oxide loading. Each strategy is critically examined regarding its underlying mechanism, material design principles, and influence on uranium adsorption capacity and selectivity. A particular emphasis is placed on synergistic effects from combined modification approaches, which consistently outperform single-component systems. Bridging insights from environmental science and energy storage technologies, this work proposes an integrated optimization framework that establishes fundamental structure-performance relationships for CDI electrodes. By systematically synthesizing current research progress while identifying key knowledge gaps, this review offers strategic guidance for the rational design of next-generation carbon-based materials to enable efficient, selective, and sustainable radioactive wastewater remediation.
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spelling doaj-art-5ed6d02675e648d0b1e2a4fce1e8bdb22025-08-20T04:00:50ZengFrontiers Media S.A.Frontiers in Materials2296-80162025-08-011210.3389/fmats.2025.16395891639589Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutionsLing Tang0Tao Wei1Yanfeng Wei2Yin Yu3Haipeng Zhang4State Key Laboratory of Heavy Oil Processing at Karamay, Department of Engineering, China University of Petroleum-Beijing at Karamay, Karamay, ChinaState Key Laboratory of Heavy Oil Processing at Karamay, Department of Engineering, China University of Petroleum-Beijing at Karamay, Karamay, ChinaState Key Laboratory of Heavy Oil Processing at Karamay, Department of Engineering, China University of Petroleum-Beijing at Karamay, Karamay, ChinaXinjiang Academy of Environment Protection Science, Urumqi, Xinjiang, ChinaState Key Laboratory of Heavy Oil Processing at Karamay, Department of Engineering, China University of Petroleum-Beijing at Karamay, Karamay, ChinaElectrosorptive removal of uranium from aqueous solutions has emerged as an auspicious approach for mitigating radioactive pollution, with carbon-based materials serving as pivotal electrode components due to their exceptional conductivity, tunable surface chemistry, and structural versatility. This review thoroughly examines recent progress in carbon-based capacitive deionization (CDI) electrodes for U(VI) removal and systematically assesses critical modification approaches, including heteroatom doping, surface functional group modification, and metal oxide loading. Each strategy is critically examined regarding its underlying mechanism, material design principles, and influence on uranium adsorption capacity and selectivity. A particular emphasis is placed on synergistic effects from combined modification approaches, which consistently outperform single-component systems. Bridging insights from environmental science and energy storage technologies, this work proposes an integrated optimization framework that establishes fundamental structure-performance relationships for CDI electrodes. By systematically synthesizing current research progress while identifying key knowledge gaps, this review offers strategic guidance for the rational design of next-generation carbon-based materials to enable efficient, selective, and sustainable radioactive wastewater remediation.https://www.frontiersin.org/articles/10.3389/fmats.2025.1639589/fulluraniumelectrosorptioncarbon-based electrodeswater treatmentelectrode modification
spellingShingle Ling Tang
Tao Wei
Yanfeng Wei
Yin Yu
Haipeng Zhang
Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions
Frontiers in Materials
uranium
electrosorption
carbon-based electrodes
water treatment
electrode modification
title Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions
title_full Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions
title_fullStr Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions
title_full_unstemmed Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions
title_short Research advances in carbon-based electrode materials for electrosorptive separation of uranium from aqueous solutions
title_sort research advances in carbon based electrode materials for electrosorptive separation of uranium from aqueous solutions
topic uranium
electrosorption
carbon-based electrodes
water treatment
electrode modification
url https://www.frontiersin.org/articles/10.3389/fmats.2025.1639589/full
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