The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids

In this research, the catalytic activity of Fe3O4@SiO2-NNO-CuII nanocomposite was investigated in Suzuki coupling reaction of 4- tosylcoumarine with various substituted arylboronic acids. This reusable copper nanocatalyst activated CO bond and with the exit of tosylate group, CC bond was formed be...

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Main Authors: F. Rafiee, O. Nazari
Format: Article
Language:English
Published: Elsevier 2025-07-01
Series:Results in Chemistry
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Online Access:http://www.sciencedirect.com/science/article/pii/S2211715625003029
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author F. Rafiee
O. Nazari
author_facet F. Rafiee
O. Nazari
author_sort F. Rafiee
collection DOAJ
description In this research, the catalytic activity of Fe3O4@SiO2-NNO-CuII nanocomposite was investigated in Suzuki coupling reaction of 4- tosylcoumarine with various substituted arylboronic acids. This reusable copper nanocatalyst activated CO bond and with the exit of tosylate group, CC bond was formed between 4-position of coumarin and arylboronic acid derivative. The substituted 4-arylcoumarines were obtained in high yields and short reaction times under mild reaction. The prepared nanocatalyst was easily separated from the reaction mixture using an external magnet and could reused in the next reaction runs for at least 4 cycles.
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spelling doaj-art-5e11a0f28fe749e5b3f4c981bceb6fcb2025-08-20T03:02:36ZengElsevierResults in Chemistry2211-71562025-07-011610231910.1016/j.rechem.2025.102319The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acidsF. Rafiee0O. Nazari1Corresponding author.; Department of Organic Chemistry, Faculty of Chemistry, Alzahra University, Tehran, IranDepartment of Organic Chemistry, Faculty of Chemistry, Alzahra University, Tehran, IranIn this research, the catalytic activity of Fe3O4@SiO2-NNO-CuII nanocomposite was investigated in Suzuki coupling reaction of 4- tosylcoumarine with various substituted arylboronic acids. This reusable copper nanocatalyst activated CO bond and with the exit of tosylate group, CC bond was formed between 4-position of coumarin and arylboronic acid derivative. The substituted 4-arylcoumarines were obtained in high yields and short reaction times under mild reaction. The prepared nanocatalyst was easily separated from the reaction mixture using an external magnet and could reused in the next reaction runs for at least 4 cycles.http://www.sciencedirect.com/science/article/pii/S2211715625003029CC bond formationCu-catalyzed4-hydroxycoumarine4-arylcoumarineSilica-coated magnetic nanoparticles
spellingShingle F. Rafiee
O. Nazari
The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids
Results in Chemistry
CC bond formation
Cu-catalyzed
4-hydroxycoumarine
4-arylcoumarine
Silica-coated magnetic nanoparticles
title The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids
title_full The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids
title_fullStr The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids
title_full_unstemmed The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids
title_short The synthesis of 4-arylcoumarines via cu-catalyzed arylation 4-hydroxycoumarine with the substituted phenylboronic acids
title_sort synthesis of 4 arylcoumarines via cu catalyzed arylation 4 hydroxycoumarine with the substituted phenylboronic acids
topic CC bond formation
Cu-catalyzed
4-hydroxycoumarine
4-arylcoumarine
Silica-coated magnetic nanoparticles
url http://www.sciencedirect.com/science/article/pii/S2211715625003029
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