Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains

Chitosan has gained considerable attention in recent years as a versatile material with applications in many fields, including food, pharmaceuticals, tissue engineering, and agriculture. The degree of deacetylation (DD) is a critical parameter of the properties and functionality of chitosan, influen...

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Main Authors: Talita Martins, Gustavo L. Oliveira, Samuel B. Henriques, Eduardo H.M. Nunes
Format: Article
Language:English
Published: Associação Brasileira de Metalurgia e Materiais (ABM); Associação Brasileira de Cerâmica (ABC); Associação Brasileira de Polímeros (ABPol) 2025-07-01
Series:Materials Research
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Online Access:http://www.scielo.br/scielo.php?script=sci_arttext&pid=S1516-14392025000200264&lng=en&tlng=en
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author Talita Martins
Gustavo L. Oliveira
Samuel B. Henriques
Eduardo H.M. Nunes
author_facet Talita Martins
Gustavo L. Oliveira
Samuel B. Henriques
Eduardo H.M. Nunes
author_sort Talita Martins
collection DOAJ
description Chitosan has gained considerable attention in recent years as a versatile material with applications in many fields, including food, pharmaceuticals, tissue engineering, and agriculture. The degree of deacetylation (DD) is a critical parameter of the properties and functionality of chitosan, influencing its solubility, bioactivity and suitability for various applications. Accurate determination of DD is crucial as it directly affects the behavior of the material in different environments. However, high-precision methods for DD measurement are often costly and difficult to access, posing a challenge for both academic research and industrial applications. In this study, we evaluated the DD of commercial chitosan using a variety of widely available techniques, including potentiometric titration (PT), Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy, UV-Vis spectroscopy, and X-ray diffraction (XRD). Despite observed differences between methods, all techniques effectively quantified DD, shedding light on factors such as sample solubility, moisture content, baseline correction, and instrument accuracy that contribute to these differences. By demonstrating the feasibility and reliability of simple and accessible techniques for DD determination, this study provides valuable insights for improving the use of chitosan in both research and industry, making these materials more accessible for a wide range of applications.
format Article
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institution Kabale University
issn 1516-1439
language English
publishDate 2025-07-01
publisher Associação Brasileira de Metalurgia e Materiais (ABM); Associação Brasileira de Cerâmica (ABC); Associação Brasileira de Polímeros (ABPol)
record_format Article
series Materials Research
spelling doaj-art-5d85bd9c86aa4bde91fd46e0d00fea582025-08-20T03:51:18ZengAssociação Brasileira de Metalurgia e Materiais (ABM); Associação Brasileira de Cerâmica (ABC); Associação Brasileira de Polímeros (ABPol)Materials Research1516-14392025-07-0128suppl 110.1590/1980-5373-mr-2025-0108Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer ChainsTalita Martinshttps://orcid.org/0000-0002-0309-9849Gustavo L. OliveiraSamuel B. HenriquesEduardo H.M. Nuneshttps://orcid.org/0000-0001-6653-5137Chitosan has gained considerable attention in recent years as a versatile material with applications in many fields, including food, pharmaceuticals, tissue engineering, and agriculture. The degree of deacetylation (DD) is a critical parameter of the properties and functionality of chitosan, influencing its solubility, bioactivity and suitability for various applications. Accurate determination of DD is crucial as it directly affects the behavior of the material in different environments. However, high-precision methods for DD measurement are often costly and difficult to access, posing a challenge for both academic research and industrial applications. In this study, we evaluated the DD of commercial chitosan using a variety of widely available techniques, including potentiometric titration (PT), Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy, UV-Vis spectroscopy, and X-ray diffraction (XRD). Despite observed differences between methods, all techniques effectively quantified DD, shedding light on factors such as sample solubility, moisture content, baseline correction, and instrument accuracy that contribute to these differences. By demonstrating the feasibility and reliability of simple and accessible techniques for DD determination, this study provides valuable insights for improving the use of chitosan in both research and industry, making these materials more accessible for a wide range of applications.http://www.scielo.br/scielo.php?script=sci_arttext&pid=S1516-14392025000200264&lng=en&tlng=enChitosanDegree of DeacetylationPotentiometric titrationSpectroscopy methodsX-ray diffraction
spellingShingle Talita Martins
Gustavo L. Oliveira
Samuel B. Henriques
Eduardo H.M. Nunes
Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains
Materials Research
Chitosan
Degree of Deacetylation
Potentiometric titration
Spectroscopy methods
X-ray diffraction
title Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains
title_full Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains
title_fullStr Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains
title_full_unstemmed Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains
title_short Comparative Analysis of Analytical Methods for Quantifying the Deacetylation Degree in Chitosan Polymer Chains
title_sort comparative analysis of analytical methods for quantifying the deacetylation degree in chitosan polymer chains
topic Chitosan
Degree of Deacetylation
Potentiometric titration
Spectroscopy methods
X-ray diffraction
url http://www.scielo.br/scielo.php?script=sci_arttext&pid=S1516-14392025000200264&lng=en&tlng=en
work_keys_str_mv AT talitamartins comparativeanalysisofanalyticalmethodsforquantifyingthedeacetylationdegreeinchitosanpolymerchains
AT gustavololiveira comparativeanalysisofanalyticalmethodsforquantifyingthedeacetylationdegreeinchitosanpolymerchains
AT samuelbhenriques comparativeanalysisofanalyticalmethodsforquantifyingthedeacetylationdegreeinchitosanpolymerchains
AT eduardohmnunes comparativeanalysisofanalyticalmethodsforquantifyingthedeacetylationdegreeinchitosanpolymerchains