Optimization and validation of bifenazate and bifenazate-diazene quantification in agricultural products using a reduction method

Abstract Bifenazate is a widely used insecticide for mite control and readily oxidizes to bifenazate-diazene, which can revert to bifenazate under mild reducing conditions. This study aimed to develop a reliable method for quantifying bifenazate in agricultural products by optimizing the reduction c...

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Main Authors: Deuk-Yeong Lee, Hee-Jin Jeong, Jong-Wook Song, Ji-Young An, Jong-Su Seo, Jong-Hwan Kim
Format: Article
Language:English
Published: SpringerOpen 2025-06-01
Series:Journal of Analytical Science and Technology
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Online Access:https://doi.org/10.1186/s40543-025-00487-z
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Summary:Abstract Bifenazate is a widely used insecticide for mite control and readily oxidizes to bifenazate-diazene, which can revert to bifenazate under mild reducing conditions. This study aimed to develop a reliable method for quantifying bifenazate in agricultural products by optimizing the reduction conditions for bifenazate-diazene and evaluating the purification efficiency of different sorbents. Ascorbic acid was employed as a reductant, and four sorbents (PSA, PSA + C18, PSA + C18 + GCB, and Z-Sep +) were tested for matrix effects and recovery in pepper, mandarin, and brown rice. The optimal reduction conditions were determined to be 50 °C for 1 h, ensuring nearly complete conversion of bifenazate-diazene. Among the adsorbents, Z-Sep + demonstrated the lowest matrix effect and the highest recovery for bifenazate, followed by PSA + C18 and PSA. Considering the balance between matrix effects and recoveries across the three tested agricultural commodities, we optimized the analytical method using Z-Sep + as the primary purification sorbent. The developed method was validated for selectivity, linearity (R 2 > 0.999), accuracy, and precision, meeting international regulatory guidelines. While this study primarily focused on common agricultural matrices, future research is needed to evaluate the method’s applicability to a wider range of agricultural products, including those with complex matrices such as high-fat and high-protein foods, as well as its performance in real-world agricultural samples.
ISSN:2093-3371