Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.

The stonefish Synanceia verrucosa and Synanceia horrida are arguably the most venomous fish species on earth and the culprits of severe stings in humans globally. Investigation into the venoms of these two species has mainly focused on protein composition, in an attempt to identify the most medicall...

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Main Authors: Silvia Luiza Saggiomo, Steve Peigneur, Jan Tytgat, Norelle L. Daly, David Thomas Wilson
Format: Article
Language:English
Published: Wiley 2025-03-01
Series:FEBS Open Bio
Subjects:
Online Access:https://doi.org/10.1002/2211-5463.13926
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author Silvia Luiza Saggiomo
Steve Peigneur
Jan Tytgat
Norelle L. Daly
David Thomas Wilson
author_facet Silvia Luiza Saggiomo
Steve Peigneur
Jan Tytgat
Norelle L. Daly
David Thomas Wilson
author_sort Silvia Luiza Saggiomo
collection DOAJ
description The stonefish Synanceia verrucosa and Synanceia horrida are arguably the most venomous fish species on earth and the culprits of severe stings in humans globally. Investigation into the venoms of these two species has mainly focused on protein composition, in an attempt to identify the most medically relevant proteins, such as the lethal verrucotoxin and stonustoxin components. This study, however, focused on medically relevant small molecules, and through nuclear magnetic resonance, mass spectroscopy, and fractionation techniques, we discovered and identified the presence of three molecules new to stonefish venom, namely γ‐aminobutyric acid (GABA), choline and 0‐acetylcholine, and provide the first report of GABA identified in a fish venom. Analysis of the crude venoms on human nicotinic acetylcholine receptors (nAChRs) and a GABAA receptor (GABAAR) showed S. horrida venom could activate neuronal (α7) and adult muscle‐type (α1β1δε) nAChRs, while both crude S. horrida and S. verrucosa venoms activated the GABAAR (α1β2γ2). Cytotoxicity studies in immunologically relevant cells (human PBMCs) indicated the venoms possess cell‐specific cytotoxicity and analysis of the venom fractions on Na+ channel subtypes involved in pain showed no activity. This work highlights the need to further investigate the small molecules found in venoms to help understand the mechanistic pathways of clinical symptoms for improved treatment of sting victims, in addition to the discovery of potential drug leads.
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spelling doaj-art-58f91bf3a1664757bf081b68ee60b31e2025-08-20T02:58:00ZengWileyFEBS Open Bio2211-54632025-03-0115339941410.1002/2211-5463.13926Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.Silvia Luiza Saggiomo0Steve Peigneur1Jan Tytgat2Norelle L. Daly3David Thomas Wilson4Australian Institute of Tropical Health and Medicine James Cook University Cairns AustraliaToxicology and Pharmacology Katholieke Universiteit (KU) Leuven BelgiumToxicology and Pharmacology Katholieke Universiteit (KU) Leuven BelgiumAustralian Institute of Tropical Health and Medicine James Cook University Cairns AustraliaAustralian Institute of Tropical Health and Medicine James Cook University Cairns AustraliaThe stonefish Synanceia verrucosa and Synanceia horrida are arguably the most venomous fish species on earth and the culprits of severe stings in humans globally. Investigation into the venoms of these two species has mainly focused on protein composition, in an attempt to identify the most medically relevant proteins, such as the lethal verrucotoxin and stonustoxin components. This study, however, focused on medically relevant small molecules, and through nuclear magnetic resonance, mass spectroscopy, and fractionation techniques, we discovered and identified the presence of three molecules new to stonefish venom, namely γ‐aminobutyric acid (GABA), choline and 0‐acetylcholine, and provide the first report of GABA identified in a fish venom. Analysis of the crude venoms on human nicotinic acetylcholine receptors (nAChRs) and a GABAA receptor (GABAAR) showed S. horrida venom could activate neuronal (α7) and adult muscle‐type (α1β1δε) nAChRs, while both crude S. horrida and S. verrucosa venoms activated the GABAAR (α1β2γ2). Cytotoxicity studies in immunologically relevant cells (human PBMCs) indicated the venoms possess cell‐specific cytotoxicity and analysis of the venom fractions on Na+ channel subtypes involved in pain showed no activity. This work highlights the need to further investigate the small molecules found in venoms to help understand the mechanistic pathways of clinical symptoms for improved treatment of sting victims, in addition to the discovery of potential drug leads.https://doi.org/10.1002/2211-5463.13926acetylcholineGABAstonefishSynanceiavenom
spellingShingle Silvia Luiza Saggiomo
Steve Peigneur
Jan Tytgat
Norelle L. Daly
David Thomas Wilson
Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.
FEBS Open Bio
acetylcholine
GABA
stonefish
Synanceia
venom
title Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.
title_full Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.
title_fullStr Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.
title_full_unstemmed Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.
title_short Interrogating stonefish venom: small molecules present in envenomation caused by Synanceia spp.
title_sort interrogating stonefish venom small molecules present in envenomation caused by synanceia spp
topic acetylcholine
GABA
stonefish
Synanceia
venom
url https://doi.org/10.1002/2211-5463.13926
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AT stevepeigneur interrogatingstonefishvenomsmallmoleculespresentinenvenomationcausedbysynanceiaspp
AT jantytgat interrogatingstonefishvenomsmallmoleculespresentinenvenomationcausedbysynanceiaspp
AT norelleldaly interrogatingstonefishvenomsmallmoleculespresentinenvenomationcausedbysynanceiaspp
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