Aluminum-Loaded Bifunctional Resins for Efficient Fluoride Removal from Aqueous Solutions

The deep defluorination of water remains a significant environmental challenge. In this work, aluminum was loaded onto the bifunctional resin S957 containing a phosphoric-sulfonic acid difunctional group for efficient fluoride removal. Al-S957 demonstrated excellent fluoride removal performance acro...

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Bibliographic Details
Main Authors: Mengfei Ma, Yingpeng Gu, Ruijie Wang, Yue Sun
Format: Article
Language:English
Published: MDPI AG 2025-07-01
Series:Applied Sciences
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Online Access:https://www.mdpi.com/2076-3417/15/14/7829
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Summary:The deep defluorination of water remains a significant environmental challenge. In this work, aluminum was loaded onto the bifunctional resin S957 containing a phosphoric-sulfonic acid difunctional group for efficient fluoride removal. Al-S957 demonstrated excellent fluoride removal performance across a broad pH range. When anions and organics coexisted, Al-S957 exhibited significantly better fluoride adsorption performance compared to aluminum-loaded monofunctional resins. The adsorption followed an endothermic chemisorption process on a monolayer surface. FTIR and XPS analyses further revealed that fluoride removal relied on a ligand exchange mechanism. Column adsorption conducted over five cycles highlighted the strong practical potential of Al-S957. The results suggested that Al-S957 exhibits significant potential for practical applications.
ISSN:2076-3417