A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution

A facile and waste-free flame thermal synthesis method was developed for preparing Pt modified C/TiO2 microspheres (Pt-C/TiO2). The photocatalysts were characterized with X-ray diffraction, field emission scanning electron microscopy, transmission electron microscope, ultraviolet-visible (UV-vis) di...

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Main Authors: Hui Li, Xiaoyan Zhang, Xiaoli Cui
Format: Article
Language:English
Published: Wiley 2014-01-01
Series:International Journal of Photoenergy
Online Access:http://dx.doi.org/10.1155/2014/414281
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author Hui Li
Xiaoyan Zhang
Xiaoli Cui
author_facet Hui Li
Xiaoyan Zhang
Xiaoli Cui
author_sort Hui Li
collection DOAJ
description A facile and waste-free flame thermal synthesis method was developed for preparing Pt modified C/TiO2 microspheres (Pt-C/TiO2). The photocatalysts were characterized with X-ray diffraction, field emission scanning electron microscopy, transmission electron microscope, ultraviolet-visible (UV-vis) diffuse reflectance spectra, X-ray photoelectron spectroscopy, and thermogravimetry analysis. The photocatalytic activity was evaluated by hydrogen evolution from water splitting under UV-vis light illumination. Benefitting from the electron-hole separation behavior and reduced overpotential of H+/H2, remarkably enhanced hydrogen production was demonstrated and the photocatalytic hydrogen generation from 0.4 wt% Pt-C/TiO2 increased by 22 times. This study also demonstrates that the novel and facile method is highly attractive, due to its easy operation, requiring no post treatment and energy-saving features.
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institution Kabale University
issn 1110-662X
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language English
publishDate 2014-01-01
publisher Wiley
record_format Article
series International Journal of Photoenergy
spelling doaj-art-5608f0d6d55b4c6a94013ac49e927efb2025-02-03T01:03:45ZengWileyInternational Journal of Photoenergy1110-662X1687-529X2014-01-01201410.1155/2014/414281414281A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen EvolutionHui Li0Xiaoyan Zhang1Xiaoli Cui2Department of Materials Science, Fudan University, Shanghai 200433, ChinaKey Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, ChinaDepartment of Materials Science, Fudan University, Shanghai 200433, ChinaA facile and waste-free flame thermal synthesis method was developed for preparing Pt modified C/TiO2 microspheres (Pt-C/TiO2). The photocatalysts were characterized with X-ray diffraction, field emission scanning electron microscopy, transmission electron microscope, ultraviolet-visible (UV-vis) diffuse reflectance spectra, X-ray photoelectron spectroscopy, and thermogravimetry analysis. The photocatalytic activity was evaluated by hydrogen evolution from water splitting under UV-vis light illumination. Benefitting from the electron-hole separation behavior and reduced overpotential of H+/H2, remarkably enhanced hydrogen production was demonstrated and the photocatalytic hydrogen generation from 0.4 wt% Pt-C/TiO2 increased by 22 times. This study also demonstrates that the novel and facile method is highly attractive, due to its easy operation, requiring no post treatment and energy-saving features.http://dx.doi.org/10.1155/2014/414281
spellingShingle Hui Li
Xiaoyan Zhang
Xiaoli Cui
A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
International Journal of Photoenergy
title A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
title_full A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
title_fullStr A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
title_full_unstemmed A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
title_short A Facile and Waste-Free Strategy to Fabricate Pt-C/TiO2 Microspheres: Enhanced Photocatalytic Performance for Hydrogen Evolution
title_sort facile and waste free strategy to fabricate pt c tio2 microspheres enhanced photocatalytic performance for hydrogen evolution
url http://dx.doi.org/10.1155/2014/414281
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