Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)

The paper presents the results of the development of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyl diglycolamide (TODGA) intended for the selective extraction of americium-241 from nitric acid solutions of liquid radioactive waste. (LRW). The structural and physico-chemical pr...

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Main Authors: Aleksandr A. Savelev, Valeriy I. Rachkov
Format: Article
Language:English
Published: National Research Nuclear University (MEPhI) 2025-06-01
Series:Nuclear Energy and Technology
Online Access:https://nucet.pensoft.net/article/152695/download/pdf/
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author Aleksandr A. Savelev
Valeriy I. Rachkov
author_facet Aleksandr A. Savelev
Valeriy I. Rachkov
author_sort Aleksandr A. Savelev
collection DOAJ
description The paper presents the results of the development of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyl diglycolamide (TODGA) intended for the selective extraction of americium-241 from nitric acid solutions of liquid radioactive waste. (LRW). The structural and physico-chemical properties of synthesized materials, including granulometric composition, porosity, and stability in nitric acid media, have been studied. The developed SPEs are stable in nitric acid solutions and meet the size requirements for use in industrial sorption columns. The results obtained can be used as a basis for creating technological schemes for the processing of LRW based on synthesized experimental modified samples of SPE TODGA, in particular for the isolation of minor actinides, including americium-241.
format Article
id doaj-art-55ecaafb6e03410097ccefcc0eb3fd82
institution OA Journals
issn 2452-3038
language English
publishDate 2025-06-01
publisher National Research Nuclear University (MEPhI)
record_format Article
series Nuclear Energy and Technology
spelling doaj-art-55ecaafb6e03410097ccefcc0eb3fd822025-08-20T02:10:16ZengNational Research Nuclear University (MEPhI)Nuclear Energy and Technology2452-30382025-06-0111210511610.3897/nucet.11.152695152695Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)Aleksandr A. Savelev0Valeriy I. Rachkov1University MEPhIJSC “Proryv”The paper presents the results of the development of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyl diglycolamide (TODGA) intended for the selective extraction of americium-241 from nitric acid solutions of liquid radioactive waste. (LRW). The structural and physico-chemical properties of synthesized materials, including granulometric composition, porosity, and stability in nitric acid media, have been studied. The developed SPEs are stable in nitric acid solutions and meet the size requirements for use in industrial sorption columns. The results obtained can be used as a basis for creating technological schemes for the processing of LRW based on synthesized experimental modified samples of SPE TODGA, in particular for the isolation of minor actinides, including americium-241.https://nucet.pensoft.net/article/152695/download/pdf/
spellingShingle Aleksandr A. Savelev
Valeriy I. Rachkov
Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)
Nuclear Energy and Technology
title Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)
title_full Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)
title_fullStr Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)
title_full_unstemmed Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)
title_short Synthesis, investigation of the structure and physico-chemical properties of modified solid-phase extractants (SPE) based on N,N,N’,N’-tetraoctyldiglycolamide (TODGA)
title_sort synthesis investigation of the structure and physico chemical properties of modified solid phase extractants spe based on n n n n tetraoctyldiglycolamide todga
url https://nucet.pensoft.net/article/152695/download/pdf/
work_keys_str_mv AT aleksandrasavelev synthesisinvestigationofthestructureandphysicochemicalpropertiesofmodifiedsolidphaseextractantsspebasedonnnnntetraoctyldiglycolamidetodga
AT valeriyirachkov synthesisinvestigationofthestructureandphysicochemicalpropertiesofmodifiedsolidphaseextractantsspebasedonnnnntetraoctyldiglycolamidetodga