Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi

Abstract The interest in the rare-earth monopnictides was boosted after the discovery of unconventional surface-state pairs in antiferromagnetically ordered NdBi. In contrast to other materials in which such states were reported, CeBi is known to have multiple antiferromagnetic phases. In this study...

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Main Authors: Yevhen Kushnirenko, Brinda Kuthanazhi, Benjamin Schrunk, Evan O’Leary, Andrew Eaton, Robert-Jan Slager, Junyeong Ahn, Lin-Lin Wang, Paul C. Canfield, Adam Kaminski
Format: Article
Language:English
Published: Nature Portfolio 2024-11-01
Series:Communications Materials
Online Access:https://doi.org/10.1038/s43246-024-00692-0
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author Yevhen Kushnirenko
Brinda Kuthanazhi
Benjamin Schrunk
Evan O’Leary
Andrew Eaton
Robert-Jan Slager
Junyeong Ahn
Lin-Lin Wang
Paul C. Canfield
Adam Kaminski
author_facet Yevhen Kushnirenko
Brinda Kuthanazhi
Benjamin Schrunk
Evan O’Leary
Andrew Eaton
Robert-Jan Slager
Junyeong Ahn
Lin-Lin Wang
Paul C. Canfield
Adam Kaminski
author_sort Yevhen Kushnirenko
collection DOAJ
description Abstract The interest in the rare-earth monopnictides was boosted after the discovery of unconventional surface-state pairs in antiferromagnetically ordered NdBi. In contrast to other materials in which such states were reported, CeBi is known to have multiple antiferromagnetic phases. In this study, we perform angle-resolved photoemission spectroscopy (ARPES) measurements in conjunction with density functional theory (DFT) calculations to investigate the evolution of the electronic structure of CeBi upon a series of antiferromagnetic (AFM) transitions. We find evidence for a new AFM transition in addition to two previously known from transport studies. We demonstrate the development of an additional Dirac state in the ( + − + − ) ordered phase and a transformation of unconventional surface-state pairs in the ( + + − − ) ordered phase. This revises the phase diagram of this intriguing material, where there are now three distinct AFM states below T N in zero magnetic field instead of two as it was previously thought.
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issn 2662-4443
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publishDate 2024-11-01
publisher Nature Portfolio
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series Communications Materials
spelling doaj-art-54ef00afdc2244aebef43cead7d89baa2025-08-20T02:13:32ZengNature PortfolioCommunications Materials2662-44432024-11-01511610.1038/s43246-024-00692-0Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBiYevhen Kushnirenko0Brinda Kuthanazhi1Benjamin Schrunk2Evan O’Leary3Andrew Eaton4Robert-Jan Slager5Junyeong Ahn6Lin-Lin Wang7Paul C. Canfield8Adam Kaminski9Division of Materials Science and Engineering, Ames National LaboratoryDivision of Materials Science and Engineering, Ames National LaboratoryDivision of Materials Science and Engineering, Ames National LaboratoryDivision of Materials Science and Engineering, Ames National LaboratoryDivision of Materials Science and Engineering, Ames National LaboratoryTCM Group, Cavendish Laboratory, University of CambridgeDepartment of Physics, Harvard UniversityDivision of Materials Science and Engineering, Ames National LaboratoryDivision of Materials Science and Engineering, Ames National LaboratoryDivision of Materials Science and Engineering, Ames National LaboratoryAbstract The interest in the rare-earth monopnictides was boosted after the discovery of unconventional surface-state pairs in antiferromagnetically ordered NdBi. In contrast to other materials in which such states were reported, CeBi is known to have multiple antiferromagnetic phases. In this study, we perform angle-resolved photoemission spectroscopy (ARPES) measurements in conjunction with density functional theory (DFT) calculations to investigate the evolution of the electronic structure of CeBi upon a series of antiferromagnetic (AFM) transitions. We find evidence for a new AFM transition in addition to two previously known from transport studies. We demonstrate the development of an additional Dirac state in the ( + − + − ) ordered phase and a transformation of unconventional surface-state pairs in the ( + + − − ) ordered phase. This revises the phase diagram of this intriguing material, where there are now three distinct AFM states below T N in zero magnetic field instead of two as it was previously thought.https://doi.org/10.1038/s43246-024-00692-0
spellingShingle Yevhen Kushnirenko
Brinda Kuthanazhi
Benjamin Schrunk
Evan O’Leary
Andrew Eaton
Robert-Jan Slager
Junyeong Ahn
Lin-Lin Wang
Paul C. Canfield
Adam Kaminski
Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi
Communications Materials
title Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi
title_full Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi
title_fullStr Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi
title_full_unstemmed Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi
title_short Unexpected band structure changes within the higher-temperature antiferromagnetic state of CeBi
title_sort unexpected band structure changes within the higher temperature antiferromagnetic state of cebi
url https://doi.org/10.1038/s43246-024-00692-0
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