Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer

Objective: To assess the detection efficiencies of liquid radioisotopes in a well-type NaI(Tl) gamma spectrometer, focusing on the short-lived isotopes 99Tcm, 131I, and 18F. Methods: The detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer were systematical...

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Main Authors: Jiayu Liu, Xiaojun Lu, Chao Zhao
Format: Article
Language:English
Published: Elsevier 2025-02-01
Series:Radiation Medicine and Protection
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Online Access:http://www.sciencedirect.com/science/article/pii/S2666555724001187
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author Jiayu Liu
Xiaojun Lu
Chao Zhao
author_facet Jiayu Liu
Xiaojun Lu
Chao Zhao
author_sort Jiayu Liu
collection DOAJ
description Objective: To assess the detection efficiencies of liquid radioisotopes in a well-type NaI(Tl) gamma spectrometer, focusing on the short-lived isotopes 99Tcm, 131I, and 18F. Methods: The detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer were systematically investigated through calibration experiments and Monte Carlo simulations, and accounting for the coincidence-summing effect. Results: The results indicated that the detection efficiencies of 99Tcm, 131I, and 18F varied from 64.4% to 72.3%, 34.8%–43.1% and 27.3%–28.5% for different sample volumes ranging from 15 ​mL to 80 ​mL, respectively. The simulated detection efficiencies were highly consistent with the experimental results, with a largest relative deviation of 5% for the 3 radionuclides and 4 different sample volumes. Conclusion: The consistent results between the calibration experiments and Monte Carlo simulations reveal that this measuring device possesses high detection efficiencies of 99Tcm, 131I, and 18F, making it suitable for measuring low-level activity radioactive liquids, such as radioactive waste liquids to be discharged.
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publishDate 2025-02-01
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series Radiation Medicine and Protection
spelling doaj-art-54aecacefd304613b4015047d718e9992025-02-12T05:32:54ZengElsevierRadiation Medicine and Protection2666-55572025-02-01614650Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometerJiayu Liu0Xiaojun Lu1Chao Zhao2Shanghai Institute of Measurement and Testing Technology, Shanghai 201203, ChinaShanghai Institute of Measurement and Testing Technology, Shanghai 201203, ChinaCorresponding author.; Shanghai Institute of Measurement and Testing Technology, Shanghai 201203, ChinaObjective: To assess the detection efficiencies of liquid radioisotopes in a well-type NaI(Tl) gamma spectrometer, focusing on the short-lived isotopes 99Tcm, 131I, and 18F. Methods: The detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer were systematically investigated through calibration experiments and Monte Carlo simulations, and accounting for the coincidence-summing effect. Results: The results indicated that the detection efficiencies of 99Tcm, 131I, and 18F varied from 64.4% to 72.3%, 34.8%–43.1% and 27.3%–28.5% for different sample volumes ranging from 15 ​mL to 80 ​mL, respectively. The simulated detection efficiencies were highly consistent with the experimental results, with a largest relative deviation of 5% for the 3 radionuclides and 4 different sample volumes. Conclusion: The consistent results between the calibration experiments and Monte Carlo simulations reveal that this measuring device possesses high detection efficiencies of 99Tcm, 131I, and 18F, making it suitable for measuring low-level activity radioactive liquids, such as radioactive waste liquids to be discharged.http://www.sciencedirect.com/science/article/pii/S2666555724001187Well-type NaI(Tl) gamma spectrometerLiquid radioactive sampleDetection efficiencyMonte Carlo simulationCoincidence summing correction
spellingShingle Jiayu Liu
Xiaojun Lu
Chao Zhao
Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer
Radiation Medicine and Protection
Well-type NaI(Tl) gamma spectrometer
Liquid radioactive sample
Detection efficiency
Monte Carlo simulation
Coincidence summing correction
title Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer
title_full Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer
title_fullStr Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer
title_full_unstemmed Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer
title_short Study on the detection efficiencies of liquid 99Tcm, 131I, and 18F in a well-type NaI(Tl) gamma spectrometer
title_sort study on the detection efficiencies of liquid 99tcm 131i and 18f in a well type nai tl gamma spectrometer
topic Well-type NaI(Tl) gamma spectrometer
Liquid radioactive sample
Detection efficiency
Monte Carlo simulation
Coincidence summing correction
url http://www.sciencedirect.com/science/article/pii/S2666555724001187
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AT xiaojunlu studyonthedetectionefficienciesofliquid99tcm131iand18finawelltypenaitlgammaspectrometer
AT chaozhao studyonthedetectionefficienciesofliquid99tcm131iand18finawelltypenaitlgammaspectrometer