Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form

Abstract A UV-chemometric approach has been developed to analyze a ternary combination of aspirin, caffeine, and orphenadrine citrate without the need for previous separation. The method is easy, specific, accurate, and highly precise. The three medications were evaluated simultaneously utilizing CL...

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Main Authors: Sobhy M. El-Adl, Amr A. Mattar, Omar M. El-Abassy, Mahmoud M. Sebaiy
Format: Article
Language:English
Published: BMC 2025-03-01
Series:BMC Chemistry
Subjects:
Online Access:https://doi.org/10.1186/s13065-025-01429-x
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author Sobhy M. El-Adl
Amr A. Mattar
Omar M. El-Abassy
Mahmoud M. Sebaiy
author_facet Sobhy M. El-Adl
Amr A. Mattar
Omar M. El-Abassy
Mahmoud M. Sebaiy
author_sort Sobhy M. El-Adl
collection DOAJ
description Abstract A UV-chemometric approach has been developed to analyze a ternary combination of aspirin, caffeine, and orphenadrine citrate without the need for previous separation. The method is easy, specific, accurate, and highly precise. The three medications were evaluated simultaneously utilizing CLS, PLS, and PCR, which were generated based on separate data sets that yielded superior findings. Regrettably, their accurate estimation could only be achieved using the PLS approach. In order to determine the prediction power of each chemometric approach, its validity has been tested using 8 synthetic mixes. The latent variable number varies across various models as the dataset changes. The comparison of various methodologies and the assessment of the predictive capacity of each set of data were done using the predicted residual error sum of squares (PRESS) and the root mean square error of prediction (RMSEP). The created approach was also used to statistically compare the performance of PLS in a dataset with zero absorption, as well as to compare the performance of the offered chemometric methods in various datasets. The environmental impact of the created approach was assessed to determine the overall ecological sustainability of the designed methodology. According to the new Blue Applicability Grade Index (BAGI) evaluation methodology, the suggested technique was also found to be practicable.
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institution Kabale University
issn 2661-801X
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publishDate 2025-03-01
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series BMC Chemistry
spelling doaj-art-5457d016044744eb9cb25fefe5553b732025-08-20T03:41:39ZengBMCBMC Chemistry2661-801X2025-03-0119111210.1186/s13065-025-01429-xDevelopment of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage formSobhy M. El-Adl0Amr A. Mattar1Omar M. El-Abassy2Mahmoud M. Sebaiy3Medicinal Chemistry Department, Faculty of Pharmacy, Zagazig UniversityMedicinal Chemistry Department, Faculty of Pharmacy, Zagazig UniversityPharmaceutical Chemistry Department, Faculty of Pharmacy, Egyptian Russian UniversityMedicinal Chemistry Department, Faculty of Pharmacy, Zagazig UniversityAbstract A UV-chemometric approach has been developed to analyze a ternary combination of aspirin, caffeine, and orphenadrine citrate without the need for previous separation. The method is easy, specific, accurate, and highly precise. The three medications were evaluated simultaneously utilizing CLS, PLS, and PCR, which were generated based on separate data sets that yielded superior findings. Regrettably, their accurate estimation could only be achieved using the PLS approach. In order to determine the prediction power of each chemometric approach, its validity has been tested using 8 synthetic mixes. The latent variable number varies across various models as the dataset changes. The comparison of various methodologies and the assessment of the predictive capacity of each set of data were done using the predicted residual error sum of squares (PRESS) and the root mean square error of prediction (RMSEP). The created approach was also used to statistically compare the performance of PLS in a dataset with zero absorption, as well as to compare the performance of the offered chemometric methods in various datasets. The environmental impact of the created approach was assessed to determine the overall ecological sustainability of the designed methodology. According to the new Blue Applicability Grade Index (BAGI) evaluation methodology, the suggested technique was also found to be practicable.https://doi.org/10.1186/s13065-025-01429-xAspirinCaffeineOrphenadrine citrateAGREEBAGIGAPI
spellingShingle Sobhy M. El-Adl
Amr A. Mattar
Omar M. El-Abassy
Mahmoud M. Sebaiy
Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
BMC Chemistry
Aspirin
Caffeine
Orphenadrine citrate
AGREE
BAGI
GAPI
title Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
title_full Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
title_fullStr Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
title_full_unstemmed Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
title_short Development of UV-Chemometric techniques for resolving the overlapped spectra of aspirin, caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
title_sort development of uv chemometric techniques for resolving the overlapped spectra of aspirin caffeine and orphenadrine citrate in their combined pharmaceutical dosage form
topic Aspirin
Caffeine
Orphenadrine citrate
AGREE
BAGI
GAPI
url https://doi.org/10.1186/s13065-025-01429-x
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