Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>

<p>Several global modelling studies have explored the effects of lightning-generated nitrogen oxides (LNO<span class="inline-formula"><sub><i>x</i></sub></span>) on gas-phase chemistry and atmospheric radiative transfer, but few have quantified LNO...

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Main Authors: A. K. Luhar, A. C. Jones, J. M. Wilkinson
Format: Article
Language:English
Published: Copernicus Publications 2024-12-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/24/14005/2024/acp-24-14005-2024.pdf
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author A. K. Luhar
A. C. Jones
J. M. Wilkinson
J. M. Wilkinson
author_facet A. K. Luhar
A. C. Jones
J. M. Wilkinson
J. M. Wilkinson
author_sort A. K. Luhar
collection DOAJ
description <p>Several global modelling studies have explored the effects of lightning-generated nitrogen oxides (LNO<span class="inline-formula"><sub><i>x</i></sub></span>) on gas-phase chemistry and atmospheric radiative transfer, but few have quantified LNO<span class="inline-formula"><sub><i>x</i></sub></span>'s impact on aerosol, particularly when nitrate aerosol is included. This study addresses two key questions: (1) how does including nitrate aerosol affect properties such as tropospheric composition, and (2) how do these effects depend on lightning parameterisation and LNO<span class="inline-formula"><sub><i>x</i></sub></span> levels? Using the Met Office's Unified Model–United Kingdom Chemistry and Aerosol (UM–UKCA) global chemistry–climate model, which now includes a modal nitrate aerosol scheme, we investigate these effects with two lightning-flash-rate parameterisations. Our findings show that both nitrate aerosol and LNO<span class="inline-formula"><sub><i>x</i></sub></span> significantly impact tropospheric composition and aerosol responses. Including nitrate aerosol reduces global mean tropospheric OH by 5 %, decreases the tropospheric ozone burden by 4 %–5 %, increases methane lifetime by a similar amount, and alters the top-of-atmosphere (TOA) net downward radiative flux by <span class="inline-formula">−0.4</span> W m<span class="inline-formula"><sup>−2</sup></span>. The inclusion of nitrate also shifts the aerosol size distribution, particularly in the Aitken and accumulation modes. A 5.2 Tg N yr<span class="inline-formula"><sup>−1</sup></span> increase in LNO<span class="inline-formula"><sub><i>x</i></sub></span> from a zero baseline results in global aerosol increases of 2.8 % in NH<span class="inline-formula"><sub>4</sub></span>, 4.7 % in fine NO<span class="inline-formula"><sub>3</sub></span>, 12 % in coarse NO<span class="inline-formula"><sub>3</sub></span>, and 5.8 % in SO<span class="inline-formula"><sub>4</sub></span> mass burdens. This much LNO<span class="inline-formula"><sub><i>x</i></sub></span> increase causes relatively small positive changes in aerosol optical depth, TOA radiative flux, and cloud droplet number concentration compared to when nitrate is included. The results, based on a fast uptake rate for HNO<span class="inline-formula"><sub>3</sub></span> to produce NH<span class="inline-formula"><sub>4</sub></span>NO<span class="inline-formula"><sub>3</sub></span>, likely represent an upper limit on nitrate effects.</p>
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spelling doaj-art-52fc852c80f24ffeb692cea58a5645742025-08-20T01:57:54ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242024-12-0124140051402810.5194/acp-24-14005-2024Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>A. K. Luhar0A. C. Jones1J. M. Wilkinson2J. M. Wilkinson3CSIRO Environment, Aspendale, Victoria 3195, AustraliaMet Office, Fitzroy Road, Exeter, EX1 3PB, UKMet Office, Fitzroy Road, Exeter, EX1 3PB, UKnow at: Forecast Department, European Centre for Medium-Range Weather Forecasts, Reading, RG2 9AX, UK<p>Several global modelling studies have explored the effects of lightning-generated nitrogen oxides (LNO<span class="inline-formula"><sub><i>x</i></sub></span>) on gas-phase chemistry and atmospheric radiative transfer, but few have quantified LNO<span class="inline-formula"><sub><i>x</i></sub></span>'s impact on aerosol, particularly when nitrate aerosol is included. This study addresses two key questions: (1) how does including nitrate aerosol affect properties such as tropospheric composition, and (2) how do these effects depend on lightning parameterisation and LNO<span class="inline-formula"><sub><i>x</i></sub></span> levels? Using the Met Office's Unified Model–United Kingdom Chemistry and Aerosol (UM–UKCA) global chemistry–climate model, which now includes a modal nitrate aerosol scheme, we investigate these effects with two lightning-flash-rate parameterisations. Our findings show that both nitrate aerosol and LNO<span class="inline-formula"><sub><i>x</i></sub></span> significantly impact tropospheric composition and aerosol responses. Including nitrate aerosol reduces global mean tropospheric OH by 5 %, decreases the tropospheric ozone burden by 4 %–5 %, increases methane lifetime by a similar amount, and alters the top-of-atmosphere (TOA) net downward radiative flux by <span class="inline-formula">−0.4</span> W m<span class="inline-formula"><sup>−2</sup></span>. The inclusion of nitrate also shifts the aerosol size distribution, particularly in the Aitken and accumulation modes. A 5.2 Tg N yr<span class="inline-formula"><sup>−1</sup></span> increase in LNO<span class="inline-formula"><sub><i>x</i></sub></span> from a zero baseline results in global aerosol increases of 2.8 % in NH<span class="inline-formula"><sub>4</sub></span>, 4.7 % in fine NO<span class="inline-formula"><sub>3</sub></span>, 12 % in coarse NO<span class="inline-formula"><sub>3</sub></span>, and 5.8 % in SO<span class="inline-formula"><sub>4</sub></span> mass burdens. This much LNO<span class="inline-formula"><sub><i>x</i></sub></span> increase causes relatively small positive changes in aerosol optical depth, TOA radiative flux, and cloud droplet number concentration compared to when nitrate is included. The results, based on a fast uptake rate for HNO<span class="inline-formula"><sub>3</sub></span> to produce NH<span class="inline-formula"><sub>4</sub></span>NO<span class="inline-formula"><sub>3</sub></span>, likely represent an upper limit on nitrate effects.</p>https://acp.copernicus.org/articles/24/14005/2024/acp-24-14005-2024.pdf
spellingShingle A. K. Luhar
A. C. Jones
J. M. Wilkinson
J. M. Wilkinson
Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>
Atmospheric Chemistry and Physics
title Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>
title_full Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>
title_fullStr Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>
title_full_unstemmed Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>
title_short Quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning NO<sub><i>x</i></sub>
title_sort quantifying the impact of global nitrate aerosol on tropospheric composition fields and its production from lightning no sub i x i sub
url https://acp.copernicus.org/articles/24/14005/2024/acp-24-14005-2024.pdf
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