Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy

This study introduces an environmentally friendly method for dyeing silk using pigments extracted from young teak leaves (Tectona grandis L.), offering a sustainable solution to reduce pollution from synthetic dyes while repurposing agricultural waste. Ethanol (95 %) extraction of teak leaves showed...

Full description

Saved in:
Bibliographic Details
Main Authors: Nattadon Rungruangkitkrai, Rattanaphol Mongkholrattanasit, Peeraya Ounu, Nawarat Chartvivatpornchai, Jirachaya Boonyarit, Kamlai Laohaphatanaleart, Rungsima Chollakup
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Current Research in Green and Sustainable Chemistry
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S266608652500013X
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850118061874479104
author Nattadon Rungruangkitkrai
Rattanaphol Mongkholrattanasit
Peeraya Ounu
Nawarat Chartvivatpornchai
Jirachaya Boonyarit
Kamlai Laohaphatanaleart
Rungsima Chollakup
author_facet Nattadon Rungruangkitkrai
Rattanaphol Mongkholrattanasit
Peeraya Ounu
Nawarat Chartvivatpornchai
Jirachaya Boonyarit
Kamlai Laohaphatanaleart
Rungsima Chollakup
author_sort Nattadon Rungruangkitkrai
collection DOAJ
description This study introduces an environmentally friendly method for dyeing silk using pigments extracted from young teak leaves (Tectona grandis L.), offering a sustainable solution to reduce pollution from synthetic dyes while repurposing agricultural waste. Ethanol (95 %) extraction of teak leaves showed a rich in polyphenols and quinonoid compounds, which yielded a reddish-brown pigment suitable for dyeing. Key dyeing conditions, including temperature (30–100 °C), duration (10–60 min), and pH (3–11), were optimized to maximize color absorption and uniformity. Color performance was evaluated through spectrophotometry (L∗, a∗, b∗ values) and K/S measurements. Three mordants including alum (aluminum potassium sulfate), ferrous sulfate, and stannous chloride were tested using pre-, meta-, and post-mordanting techniques. Pre-mordanting with ferrous sulfate delivered the darkest shades and highest color intensity, along with excellent wash and light fastness (rated ≥4 on the Grey scale). FTIR spectroscopy revealed stable dye-mordant complexes formed through molecular coordination. The dyed silk exhibited mild antibacterial properties against Staphylococcus aureus and Escherichia coli in agar well diffusion tests, though inhibition zones were modest (<0.20 cm), likely due to residual bioactive compounds. These results position teak leaf extract as a multifunctional natural dye, combining aesthetic, ecological, and hygienic advantages. By aligning with circular economy principles, this approach presents a viable pathway for sustainable textile production. Nonetheless, future research should focus on optimizing extraction methods, boosting antimicrobial efficacy, and scaling the process for industrial applications.
format Article
id doaj-art-512d69a4260741de944831e7a07f7d3c
institution OA Journals
issn 2666-0865
language English
publishDate 2025-01-01
publisher Elsevier
record_format Article
series Current Research in Green and Sustainable Chemistry
spelling doaj-art-512d69a4260741de944831e7a07f7d3c2025-08-20T02:35:57ZengElsevierCurrent Research in Green and Sustainable Chemistry2666-08652025-01-011010045710.1016/j.crgsc.2025.100457Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacyNattadon Rungruangkitkrai0Rattanaphol Mongkholrattanasit1Peeraya Ounu2Nawarat Chartvivatpornchai3Jirachaya Boonyarit4Kamlai Laohaphatanaleart5Rungsima Chollakup6Department of Textile Science, Faculty of Agro-Industry, Kasetsart University, Bangkok, 10900, ThailandDepartment of Textile Chemistry Technology, Faculty of Industrial Textiles and Fashion Design, Rajamangala University of Technology Phra Nakhon, Bangkok, 10300, ThailandKasetsart Agricultural and Agro-Industrial Product Improvement Institute (KAPI), Kasetsart University, Bangkok, 10900, ThailandDepartment of Textile Science, Faculty of Agro-Industry, Kasetsart University, Bangkok, 10900, ThailandKasetsart Agricultural and Agro-Industrial Product Improvement Institute (KAPI), Kasetsart University, Bangkok, 10900, ThailandRattanakosin International College of Creative Entrepreneurship, Rajamangala University of Technology Rattanakosin, Nakhon Pathom, 73170, ThailandKasetsart Agricultural and Agro-Industrial Product Improvement Institute (KAPI), Kasetsart University, Bangkok, 10900, Thailand; Corresponding author. Kasetsart Agricultural and Agro-Industrial Product Improvement Institute (KAPI), Kasetsart University, 50 Ngam Wong Wan Rd., Chatujak, Bangkok, 10900, Thailand.This study introduces an environmentally friendly method for dyeing silk using pigments extracted from young teak leaves (Tectona grandis L.), offering a sustainable solution to reduce pollution from synthetic dyes while repurposing agricultural waste. Ethanol (95 %) extraction of teak leaves showed a rich in polyphenols and quinonoid compounds, which yielded a reddish-brown pigment suitable for dyeing. Key dyeing conditions, including temperature (30–100 °C), duration (10–60 min), and pH (3–11), were optimized to maximize color absorption and uniformity. Color performance was evaluated through spectrophotometry (L∗, a∗, b∗ values) and K/S measurements. Three mordants including alum (aluminum potassium sulfate), ferrous sulfate, and stannous chloride were tested using pre-, meta-, and post-mordanting techniques. Pre-mordanting with ferrous sulfate delivered the darkest shades and highest color intensity, along with excellent wash and light fastness (rated ≥4 on the Grey scale). FTIR spectroscopy revealed stable dye-mordant complexes formed through molecular coordination. The dyed silk exhibited mild antibacterial properties against Staphylococcus aureus and Escherichia coli in agar well diffusion tests, though inhibition zones were modest (<0.20 cm), likely due to residual bioactive compounds. These results position teak leaf extract as a multifunctional natural dye, combining aesthetic, ecological, and hygienic advantages. By aligning with circular economy principles, this approach presents a viable pathway for sustainable textile production. Nonetheless, future research should focus on optimizing extraction methods, boosting antimicrobial efficacy, and scaling the process for industrial applications.http://www.sciencedirect.com/science/article/pii/S266608652500013XNatural dyeTeak leavesSilk fabricMordantAntibacterial activitySustainable textiles
spellingShingle Nattadon Rungruangkitkrai
Rattanaphol Mongkholrattanasit
Peeraya Ounu
Nawarat Chartvivatpornchai
Jirachaya Boonyarit
Kamlai Laohaphatanaleart
Rungsima Chollakup
Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy
Current Research in Green and Sustainable Chemistry
Natural dye
Teak leaves
Silk fabric
Mordant
Antibacterial activity
Sustainable textiles
title Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy
title_full Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy
title_fullStr Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy
title_full_unstemmed Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy
title_short Enhancing sustainable silk Textiles: Optimization of teak leaf extract dyeing and antibacterial efficacy
title_sort enhancing sustainable silk textiles optimization of teak leaf extract dyeing and antibacterial efficacy
topic Natural dye
Teak leaves
Silk fabric
Mordant
Antibacterial activity
Sustainable textiles
url http://www.sciencedirect.com/science/article/pii/S266608652500013X
work_keys_str_mv AT nattadonrungruangkitkrai enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy
AT rattanapholmongkholrattanasit enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy
AT peerayaounu enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy
AT nawaratchartvivatpornchai enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy
AT jirachayaboonyarit enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy
AT kamlailaohaphatanaleart enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy
AT rungsimachollakup enhancingsustainablesilktextilesoptimizationofteakleafextractdyeingandantibacterialefficacy