Study of Surface Treatment by Ionic Plasma and Self-Protective Pastes of AISI 304 and 316L Stainless Steels: Chemical, Microstructural, and Nanohardness Evaluation

This work studied the effect of self-protective paste nitriding (SPN) and ion plasma nitriding (IPN) on the surface chemistry, microstructure, and nanohardness of AISI 304 and 316L stainless steels, with both treated at 440 °C for 5 h. Surface modifications analyzed using SEM and nanoindentation rev...

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Bibliographic Details
Main Authors: Francisco Martínez-Baltodano, Juan C. Díaz-Guillén, Lizsandra López-Ojeda, Gregorio Vargas-Gutiérrez, Wilian Pech-Rodríguez
Format: Article
Language:English
Published: MDPI AG 2025-04-01
Series:Lubricants
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Online Access:https://www.mdpi.com/2075-4442/13/5/195
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Summary:This work studied the effect of self-protective paste nitriding (SPN) and ion plasma nitriding (IPN) on the surface chemistry, microstructure, and nanohardness of AISI 304 and 316L stainless steels, with both treated at 440 °C for 5 h. Surface modifications analyzed using SEM and nanoindentation revealed distinct outcomes. SPN induced an oxynitriding effect due to the oxidation properties of the pastes, forming Fe<sub>3</sub>O<sub>4</sub> and Fe<sub>x</sub>C phases, while IPN produced an expanded austenite layer. Both methods enhanced surface nanohardness, but SPN showed superior results. For 316L SS, SPN increased nanohardness by 367.81% (6.83 GPa) compared to a 133.5% increase (3.41 GPa) with IPN. For 304 SS, SPN improved nanohardness by 26% (2.23 GPa), whereas IPN reduced it by 48% (0.92 GPa). These findings highlight SPN’s potential as an effective anti-wear treatment, particularly for 316L SS. The SPN process utilized a eutectic mixture of sodium cyanate and sodium carbonate, while IPN employed a N<sub>2</sub>:H<sub>2</sub> (1:1) gas mixture. SEM analyses confirmed the formation of γ-Fe(N) phases, indicating dispersed iron nitrides (FeN, Fe<sub>3</sub>N, Fe<sub>4</sub>N). SPN’s simultaneous oxidation and nitrocarburization led to an oxide layer above the nitride diffusion layer, enhancing mechanical properties through iron oxides (Fe<sub>3</sub>O<sub>4</sub>) and carbides (Fe<sub>x</sub>C). Comparative analysis showed that AISI 316L exhibited better performance than AISI 304, underscoring SPN’s effectiveness for surface modification.
ISSN:2075-4442