Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren

Among the various methods of preparing optically active polymers the so-called asymmetric-selective (stereoelective) polymerization of racemic monomers is particularly attractive. Racemic compounds such as propylene oxide, propylene sulfide and α-amino acid NCA have thus been polymerized with optic...

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Main Author: H.G. Bührer
Format: Article
Language:deu
Published: Swiss Chemical Society 1972-10-01
Series:CHIMIA
Online Access:https://www.chimia.ch/chimia/article/view/9033
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author H.G. Bührer
author_facet H.G. Bührer
author_sort H.G. Bührer
collection DOAJ
description Among the various methods of preparing optically active polymers the so-called asymmetric-selective (stereoelective) polymerization of racemic monomers is particularly attractive. Racemic compounds such as propylene oxide, propylene sulfide and α-amino acid NCA have thus been polymerized with optically active initiators to high-molecular weight optically active polymers. The interrelations between the structures of monomer and initiator on the one hand, and the stereoelectivity of the process on the other are discussed, together with some quantitative models. For highly stereoelective systems, e. g. propylene sulfide / ZnEt2 / optically active α-glycol, this type of polymerization is also an elegant way of separating racemic mixtures kinetically.
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spelling doaj-art-4ff7888f382a46f7aa4a8a4a90e0ea702025-08-20T02:20:29ZdeuSwiss Chemical SocietyCHIMIA0009-42932673-24241972-10-01261010.2533/chimia.1972.501Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen MonomerenH.G. Bührer0Midland Macromolecular Institute, 1910 West St.Andrews Drive, Midland, Michigan 48640, USA Among the various methods of preparing optically active polymers the so-called asymmetric-selective (stereoelective) polymerization of racemic monomers is particularly attractive. Racemic compounds such as propylene oxide, propylene sulfide and α-amino acid NCA have thus been polymerized with optically active initiators to high-molecular weight optically active polymers. The interrelations between the structures of monomer and initiator on the one hand, and the stereoelectivity of the process on the other are discussed, together with some quantitative models. For highly stereoelective systems, e. g. propylene sulfide / ZnEt2 / optically active α-glycol, this type of polymerization is also an elegant way of separating racemic mixtures kinetically. https://www.chimia.ch/chimia/article/view/9033
spellingShingle H.G. Bührer
Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren
CHIMIA
title Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren
title_full Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren
title_fullStr Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren
title_full_unstemmed Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren
title_short Asymmetrisch-Selektive Polymerisation von Nicht-Olefinischen Monomeren
title_sort asymmetrisch selektive polymerisation von nicht olefinischen monomeren
url https://www.chimia.ch/chimia/article/view/9033
work_keys_str_mv AT hgbuhrer asymmetrischselektivepolymerisationvonnichtolefinischenmonomeren