Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)

The structure of the title compound, [CdCl2(C15H16N4S)], at 100 K has monoclinic (P21/c) symmetry. The compound has a layer structure and is a 1:1 complex of the organic ligand and cadmium chloride. The ligand, 3,3-dimethyl-1-[(E)-[phenyl(pyridine-2-yl)methylidene]amino]thiourea (L, Bp44mT), is of i...

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Main Authors: Christian S. Parry, Bernard Kwabi-Addo, Timothy R. Ramadhar, Raymond J. Butcher
Format: Article
Language:English
Published: International Union of Crystallography 2025-05-01
Series:IUCrData
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Online Access:https://journals.iucr.org/paper?S241431462500464X
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author Christian S. Parry
Bernard Kwabi-Addo
Timothy R. Ramadhar
Raymond J. Butcher
author_facet Christian S. Parry
Bernard Kwabi-Addo
Timothy R. Ramadhar
Raymond J. Butcher
author_sort Christian S. Parry
collection DOAJ
description The structure of the title compound, [CdCl2(C15H16N4S)], at 100 K has monoclinic (P21/c) symmetry. The compound has a layer structure and is a 1:1 complex of the organic ligand and cadmium chloride. The ligand, 3,3-dimethyl-1-[(E)-[phenyl(pyridine-2-yl)methylidene]amino]thiourea (L, Bp44mT), is of interest with respect to anticancer activity, antiviral properties and potential use in conditions of iron overload, from hemochromatosis or from multiple transfusions in hematological disorders such as sickle cell disease or beta thalassemia. This study is aimed at uncovering the basis of selectivity of the ligand as a chelator and for lead optimization. We also examine the ligand's potential use in treating heavy metal poisoning from cadmium, arsenic, lead or mercury, and for environmental remediation. The crystal structure exhibits no intermolecular or intramolecular hydrogen bonding with the supramolecular features being driven by hydrophobic, π–π and long-range dispersion forces.
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publisher International Union of Crystallography
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spelling doaj-art-4fcfac72797e440c9d07db49e301f7ef2025-08-20T02:32:12ZengInternational Union of CrystallographyIUCrData2414-31462025-05-01105x25046410.1107/S241431462500464Xbt4171Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)Christian S. Parry0Bernard Kwabi-Addo1Timothy R. Ramadhar2Raymond J. Butcher3Department of Microbiology, College of Medicine, Howard University, Washington, DC 20059, USADepartment of Biochemistry, College of Medicine, Howard University, Washington, DC 20059, USADepartment of Chemistry, College of Arts and Science, Howard University, Washington, DC 20059, USADepartment of Chemistry, College of Arts and Science, Howard University, Washington, DC 20059, USAThe structure of the title compound, [CdCl2(C15H16N4S)], at 100 K has monoclinic (P21/c) symmetry. The compound has a layer structure and is a 1:1 complex of the organic ligand and cadmium chloride. The ligand, 3,3-dimethyl-1-[(E)-[phenyl(pyridine-2-yl)methylidene]amino]thiourea (L, Bp44mT), is of interest with respect to anticancer activity, antiviral properties and potential use in conditions of iron overload, from hemochromatosis or from multiple transfusions in hematological disorders such as sickle cell disease or beta thalassemia. This study is aimed at uncovering the basis of selectivity of the ligand as a chelator and for lead optimization. We also examine the ligand's potential use in treating heavy metal poisoning from cadmium, arsenic, lead or mercury, and for environmental remediation. The crystal structure exhibits no intermolecular or intramolecular hydrogen bonding with the supramolecular features being driven by hydrophobic, π–π and long-range dispersion forces.https://journals.iucr.org/paper?S241431462500464Xcrystal structurepost-industrial pollutionriverways and food chainthiosemicarbazone heterocycle ligandsheavy metals
spellingShingle Christian S. Parry
Bernard Kwabi-Addo
Timothy R. Ramadhar
Raymond J. Butcher
Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)
IUCrData
crystal structure
post-industrial pollution
riverways and food chain
thiosemicarbazone heterocycle ligands
heavy metals
title Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)
title_full Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)
title_fullStr Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)
title_full_unstemmed Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)
title_short Dichlorido{(E)-N,N-dimethyl-2-[phenyl(pyridin-2-yl)methylidene]hydrazine-1-carbothioamide}cadmium(II)
title_sort dichlorido e n n dimethyl 2 phenyl pyridin 2 yl methylidene hydrazine 1 carbothioamide cadmium ii
topic crystal structure
post-industrial pollution
riverways and food chain
thiosemicarbazone heterocycle ligands
heavy metals
url https://journals.iucr.org/paper?S241431462500464X
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AT timothyrramadhar dichloridoenndimethyl2phenylpyridin2ylmethylidenehydrazine1carbothioamidecadmiumii
AT raymondjbutcher dichloridoenndimethyl2phenylpyridin2ylmethylidenehydrazine1carbothioamidecadmiumii