Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity

This research includes synthesis of new heterocyclic containing (1,3-oxazepine) derivatives of 6- methyl 2-thiouracil. The preparation process started by the reaction of 6- methyl 2-thiouracil with ethyl chloroacete to give ethyl 2-((4-hydroxy-6-methylpyrimidin-2-yl) thio) acetate (1). Compound (1)...

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Main Authors: Khalid M. Mohammad, Mohammad R. Ahmed, Mahmoud H. Mahmoud
Format: Article
Language:English
Published: Tikrit University 2023-01-01
Series:Tikrit Journal of Pure Science
Subjects:
Online Access:https://tjpsj.org/index.php/tjps/article/view/630
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author Khalid M. Mohammad
Mohammad R. Ahmed
Mahmoud H. Mahmoud
author_facet Khalid M. Mohammad
Mohammad R. Ahmed
Mahmoud H. Mahmoud
author_sort Khalid M. Mohammad
collection DOAJ
description This research includes synthesis of new heterocyclic containing (1,3-oxazepine) derivatives of 6- methyl 2-thiouracil. The preparation process started by the reaction of 6- methyl 2-thiouracil with ethyl chloroacete to give ethyl 2-((4-hydroxy-6-methylpyrimidin-2-yl) thio) acetate (1). Compound (1) reacted with hydrazine hydrate to give 2-((4-hydroxy-6-methylpyrimidin-2-yl)thio) aceto hydrazide (2). That reacted with various substituted benzaldehydes in the presence of glacial acetic acid as catalyst in absolute ethanol to obtain new Schiff bases derivatives (3-11). The new 1,3-oxazepine derivatives [12-38] were obtained from treatment of each new Schiff bases derivatives (3-11) with each (phthalic anhydride ,maleic anhydride and succinic anhydride) respectively. Newly synthesized compounds were identified via spectral methods; their [FT-IR and some of them by 1H-NMR, 13C-NMR] and measurements of some of its physical properties. Furthermore some of the new compounds were screened for their antimicrobial activity against four strains of bacteria –ve (Escherichia coli and klibsialla) and +ve (Bacillus and Staphylococcus aureus). Most of the tested compounds show significant antibacterial activity.  
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publishDate 2023-01-01
publisher Tikrit University
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spelling doaj-art-4ee452c24f7d456a8131b7db187da0152025-08-20T03:16:51ZengTikrit UniversityTikrit Journal of Pure Science1813-16622415-17262023-01-0122210.25130/tjps.v22i2.630Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activityKhalid M. MohammadMohammad R. AhmedMahmoud H. Mahmoud This research includes synthesis of new heterocyclic containing (1,3-oxazepine) derivatives of 6- methyl 2-thiouracil. The preparation process started by the reaction of 6- methyl 2-thiouracil with ethyl chloroacete to give ethyl 2-((4-hydroxy-6-methylpyrimidin-2-yl) thio) acetate (1). Compound (1) reacted with hydrazine hydrate to give 2-((4-hydroxy-6-methylpyrimidin-2-yl)thio) aceto hydrazide (2). That reacted with various substituted benzaldehydes in the presence of glacial acetic acid as catalyst in absolute ethanol to obtain new Schiff bases derivatives (3-11). The new 1,3-oxazepine derivatives [12-38] were obtained from treatment of each new Schiff bases derivatives (3-11) with each (phthalic anhydride ,maleic anhydride and succinic anhydride) respectively. Newly synthesized compounds were identified via spectral methods; their [FT-IR and some of them by 1H-NMR, 13C-NMR] and measurements of some of its physical properties. Furthermore some of the new compounds were screened for their antimicrobial activity against four strains of bacteria –ve (Escherichia coli and klibsialla) and +ve (Bacillus and Staphylococcus aureus). Most of the tested compounds show significant antibacterial activity.   https://tjpsj.org/index.php/tjps/article/view/6306- methyl 2- thiouracilshichff bases1,3 oxazepin derivativeantibacterial
spellingShingle Khalid M. Mohammad
Mohammad R. Ahmed
Mahmoud H. Mahmoud
Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity
Tikrit Journal of Pure Science
6- methyl 2- thiouracil
shichff bases
1,3 oxazepin derivative
antibacterial
title Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity
title_full Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity
title_fullStr Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity
title_full_unstemmed Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity
title_short Synthesis and characterization of some new (1,3-Oxazepine) derivative from 6-methyl 2-thiouracil and study their biological activity
title_sort synthesis and characterization of some new 1 3 oxazepine derivative from 6 methyl 2 thiouracil and study their biological activity
topic 6- methyl 2- thiouracil
shichff bases
1,3 oxazepin derivative
antibacterial
url https://tjpsj.org/index.php/tjps/article/view/630
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AT mohammadrahmed synthesisandcharacterizationofsomenew13oxazepinederivativefrom6methyl2thiouracilandstudytheirbiologicalactivity
AT mahmoudhmahmoud synthesisandcharacterizationofsomenew13oxazepinederivativefrom6methyl2thiouracilandstudytheirbiologicalactivity