Microstructural and Magnetic Properties of Polyamide-Based Recycled Composites with Iron Oxide Nanoparticles

This study explores a sustainable approach to developing magnetic nanocomposites by synthesizing a mixed-phase iron oxide (IO) and recycled polyamide (RPA) composite from textile waste. The RPA/IO nanocomposite’s microstructural and magnetic properties were characterized using X-ray diffraction (XRD...

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Bibliographic Details
Main Authors: Lucas G. Dos Santos, Daina D. A. Buelvas, Daniel F. Valezi, Bruno L. S. Vicentin, Christian M. M. Rocha, Eduardo Di Mauro, Felipe de A. La Porta
Format: Article
Language:English
Published: MDPI AG 2025-02-01
Series:Magnetism
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Online Access:https://www.mdpi.com/2673-8724/5/1/5
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Summary:This study explores a sustainable approach to developing magnetic nanocomposites by synthesizing a mixed-phase iron oxide (IO) and recycled polyamide (RPA) composite from textile waste. The RPA/IO nanocomposite’s microstructural and magnetic properties were characterized using X-ray diffraction (XRD) with Rietveld refinement, scanning, transmission electron microscopy (SEM, TEM), and vibrating sample magnetometry (VSM). The proportions of the Fe<sub>3</sub>O<sub>4</sub> and γ-Fe<sub>2</sub>O<sub>3</sub> phases were found to be 23.2 wt% and 76.8 wt%, respectively. SEM and TEM showed a porous, agglomerated IO surface morphology with an average particle size of 14 nm. Magnetic analysis revealed ferrimagnetic and superparamagnetic behavior, with VSM showing saturation magnetization values of 21.81 emu g<sup>−1</sup> at 5 K and 18.84 emu g<sup>−1</sup> at 300 K. Anisotropy constants were estimated at 4.28 × 10<sup>5</sup> and 1.53 × 10<sup>5</sup>, respectively, for IO and the composite, with a blocking temperature of approximately 178 K at 300 K. These results contribute to understanding the magnetic behavior of IO and their nanocomposites, which is crucial for their potential applications in emerging technologies.
ISSN:2673-8724