An infrared, Raman, and X-ray database of battery interphase components

Abstract Further improvements to lithium-ion and emerging battery technologies can be enabled by an improved understanding of the chemistry and working mechanisms of interphases that form at electrochemically active battery interfaces. However, it is difficult to collect and interpret spectra of int...

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Main Authors: Lukas Karapin-Springorum, Asia Sarycheva, Andrew Dopilka, Hyungyeon Cha, Muhammad Ihsan-Ul-Haq, Jonathan M. Larson, Robert Kostecki
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Scientific Data
Online Access:https://doi.org/10.1038/s41597-024-04236-6
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author Lukas Karapin-Springorum
Asia Sarycheva
Andrew Dopilka
Hyungyeon Cha
Muhammad Ihsan-Ul-Haq
Jonathan M. Larson
Robert Kostecki
author_facet Lukas Karapin-Springorum
Asia Sarycheva
Andrew Dopilka
Hyungyeon Cha
Muhammad Ihsan-Ul-Haq
Jonathan M. Larson
Robert Kostecki
author_sort Lukas Karapin-Springorum
collection DOAJ
description Abstract Further improvements to lithium-ion and emerging battery technologies can be enabled by an improved understanding of the chemistry and working mechanisms of interphases that form at electrochemically active battery interfaces. However, it is difficult to collect and interpret spectra of interphases for several reasons, including the presence of a variety of compounds. To address this challenge, we herein present a vibrational spectroscopy and X-ray diffraction data library of ten compounds that have been identified as interphase constituents in lithium-ion or emerging battery chemistries. The data library includes attenuated total reflectance Fourier transform infrared spectroscopy, Raman spectroscopy, and X-ray diffraction data, collected in inert atmospheres provided by custom sample chambers. The data library presented in this work (and online repository) simplifies access to reference data that is otherwise either diffusely spread throughout the literature or non-existent, and provides energy storage researchers streamlined access to vital interphase-relevant data that can accelerate battery research efforts.
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spelling doaj-art-4e70343ff8614137a4da7147e7f1ec4a2025-08-20T02:40:39ZengNature PortfolioScientific Data2052-44632025-01-0112111910.1038/s41597-024-04236-6An infrared, Raman, and X-ray database of battery interphase componentsLukas Karapin-Springorum0Asia Sarycheva1Andrew Dopilka2Hyungyeon Cha3Muhammad Ihsan-Ul-Haq4Jonathan M. Larson5Robert Kostecki6Energy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage & Distributed Resources Division, Lawrence Berkeley National LaboratoryAbstract Further improvements to lithium-ion and emerging battery technologies can be enabled by an improved understanding of the chemistry and working mechanisms of interphases that form at electrochemically active battery interfaces. However, it is difficult to collect and interpret spectra of interphases for several reasons, including the presence of a variety of compounds. To address this challenge, we herein present a vibrational spectroscopy and X-ray diffraction data library of ten compounds that have been identified as interphase constituents in lithium-ion or emerging battery chemistries. The data library includes attenuated total reflectance Fourier transform infrared spectroscopy, Raman spectroscopy, and X-ray diffraction data, collected in inert atmospheres provided by custom sample chambers. The data library presented in this work (and online repository) simplifies access to reference data that is otherwise either diffusely spread throughout the literature or non-existent, and provides energy storage researchers streamlined access to vital interphase-relevant data that can accelerate battery research efforts.https://doi.org/10.1038/s41597-024-04236-6
spellingShingle Lukas Karapin-Springorum
Asia Sarycheva
Andrew Dopilka
Hyungyeon Cha
Muhammad Ihsan-Ul-Haq
Jonathan M. Larson
Robert Kostecki
An infrared, Raman, and X-ray database of battery interphase components
Scientific Data
title An infrared, Raman, and X-ray database of battery interphase components
title_full An infrared, Raman, and X-ray database of battery interphase components
title_fullStr An infrared, Raman, and X-ray database of battery interphase components
title_full_unstemmed An infrared, Raman, and X-ray database of battery interphase components
title_short An infrared, Raman, and X-ray database of battery interphase components
title_sort infrared raman and x ray database of battery interphase components
url https://doi.org/10.1038/s41597-024-04236-6
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