Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment

Technological solutions to address climate change are coalescing around renewable energy deployment. Yet, the deployment of renewables alone may not be sufficient to restrict temperature increases in line with Paris Agreement targets. The emergence of carbon negative technologies to bridge this shor...

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Main Authors: Tianhui Fan, Siyu Shen, Chun Yat (Benjamin) Sit, Paul J.A. Kenis, Andrew Chapman
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Journal of CO2 Utilization
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Online Access:http://www.sciencedirect.com/science/article/pii/S2212982024003378
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author Tianhui Fan
Siyu Shen
Chun Yat (Benjamin) Sit
Paul J.A. Kenis
Andrew Chapman
author_facet Tianhui Fan
Siyu Shen
Chun Yat (Benjamin) Sit
Paul J.A. Kenis
Andrew Chapman
author_sort Tianhui Fan
collection DOAJ
description Technological solutions to address climate change are coalescing around renewable energy deployment. Yet, the deployment of renewables alone may not be sufficient to restrict temperature increases in line with Paris Agreement targets. The emergence of carbon negative technologies to bridge this shortfall is needed and expected to overcome this gap. Among these technologies, direct air capture (DAC) is being deployed at multiple scales using various approaches. This study investigates membrane-based DAC integrated with subsequent carbon dioxide to carbon fuel conversion, i.e., DAC with utilization (DAC-U). The DAC-U evaluation is undertaken holistically, beginning with a cradle-to-grave life cycle assessment, followed by economic feasibility scenario analysis and social acceptability analysis to establish acceptable deployment pricing and necessary policy interventions. This study reveals that, although the DAC-U represents a carbon negative capable technology with positive lifestyle and environmental outcomes, high capital costs present a significant barrier to deployment. To overcome this barrier, a robust policy regime including subsidies or fuel credits may be necessary. Further technological innovation and efficiency gains will also close this gap, meaning that the membrane-based DAC-U concept may play a role in achieving carbon neutrality goals in the near future.
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spelling doaj-art-4d19ce8cb68145598e72f84f433d4f812025-01-13T04:18:50ZengElsevierJournal of CO2 Utilization2212-98392025-01-0191103002Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessmentTianhui Fan0Siyu Shen1Chun Yat (Benjamin) Sit2Paul J.A. Kenis3Andrew Chapman4Graduate School of Economics, Kyushu University, 744 Motooka Nishiku, Fukuoka 819-0395, JapanGraduate School of Economics, Kyushu University, 744 Motooka Nishiku, Fukuoka 819-0395, JapanDepartment of Chemical & Biomolecular Engineering, University of Illinois Urbana, Champaign 600 South Mathews Avenue, Urbana, IL 61801, USADepartment of Chemical & Biomolecular Engineering, University of Illinois Urbana, Champaign 600 South Mathews Avenue, Urbana, IL 61801, USA; International Institute for Carbon-Neutral Energy Research, Kyushu University, 744 Motooka Nishiku, Fukuoka 819-0395, JapanGraduate School of Economics, Kyushu University, 744 Motooka Nishiku, Fukuoka 819-0395, Japan; International Institute for Carbon-Neutral Energy Research, Kyushu University, 744 Motooka Nishiku, Fukuoka 819-0395, Japan; Corresponding author at: Graduate School of Economics, Kyushu University, 744 Motooka Nishiku, Fukuoka 819-0395, Japan.Technological solutions to address climate change are coalescing around renewable energy deployment. Yet, the deployment of renewables alone may not be sufficient to restrict temperature increases in line with Paris Agreement targets. The emergence of carbon negative technologies to bridge this shortfall is needed and expected to overcome this gap. Among these technologies, direct air capture (DAC) is being deployed at multiple scales using various approaches. This study investigates membrane-based DAC integrated with subsequent carbon dioxide to carbon fuel conversion, i.e., DAC with utilization (DAC-U). The DAC-U evaluation is undertaken holistically, beginning with a cradle-to-grave life cycle assessment, followed by economic feasibility scenario analysis and social acceptability analysis to establish acceptable deployment pricing and necessary policy interventions. This study reveals that, although the DAC-U represents a carbon negative capable technology with positive lifestyle and environmental outcomes, high capital costs present a significant barrier to deployment. To overcome this barrier, a robust policy regime including subsidies or fuel credits may be necessary. Further technological innovation and efficiency gains will also close this gap, meaning that the membrane-based DAC-U concept may play a role in achieving carbon neutrality goals in the near future.http://www.sciencedirect.com/science/article/pii/S2212982024003378DACLife cycle assessmentCarbon creditCarbon market
spellingShingle Tianhui Fan
Siyu Shen
Chun Yat (Benjamin) Sit
Paul J.A. Kenis
Andrew Chapman
Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment
Journal of CO2 Utilization
DAC
Life cycle assessment
Carbon credit
Carbon market
title Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment
title_full Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment
title_fullStr Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment
title_full_unstemmed Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment
title_short Environmental, economic and social trade-offs of membrane-based direct air capture technologies integrated with CO2 conversion using life cycle assessment
title_sort environmental economic and social trade offs of membrane based direct air capture technologies integrated with co2 conversion using life cycle assessment
topic DAC
Life cycle assessment
Carbon credit
Carbon market
url http://www.sciencedirect.com/science/article/pii/S2212982024003378
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AT chunyatbenjaminsit environmentaleconomicandsocialtradeoffsofmembranebaseddirectaircapturetechnologiesintegratedwithco2conversionusinglifecycleassessment
AT pauljakenis environmentaleconomicandsocialtradeoffsofmembranebaseddirectaircapturetechnologiesintegratedwithco2conversionusinglifecycleassessment
AT andrewchapman environmentaleconomicandsocialtradeoffsofmembranebaseddirectaircapturetechnologiesintegratedwithco2conversionusinglifecycleassessment