High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces

Abstract Superhydrophobic surfaces (SHS), with their exceptional water‐repellent properties, have attracted great interest due to their versatile applications. The robustness of SHS has emerged as an essential issue for practical applications, as SHS are directly exposed to various harsh environment...

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Main Authors: Jinpyeo Jeung, Inyeol Yun, Hyuk Park, Yoonyoung Chung
Format: Article
Language:English
Published: Wiley-VCH 2025-05-01
Series:Advanced Materials Interfaces
Subjects:
Online Access:https://doi.org/10.1002/admi.202400839
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author Jinpyeo Jeung
Inyeol Yun
Hyuk Park
Yoonyoung Chung
author_facet Jinpyeo Jeung
Inyeol Yun
Hyuk Park
Yoonyoung Chung
author_sort Jinpyeo Jeung
collection DOAJ
description Abstract Superhydrophobic surfaces (SHS), with their exceptional water‐repellent properties, have attracted great interest due to their versatile applications. The robustness of SHS has emerged as an essential issue for practical applications, as SHS are directly exposed to various harsh environments, such as continuous raindrop impact, corrosive media, and extreme temperatures. Polyimide (PI) is an ideal candidate for robust SHS due to its superior mechanical, thermal, and chemical properties. However, the low processability of PI in surface microstructuring has limited its application in SHS. In this study, a high‐yield and cost‐effective fabrication method for constructing high‐aspect‐ratio PI microstructures has been developed by controlling the template surface treatment, precursor molecular weight, and vacuum process. This approach achieves an exceptional yield rate of 99.8% and an aspect ratio of 10.7, enabling the construction of various microstructures. The SHS is demonstrated by fabricating microstructures on PI surfaces using the proposed method. The PI SHS exhibits a water contact angle of up to 162° and a roll‐off angle of less than 9°. The water repellency withstands 100 tape peeling tests and remains stable after continuous exposure to temperatures up to 250 °C and various chemical reagents for 60 days, which presents excellent robustness against environmental factors.
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spelling doaj-art-4b0ec2b6636748d7a8ee6181a1325b6a2025-08-20T01:53:37ZengWiley-VCHAdvanced Materials Interfaces2196-73502025-05-011210n/an/a10.1002/admi.202400839High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic SurfacesJinpyeo Jeung0Inyeol Yun1Hyuk Park2Yoonyoung Chung3Department of Electrical Engineering Pohang University of Science and Technology (POSTECH) 77 Cheongam‐ro Nam‐gu Pohang Gyeongbuk 37673 Republic of KoreaDepartment of Electrical Engineering Pohang University of Science and Technology (POSTECH) 77 Cheongam‐ro Nam‐gu Pohang Gyeongbuk 37673 Republic of KoreaDepartment of Electrical Engineering Pohang University of Science and Technology (POSTECH) 77 Cheongam‐ro Nam‐gu Pohang Gyeongbuk 37673 Republic of KoreaDepartment of Electrical Engineering Pohang University of Science and Technology (POSTECH) 77 Cheongam‐ro Nam‐gu Pohang Gyeongbuk 37673 Republic of KoreaAbstract Superhydrophobic surfaces (SHS), with their exceptional water‐repellent properties, have attracted great interest due to their versatile applications. The robustness of SHS has emerged as an essential issue for practical applications, as SHS are directly exposed to various harsh environments, such as continuous raindrop impact, corrosive media, and extreme temperatures. Polyimide (PI) is an ideal candidate for robust SHS due to its superior mechanical, thermal, and chemical properties. However, the low processability of PI in surface microstructuring has limited its application in SHS. In this study, a high‐yield and cost‐effective fabrication method for constructing high‐aspect‐ratio PI microstructures has been developed by controlling the template surface treatment, precursor molecular weight, and vacuum process. This approach achieves an exceptional yield rate of 99.8% and an aspect ratio of 10.7, enabling the construction of various microstructures. The SHS is demonstrated by fabricating microstructures on PI surfaces using the proposed method. The PI SHS exhibits a water contact angle of up to 162° and a roll‐off angle of less than 9°. The water repellency withstands 100 tape peeling tests and remains stable after continuous exposure to temperatures up to 250 °C and various chemical reagents for 60 days, which presents excellent robustness against environmental factors.https://doi.org/10.1002/admi.202400839high‐aspect‐ratiomoldingpolyimide microfabricationrobust superhydrophobic surfacessurface treatment
spellingShingle Jinpyeo Jeung
Inyeol Yun
Hyuk Park
Yoonyoung Chung
High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces
Advanced Materials Interfaces
high‐aspect‐ratio
molding
polyimide microfabrication
robust superhydrophobic surfaces
surface treatment
title High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces
title_full High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces
title_fullStr High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces
title_full_unstemmed High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces
title_short High‐Yield, Cost‐Effective Fabrication of High‐Aspect‐Ratio Polyimide Microstructures for Robust Superhydrophobic Surfaces
title_sort high yield cost effective fabrication of high aspect ratio polyimide microstructures for robust superhydrophobic surfaces
topic high‐aspect‐ratio
molding
polyimide microfabrication
robust superhydrophobic surfaces
surface treatment
url https://doi.org/10.1002/admi.202400839
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AT inyeolyun highyieldcosteffectivefabricationofhighaspectratiopolyimidemicrostructuresforrobustsuperhydrophobicsurfaces
AT hyukpark highyieldcosteffectivefabricationofhighaspectratiopolyimidemicrostructuresforrobustsuperhydrophobicsurfaces
AT yoonyoungchung highyieldcosteffectivefabricationofhighaspectratiopolyimidemicrostructuresforrobustsuperhydrophobicsurfaces