Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions

In this study, the efficiency of a low-cost K 2 CO 3 /Al 2 O 3 sorbent as a CO 2 capture support was investigated. The sorbent was prepared by impregnating K 2 CO 3 on industrial-grade Al 2 O 3 . The CO 2 capture capacity of the sorbent was calculated from the breakthrough curve of the CO 2 adsorpti...

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Main Authors: Javad Esmaili, Mohammad Reza Ehsani
Format: Article
Language:English
Published: SAGE Publishing 2013-08-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1260/0263-6174.31.8.683
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author Javad Esmaili
Mohammad Reza Ehsani
author_facet Javad Esmaili
Mohammad Reza Ehsani
author_sort Javad Esmaili
collection DOAJ
description In this study, the efficiency of a low-cost K 2 CO 3 /Al 2 O 3 sorbent as a CO 2 capture support was investigated. The sorbent was prepared by impregnating K 2 CO 3 on industrial-grade Al 2 O 3 . The CO 2 capture capacity of the sorbent was calculated from the breakthrough curve of the CO 2 adsorption inside a fixed-bed reactor, in the presence of H 2 O and at an adsorption temperature of 60 °C. An adsorption capacity of 75.4 mg CO 2 /g of sorbent was obtained. The stability of capture capacity of the sorbent was higher than that of the reference sorbent. The changes in the pore volume and surface area were 0.020 cm 3 /g and 5.5 m 2 /g, respectively, after five cycles of adsorption and regeneration. However, there were minor changes in the pore-size distribution and surface area of the sorbent after five cycles. This sorbent can be considered to be used in large-scale applications.
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institution Kabale University
issn 0263-6174
2048-4038
language English
publishDate 2013-08-01
publisher SAGE Publishing
record_format Article
series Adsorption Science & Technology
spelling doaj-art-490cb67c8df4437db2dbd8a92be6328b2025-01-03T00:10:29ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382013-08-013110.1260/0263-6174.31.8.683Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating ConditionsJavad EsmailiMohammad Reza EhsaniIn this study, the efficiency of a low-cost K 2 CO 3 /Al 2 O 3 sorbent as a CO 2 capture support was investigated. The sorbent was prepared by impregnating K 2 CO 3 on industrial-grade Al 2 O 3 . The CO 2 capture capacity of the sorbent was calculated from the breakthrough curve of the CO 2 adsorption inside a fixed-bed reactor, in the presence of H 2 O and at an adsorption temperature of 60 °C. An adsorption capacity of 75.4 mg CO 2 /g of sorbent was obtained. The stability of capture capacity of the sorbent was higher than that of the reference sorbent. The changes in the pore volume and surface area were 0.020 cm 3 /g and 5.5 m 2 /g, respectively, after five cycles of adsorption and regeneration. However, there were minor changes in the pore-size distribution and surface area of the sorbent after five cycles. This sorbent can be considered to be used in large-scale applications.https://doi.org/10.1260/0263-6174.31.8.683
spellingShingle Javad Esmaili
Mohammad Reza Ehsani
Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
Adsorption Science & Technology
title Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
title_full Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
title_fullStr Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
title_full_unstemmed Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
title_short Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
title_sort preparation of a low cost kco alo sorbent for co capture at flue gas operating conditions
url https://doi.org/10.1260/0263-6174.31.8.683
work_keys_str_mv AT javadesmaili preparationofalowcostkcoalosorbentforcocaptureatfluegasoperatingconditions
AT mohammadrezaehsani preparationofalowcostkcoalosorbentforcocaptureatfluegasoperatingconditions