Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions
In this study, the efficiency of a low-cost K 2 CO 3 /Al 2 O 3 sorbent as a CO 2 capture support was investigated. The sorbent was prepared by impregnating K 2 CO 3 on industrial-grade Al 2 O 3 . The CO 2 capture capacity of the sorbent was calculated from the breakthrough curve of the CO 2 adsorpti...
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SAGE Publishing
2013-08-01
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Series: | Adsorption Science & Technology |
Online Access: | https://doi.org/10.1260/0263-6174.31.8.683 |
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author | Javad Esmaili Mohammad Reza Ehsani |
author_facet | Javad Esmaili Mohammad Reza Ehsani |
author_sort | Javad Esmaili |
collection | DOAJ |
description | In this study, the efficiency of a low-cost K 2 CO 3 /Al 2 O 3 sorbent as a CO 2 capture support was investigated. The sorbent was prepared by impregnating K 2 CO 3 on industrial-grade Al 2 O 3 . The CO 2 capture capacity of the sorbent was calculated from the breakthrough curve of the CO 2 adsorption inside a fixed-bed reactor, in the presence of H 2 O and at an adsorption temperature of 60 °C. An adsorption capacity of 75.4 mg CO 2 /g of sorbent was obtained. The stability of capture capacity of the sorbent was higher than that of the reference sorbent. The changes in the pore volume and surface area were 0.020 cm 3 /g and 5.5 m 2 /g, respectively, after five cycles of adsorption and regeneration. However, there were minor changes in the pore-size distribution and surface area of the sorbent after five cycles. This sorbent can be considered to be used in large-scale applications. |
format | Article |
id | doaj-art-490cb67c8df4437db2dbd8a92be6328b |
institution | Kabale University |
issn | 0263-6174 2048-4038 |
language | English |
publishDate | 2013-08-01 |
publisher | SAGE Publishing |
record_format | Article |
series | Adsorption Science & Technology |
spelling | doaj-art-490cb67c8df4437db2dbd8a92be6328b2025-01-03T00:10:29ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382013-08-013110.1260/0263-6174.31.8.683Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating ConditionsJavad EsmailiMohammad Reza EhsaniIn this study, the efficiency of a low-cost K 2 CO 3 /Al 2 O 3 sorbent as a CO 2 capture support was investigated. The sorbent was prepared by impregnating K 2 CO 3 on industrial-grade Al 2 O 3 . The CO 2 capture capacity of the sorbent was calculated from the breakthrough curve of the CO 2 adsorption inside a fixed-bed reactor, in the presence of H 2 O and at an adsorption temperature of 60 °C. An adsorption capacity of 75.4 mg CO 2 /g of sorbent was obtained. The stability of capture capacity of the sorbent was higher than that of the reference sorbent. The changes in the pore volume and surface area were 0.020 cm 3 /g and 5.5 m 2 /g, respectively, after five cycles of adsorption and regeneration. However, there were minor changes in the pore-size distribution and surface area of the sorbent after five cycles. This sorbent can be considered to be used in large-scale applications.https://doi.org/10.1260/0263-6174.31.8.683 |
spellingShingle | Javad Esmaili Mohammad Reza Ehsani Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions Adsorption Science & Technology |
title | Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions |
title_full | Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions |
title_fullStr | Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions |
title_full_unstemmed | Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions |
title_short | Preparation of a Low-Cost KCO/AlO Sorbent for CO Capture at Flue-Gas Operating Conditions |
title_sort | preparation of a low cost kco alo sorbent for co capture at flue gas operating conditions |
url | https://doi.org/10.1260/0263-6174.31.8.683 |
work_keys_str_mv | AT javadesmaili preparationofalowcostkcoalosorbentforcocaptureatfluegasoperatingconditions AT mohammadrezaehsani preparationofalowcostkcoalosorbentforcocaptureatfluegasoperatingconditions |