Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries

ABSTRACT Lithium–carbon dioxide (Li–CO2) batteries with high theoretical energy density are regarded as promising energy storage system toward carbon neutrality. However, bidirectional catalysts design for improving the sluggish CO2 reduction reaction (CO2RR)/CO2 evolution reaction (CO2ER) kinetics...

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Main Authors: Yanze Song, Bingyi Lu, Zhiwen Min, Haotian Qu, Yingqi Liu, Rui Mao, Yanli Chen, Yuanmiao Sun, Guangmin Zhou
Format: Article
Language:English
Published: Wiley 2025-05-01
Series:Carbon Energy
Subjects:
Online Access:https://doi.org/10.1002/cey2.692
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author Yanze Song
Bingyi Lu
Zhiwen Min
Haotian Qu
Yingqi Liu
Rui Mao
Yanli Chen
Yuanmiao Sun
Guangmin Zhou
author_facet Yanze Song
Bingyi Lu
Zhiwen Min
Haotian Qu
Yingqi Liu
Rui Mao
Yanli Chen
Yuanmiao Sun
Guangmin Zhou
author_sort Yanze Song
collection DOAJ
description ABSTRACT Lithium–carbon dioxide (Li–CO2) batteries with high theoretical energy density are regarded as promising energy storage system toward carbon neutrality. However, bidirectional catalysts design for improving the sluggish CO2 reduction reaction (CO2RR)/CO2 evolution reaction (CO2ER) kinetics remains a huge challenge. In this work, an advanced catalyst with fast‐interfacial charge transfer was subtly synthesized through element segregation, which significantly improves the electrocatalytic activity for both CO2RR and CO2ER. Theoretical calculations and characterization analysis demonstrate local charge redistribution at the constructed interface, which leads to optimized binding affinity towards reactants and preferred Li2CO3 decomposition behavior, enabling excellent catalytic activity during CO2 redox. Benefiting from the enhanced charge transfer ability, the designed highly efficient catalyst with dual active centers and large exposed catalytic area can maintain an ultra‐small voltage gap of 0.33 V and high energy efficiency of 90.2%. This work provides an attractive strategy to construct robust catalysts by interface engineering, which could inspire further design of superior bidirectional catalysts for Li–CO2 batteries.
format Article
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institution DOAJ
issn 2637-9368
language English
publishDate 2025-05-01
publisher Wiley
record_format Article
series Carbon Energy
spelling doaj-art-48d9d91f8eca49faa739b443f9388fc32025-08-20T03:12:45ZengWileyCarbon Energy2637-93682025-05-0175n/an/a10.1002/cey2.692Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 BatteriesYanze Song0Bingyi Lu1Zhiwen Min2Haotian Qu3Yingqi Liu4Rui Mao5Yanli Chen6Yuanmiao Sun7Guangmin Zhou8Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaTsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaFaculty of Materials Science and Energy Engineering/Institute of Technology for Carbon Neutrality, Shenzhen Institute of Advanced Technology Chinese Academy of Sciences Shenzhen ChinaTsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaTsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaTsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaTsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaFaculty of Materials Science and Energy Engineering/Institute of Technology for Carbon Neutrality, Shenzhen Institute of Advanced Technology Chinese Academy of Sciences Shenzhen ChinaTsinghua Shenzhen International Graduate School Tsinghua University Shenzhen ChinaABSTRACT Lithium–carbon dioxide (Li–CO2) batteries with high theoretical energy density are regarded as promising energy storage system toward carbon neutrality. However, bidirectional catalysts design for improving the sluggish CO2 reduction reaction (CO2RR)/CO2 evolution reaction (CO2ER) kinetics remains a huge challenge. In this work, an advanced catalyst with fast‐interfacial charge transfer was subtly synthesized through element segregation, which significantly improves the electrocatalytic activity for both CO2RR and CO2ER. Theoretical calculations and characterization analysis demonstrate local charge redistribution at the constructed interface, which leads to optimized binding affinity towards reactants and preferred Li2CO3 decomposition behavior, enabling excellent catalytic activity during CO2 redox. Benefiting from the enhanced charge transfer ability, the designed highly efficient catalyst with dual active centers and large exposed catalytic area can maintain an ultra‐small voltage gap of 0.33 V and high energy efficiency of 90.2%. This work provides an attractive strategy to construct robust catalysts by interface engineering, which could inspire further design of superior bidirectional catalysts for Li–CO2 batteries.https://doi.org/10.1002/cey2.692electronic redistributioninterface engineeringLi2CO3 decompositionLi–CO2 battery
spellingShingle Yanze Song
Bingyi Lu
Zhiwen Min
Haotian Qu
Yingqi Liu
Rui Mao
Yanli Chen
Yuanmiao Sun
Guangmin Zhou
Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries
Carbon Energy
electronic redistribution
interface engineering
Li2CO3 decomposition
Li–CO2 battery
title Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries
title_full Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries
title_fullStr Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries
title_full_unstemmed Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries
title_short Interface Engineering Toward Surface‐Activated Catalysts for Advanced Li–CO2 Batteries
title_sort interface engineering toward surface activated catalysts for advanced li co2 batteries
topic electronic redistribution
interface engineering
Li2CO3 decomposition
Li–CO2 battery
url https://doi.org/10.1002/cey2.692
work_keys_str_mv AT yanzesong interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT bingyilu interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT zhiwenmin interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT haotianqu interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT yingqiliu interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT ruimao interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT yanlichen interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
AT yuanmiaosun interfaceengineeringtowardsurfaceactivatedcatalystsforadvancedlico2batteries
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