Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling

The present work introduces a quantitative structure-property relationship (QSPR)-based stochastic gradient boosting (SGB) decision tree framework for simulating and capturing of the thermal decomposition kinetics of biomass considering effective parameters of the ultimate analysis (such as carbon,...

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Main Authors: Lei Dong, RanRan Wang, PeiDe Liu, Saeed Sarvazizi
Format: Article
Language:English
Published: Wiley 2022-01-01
Series:International Journal of Chemical Engineering
Online Access:http://dx.doi.org/10.1155/2022/6491745
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author Lei Dong
RanRan Wang
PeiDe Liu
Saeed Sarvazizi
author_facet Lei Dong
RanRan Wang
PeiDe Liu
Saeed Sarvazizi
author_sort Lei Dong
collection DOAJ
description The present work introduces a quantitative structure-property relationship (QSPR)-based stochastic gradient boosting (SGB) decision tree framework for simulating and capturing of the thermal decomposition kinetics of biomass considering effective parameters of the ultimate analysis (such as carbon, hydrogen, oxygen, nitrogen, and sulfur content) and process heating rate. Through a total of 149 pyrolysis kinetics, this study developed an artificial model and subjected it to training and testing phases. The proposed model was validated using error analysis, sensitivity, regression, and outlier detection. The coefficient of determination (R2) and mean relative error (%MRE) were calculated to be 0.993 and 4.354%, respectively, suggesting good performance in the estimation of the pyrolysis kinetic parameters. Also, the sensitivity results indicated the process heating rate to have the strongest effect on the model output with a relevancy factor of 0.43. Eventually, the proposed model showed superior performance compared to earlier frameworks.
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institution OA Journals
issn 1687-8078
language English
publishDate 2022-01-01
publisher Wiley
record_format Article
series International Journal of Chemical Engineering
spelling doaj-art-482014af53d64b14a2488cfcda5b8e582025-08-20T02:38:01ZengWileyInternational Journal of Chemical Engineering1687-80782022-01-01202210.1155/2022/6491745Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based ModelingLei Dong0RanRan Wang1PeiDe Liu2Saeed Sarvazizi3Department of Mechanical EngineeringAviation Service DepartmentYantai Lutong Precision Technology Co.,Ltd.Department of Petroleum EngineeringThe present work introduces a quantitative structure-property relationship (QSPR)-based stochastic gradient boosting (SGB) decision tree framework for simulating and capturing of the thermal decomposition kinetics of biomass considering effective parameters of the ultimate analysis (such as carbon, hydrogen, oxygen, nitrogen, and sulfur content) and process heating rate. Through a total of 149 pyrolysis kinetics, this study developed an artificial model and subjected it to training and testing phases. The proposed model was validated using error analysis, sensitivity, regression, and outlier detection. The coefficient of determination (R2) and mean relative error (%MRE) were calculated to be 0.993 and 4.354%, respectively, suggesting good performance in the estimation of the pyrolysis kinetic parameters. Also, the sensitivity results indicated the process heating rate to have the strongest effect on the model output with a relevancy factor of 0.43. Eventually, the proposed model showed superior performance compared to earlier frameworks.http://dx.doi.org/10.1155/2022/6491745
spellingShingle Lei Dong
RanRan Wang
PeiDe Liu
Saeed Sarvazizi
Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling
International Journal of Chemical Engineering
title Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling
title_full Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling
title_fullStr Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling
title_full_unstemmed Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling
title_short Prediction of Pyrolysis Kinetics of Biomass: New Insights from Artificial Intelligence-Based Modeling
title_sort prediction of pyrolysis kinetics of biomass new insights from artificial intelligence based modeling
url http://dx.doi.org/10.1155/2022/6491745
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AT ranranwang predictionofpyrolysiskineticsofbiomassnewinsightsfromartificialintelligencebasedmodeling
AT peideliu predictionofpyrolysiskineticsofbiomassnewinsightsfromartificialintelligencebasedmodeling
AT saeedsarvazizi predictionofpyrolysiskineticsofbiomassnewinsightsfromartificialintelligencebasedmodeling