Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>

<i>Sanghuangporous vaninii</i>, as an edible and medicinal macrofungus, represents a high source of polyphenols with considerable antioxidant activities. However, due to the significant differences in polyphenol content and bioactivity caused by different cultivation substrates, its anti...

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Main Authors: Peng Liu, Yuyang Wang, Daoyou Chen, Zhengpeng Li, Di Wu, Zhong Zhang, Wanchao Chen, Wen Li, Yan Yang
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Antioxidants
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Online Access:https://www.mdpi.com/2076-3921/13/12/1487
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author Peng Liu
Yuyang Wang
Daoyou Chen
Zhengpeng Li
Di Wu
Zhong Zhang
Wanchao Chen
Wen Li
Yan Yang
author_facet Peng Liu
Yuyang Wang
Daoyou Chen
Zhengpeng Li
Di Wu
Zhong Zhang
Wanchao Chen
Wen Li
Yan Yang
author_sort Peng Liu
collection DOAJ
description <i>Sanghuangporous vaninii</i>, as an edible and medicinal macrofungus, represents a high source of polyphenols with considerable antioxidant activities. However, due to the significant differences in polyphenol content and bioactivity caused by different cultivation substrates, its antioxidant mechanism has not been fully determined. In this paper, five groups of <i>S. vaninii</i> fruiting bodies were collected from cultivation substrates from different areas. The ethanol extracts of mulberry sawdust from Haining City (HNMS) had the highest polyphenol content, as well as excellent antioxidant activity. HNMS3, a polyphenol component with promising antioxidant capacity, was further isolated through optimization with different extractants, silica gel column chromatography, and thin layer chromatography analysis. UPLC-Q-TOF-MS analysis showed that HNMS3 was composed of 33 compounds, corresponding to 257 targets of oxidative stress by network pharmacology analysis, which were strongly associated with mental health and neurodegenerative diseases. Protein–protein interaction and molecular docking analysis indicated that eight hub genes (PPARG, IL-6, STAT3, PTGS2, SRC, MTOR, ERS1, and EGFR) are attributed to the regulation of the key compounds hispidin, inoscavin A, inoscavin_C, and phellibaumin B. Consequently, this study obtains <i>S. vaninii</i> polyphenolic component HNMS3 with excellent antioxidant capacity, simultaneously revealing its potential antioxidant mechanisms, providing new insights into the application of <i>S. vaninii</i>.
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spelling doaj-art-48140f030af74f9b8ec651b28cddfe9e2025-08-20T02:01:01ZengMDPI AGAntioxidants2076-39212024-12-011312148710.3390/antiox13121487Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>Peng Liu0Yuyang Wang1Daoyou Chen2Zhengpeng Li3Di Wu4Zhong Zhang5Wanchao Chen6Wen Li7Yan Yang8Institute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaShanghai Engineering Research Center of Molecular Therapeutics and New Drug Development, School of Chemistry and Molecular Engineering, East China Normal University, Shanghai 200062, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, ChinaInstitute of Edible Fungi, Shanghai Academy of Agricultural Sciences, Key Laboratory of Edible Fungi Resources and Utilization (South), Ministry of Agriculture, National Engineering Research Center of Edible Fungi, Shanghai 201403, China<i>Sanghuangporous vaninii</i>, as an edible and medicinal macrofungus, represents a high source of polyphenols with considerable antioxidant activities. However, due to the significant differences in polyphenol content and bioactivity caused by different cultivation substrates, its antioxidant mechanism has not been fully determined. In this paper, five groups of <i>S. vaninii</i> fruiting bodies were collected from cultivation substrates from different areas. The ethanol extracts of mulberry sawdust from Haining City (HNMS) had the highest polyphenol content, as well as excellent antioxidant activity. HNMS3, a polyphenol component with promising antioxidant capacity, was further isolated through optimization with different extractants, silica gel column chromatography, and thin layer chromatography analysis. UPLC-Q-TOF-MS analysis showed that HNMS3 was composed of 33 compounds, corresponding to 257 targets of oxidative stress by network pharmacology analysis, which were strongly associated with mental health and neurodegenerative diseases. Protein–protein interaction and molecular docking analysis indicated that eight hub genes (PPARG, IL-6, STAT3, PTGS2, SRC, MTOR, ERS1, and EGFR) are attributed to the regulation of the key compounds hispidin, inoscavin A, inoscavin_C, and phellibaumin B. Consequently, this study obtains <i>S. vaninii</i> polyphenolic component HNMS3 with excellent antioxidant capacity, simultaneously revealing its potential antioxidant mechanisms, providing new insights into the application of <i>S. vaninii</i>.https://www.mdpi.com/2076-3921/13/12/1487<i>Sanghuangporous vaninii</i>polyphenolsantioxidant activityisolationnetwork pharmacology
spellingShingle Peng Liu
Yuyang Wang
Daoyou Chen
Zhengpeng Li
Di Wu
Zhong Zhang
Wanchao Chen
Wen Li
Yan Yang
Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>
Antioxidants
<i>Sanghuangporous vaninii</i>
polyphenols
antioxidant activity
isolation
network pharmacology
title Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>
title_full Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>
title_fullStr Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>
title_full_unstemmed Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>
title_short Isolation and Antioxidant Mechanism of Polyphenols from <i>Sanghuangporous vaninii</i>
title_sort isolation and antioxidant mechanism of polyphenols from i sanghuangporous vaninii i
topic <i>Sanghuangporous vaninii</i>
polyphenols
antioxidant activity
isolation
network pharmacology
url https://www.mdpi.com/2076-3921/13/12/1487
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