Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems

Effective thermal management is critical to mitigating thermal runaway risks, optimizing performance, and extending the operational lifespan of lithium-ion batteries (LIBs) in high-rate applications. This study systematically evaluates four thermal management strategies for a 14.6 Ah LIB under aggre...

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Main Authors: Saeed Rahmanian, Hossein Rahmanian-Koushkaki, Khashayar Hosseinzadeh
Format: Article
Language:English
Published: Elsevier 2025-10-01
Series:Case Studies in Thermal Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2214157X25010317
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author Saeed Rahmanian
Hossein Rahmanian-Koushkaki
Khashayar Hosseinzadeh
author_facet Saeed Rahmanian
Hossein Rahmanian-Koushkaki
Khashayar Hosseinzadeh
author_sort Saeed Rahmanian
collection DOAJ
description Effective thermal management is critical to mitigating thermal runaway risks, optimizing performance, and extending the operational lifespan of lithium-ion batteries (LIBs) in high-rate applications. This study systematically evaluates four thermal management strategies for a 14.6 Ah LIB under aggressive discharge currents (1C, 3C, 5C): (1) baseline (no thermal control), (2) phase change material (PCM) with thickness variations, (3) hybrid PCM-K-enhancer (copper foam, graphene, metal plates) systems, and (4) active cooling (heat pipes + forced air convection). High-fidelity 3D simulations in ANSYS Fluent V22 quantified temperature uniformity, peak temperature suppression, and transient phase change behavior.At 5C discharge, baseline tests revealed unsafe peak temperatures of 84.03 °C. PCM thickness optimization demonstrated a nonlinear cooling effect: 1 mm PCM reduced peak temperature to 66.91 °C, while 3 mm PCM achieved 55.38 °C, underscoring the role of latent heat capacity scaling. Graphene-based K-enhancers outperformed copper foam and metal plates, synergizing with PCM to limit temperatures to 47.82 °C through thermal bridging. Synergistic integration of optimized PCM thickness (2 mm), graphene-enhanced thermal bridges, and heat-pipe cooling achieved a 53.3 % temperature reduction vs. baseline (39.23 °C).The study introduces a hierarchical thermal management framework, demonstrating that hybrid systems integrating optimized PCM thickness, graphene-enhanced interfacial conductivity, and active cooling achieve superior thermal equilibrium. These findings advance the design of multi-scale thermal regulation strategies for high-power LIB packs in electric vehicles.
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spelling doaj-art-4751f81dc2b74d70b5e87e1cb64deea52025-08-20T03:16:12ZengElsevierCase Studies in Thermal Engineering2214-157X2025-10-017410677110.1016/j.csite.2025.106771Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systemsSaeed Rahmanian0Hossein Rahmanian-Koushkaki1Khashayar Hosseinzadeh2Department of Mechanical Engineering, Engineering Faculty, Jahrom University, Jahrom, Iran; Corresponding author.Department of Mechanical Engineering of Biosystems, Agriculture Faculty, Jahrom University, Jahrom, IranDepartment of Mechanical Engineering, University of Mazandaran, Babolsar, Iran; Corresponding author.Effective thermal management is critical to mitigating thermal runaway risks, optimizing performance, and extending the operational lifespan of lithium-ion batteries (LIBs) in high-rate applications. This study systematically evaluates four thermal management strategies for a 14.6 Ah LIB under aggressive discharge currents (1C, 3C, 5C): (1) baseline (no thermal control), (2) phase change material (PCM) with thickness variations, (3) hybrid PCM-K-enhancer (copper foam, graphene, metal plates) systems, and (4) active cooling (heat pipes + forced air convection). High-fidelity 3D simulations in ANSYS Fluent V22 quantified temperature uniformity, peak temperature suppression, and transient phase change behavior.At 5C discharge, baseline tests revealed unsafe peak temperatures of 84.03 °C. PCM thickness optimization demonstrated a nonlinear cooling effect: 1 mm PCM reduced peak temperature to 66.91 °C, while 3 mm PCM achieved 55.38 °C, underscoring the role of latent heat capacity scaling. Graphene-based K-enhancers outperformed copper foam and metal plates, synergizing with PCM to limit temperatures to 47.82 °C through thermal bridging. Synergistic integration of optimized PCM thickness (2 mm), graphene-enhanced thermal bridges, and heat-pipe cooling achieved a 53.3 % temperature reduction vs. baseline (39.23 °C).The study introduces a hierarchical thermal management framework, demonstrating that hybrid systems integrating optimized PCM thickness, graphene-enhanced interfacial conductivity, and active cooling achieve superior thermal equilibrium. These findings advance the design of multi-scale thermal regulation strategies for high-power LIB packs in electric vehicles.http://www.sciencedirect.com/science/article/pii/S2214157X25010317Lithium batteryBattery thermal managementPhase change materialsHeat pipeModel NTGK
spellingShingle Saeed Rahmanian
Hossein Rahmanian-Koushkaki
Khashayar Hosseinzadeh
Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems
Case Studies in Thermal Engineering
Lithium battery
Battery thermal management
Phase change materials
Heat pipe
Model NTGK
title Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems
title_full Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems
title_fullStr Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems
title_full_unstemmed Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems
title_short Thermal management in high-power lithium-ion Batteries: Synergistic effects of phase change material thickness, graphene enhancers, and active cooling systems
title_sort thermal management in high power lithium ion batteries synergistic effects of phase change material thickness graphene enhancers and active cooling systems
topic Lithium battery
Battery thermal management
Phase change materials
Heat pipe
Model NTGK
url http://www.sciencedirect.com/science/article/pii/S2214157X25010317
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AT hosseinrahmaniankoushkaki thermalmanagementinhighpowerlithiumionbatteriessynergisticeffectsofphasechangematerialthicknessgrapheneenhancersandactivecoolingsystems
AT khashayarhosseinzadeh thermalmanagementinhighpowerlithiumionbatteriessynergisticeffectsofphasechangematerialthicknessgrapheneenhancersandactivecoolingsystems