Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers

Toughened epoxy has been widely used in industrial areas such as automotive and electronics. In this study, nanosized hyperbranched polymers (HBPs) as a flexibilizer are synthesized and embedded into epoxy resin to enhance the toughness and flexibility. Two different HBPs, hyperbranched poly(methyla...

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Main Authors: Hangyu Park, Youngson Choe
Format: Article
Language:English
Published: Wiley 2021-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2021/9984174
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author Hangyu Park
Youngson Choe
author_facet Hangyu Park
Youngson Choe
author_sort Hangyu Park
collection DOAJ
description Toughened epoxy has been widely used in industrial areas such as automotive and electronics. In this study, nanosized hyperbranched polymers (HBPs) as a flexibilizer are synthesized and embedded into epoxy resin to enhance the toughness and flexibility. Two different HBPs, hyperbranched poly(methylacrylate-diethanolamine) (poly(MA-DEA)) and poly(methylacrylate- ethanolamine) (poly(MA-EA)), were prepared and blended with both epoxy and polyetheramine, a curing agent. The molecular size of HBPs was estimated to be 6 ~ 14 nm in diameter. The molecular weight of HBPs ranges from 1500(1.5 K) to 7000(7.0 K) g/mol. In cured epoxy/HBP blends, no phase separations are occurred, indicating that HBPs possess sufficient miscibility with epoxy. The tensile toughness of the blends increased with changing the molecular weight of HBPs without sacrificing tensile strengths. The impact strength of the blends increases stiffly until the loading % of HBPs in the blends reaches 10 wt%. In addition, the experimental studies showed that impact resistance also increased with an increase in molecular weight of HBPs. The obtained impact resistance of the epoxy/HBP blends with 10 wt% was 270% more effective compared to that of cured neat epoxy.
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spelling doaj-art-46f464a1efbd4c5ea46c273de434fed22025-08-20T03:36:45ZengWileyInternational Journal of Polymer Science1687-94302021-01-01202110.1155/2021/9984174Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched PolymersHangyu Park0Youngson Choe1Department of Polymer Science and Chemical EngineeringDepartment of Polymer Science and Chemical EngineeringToughened epoxy has been widely used in industrial areas such as automotive and electronics. In this study, nanosized hyperbranched polymers (HBPs) as a flexibilizer are synthesized and embedded into epoxy resin to enhance the toughness and flexibility. Two different HBPs, hyperbranched poly(methylacrylate-diethanolamine) (poly(MA-DEA)) and poly(methylacrylate- ethanolamine) (poly(MA-EA)), were prepared and blended with both epoxy and polyetheramine, a curing agent. The molecular size of HBPs was estimated to be 6 ~ 14 nm in diameter. The molecular weight of HBPs ranges from 1500(1.5 K) to 7000(7.0 K) g/mol. In cured epoxy/HBP blends, no phase separations are occurred, indicating that HBPs possess sufficient miscibility with epoxy. The tensile toughness of the blends increased with changing the molecular weight of HBPs without sacrificing tensile strengths. The impact strength of the blends increases stiffly until the loading % of HBPs in the blends reaches 10 wt%. In addition, the experimental studies showed that impact resistance also increased with an increase in molecular weight of HBPs. The obtained impact resistance of the epoxy/HBP blends with 10 wt% was 270% more effective compared to that of cured neat epoxy.http://dx.doi.org/10.1155/2021/9984174
spellingShingle Hangyu Park
Youngson Choe
Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers
International Journal of Polymer Science
title Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers
title_full Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers
title_fullStr Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers
title_full_unstemmed Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers
title_short Enhancing Toughness and Impact Strength of Epoxy Resins by Using Hyperbranched Polymers
title_sort enhancing toughness and impact strength of epoxy resins by using hyperbranched polymers
url http://dx.doi.org/10.1155/2021/9984174
work_keys_str_mv AT hangyupark enhancingtoughnessandimpactstrengthofepoxyresinsbyusinghyperbranchedpolymers
AT youngsonchoe enhancingtoughnessandimpactstrengthofepoxyresinsbyusinghyperbranchedpolymers