Synthesis and Application of Nanomagnetic Immobilized Phospholipase C

The nanomagnetic carrier (Fe3O4@SiO2@p(GMA)) was prepared by atom transfer radical polymerization, and then, the free phospholipase C (PLC) was immobilized on it proved by the results of FT-IR analysis. The enzyme loading was 135.64 mg/g, the enzyme activity was 8560.7 U/g, the average particle size...

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Main Authors: Yang Jiang, Jing Du, Honglin Tang, Xin Zhang, Wenbin Li, Liqi Wang, Lianzhou Jiang, Dianyu Yu
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2019/5951793
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author Yang Jiang
Jing Du
Honglin Tang
Xin Zhang
Wenbin Li
Liqi Wang
Lianzhou Jiang
Dianyu Yu
author_facet Yang Jiang
Jing Du
Honglin Tang
Xin Zhang
Wenbin Li
Liqi Wang
Lianzhou Jiang
Dianyu Yu
author_sort Yang Jiang
collection DOAJ
description The nanomagnetic carrier (Fe3O4@SiO2@p(GMA)) was prepared by atom transfer radical polymerization, and then, the free phospholipase C (PLC) was immobilized on it proved by the results of FT-IR analysis. The enzyme loading was 135.64 mg/g, the enzyme activity was 8560.7 U/g, the average particle size was 99.86 ± 0.80 nm, and the specific saturation magnetization was 16.00 ± 0.20 emu/g. PLC-Fe3O4@SiO2@p(GMA) showed the highest activities at the pH of 7.5, and tolerance temperature raised to 65°C in soybean lecithin emulsion. Enzymatic degumming with PLC-Fe3O4@SiO2@p(GMA) under the conditions of the enzyme dosage of 110 mg/kg, reaction temperature of 65°C, pH of 7.5, and reaction time of 2.5 h resulted in residual phosphorus of 64.7 mg/kg, 1,2-diacylglycerol (1,2-DAG) contents of 1.07%, and oil yield of 98.1%. Moreover, PLC-Fe3O4@SiO2@p(GMA) still possessed more than 80% of its initial activity after 5 cycles.
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institution Kabale University
issn 2090-9063
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language English
publishDate 2019-01-01
publisher Wiley
record_format Article
series Journal of Chemistry
spelling doaj-art-4696a040f8ba459bb9b1c8e5af82bdab2025-08-20T03:36:13ZengWileyJournal of Chemistry2090-90632090-90712019-01-01201910.1155/2019/59517935951793Synthesis and Application of Nanomagnetic Immobilized Phospholipase CYang Jiang0Jing Du1Honglin Tang2Xin Zhang3Wenbin Li4Liqi Wang5Lianzhou Jiang6Dianyu Yu7School of Food Science, Northeast Agricultural University, Harbin 150030, ChinaThe Key Laboratory of Soybean Biology in Chinese Ministry of Education, Northeast Agricultural University, Harbin 150030, ChinaSchool of Food Science, Northeast Agricultural University, Harbin 150030, ChinaSchool of Food Science, Northeast Agricultural University, Harbin 150030, ChinaThe Key Laboratory of Soybean Biology in Chinese Ministry of Education, Northeast Agricultural University, Harbin 150030, ChinaSchool of Computer and Information Engineering, Harbin University of Commerce, Harbin 150028, ChinaSchool of Food Science, Northeast Agricultural University, Harbin 150030, ChinaSchool of Food Science, Northeast Agricultural University, Harbin 150030, ChinaThe nanomagnetic carrier (Fe3O4@SiO2@p(GMA)) was prepared by atom transfer radical polymerization, and then, the free phospholipase C (PLC) was immobilized on it proved by the results of FT-IR analysis. The enzyme loading was 135.64 mg/g, the enzyme activity was 8560.7 U/g, the average particle size was 99.86 ± 0.80 nm, and the specific saturation magnetization was 16.00 ± 0.20 emu/g. PLC-Fe3O4@SiO2@p(GMA) showed the highest activities at the pH of 7.5, and tolerance temperature raised to 65°C in soybean lecithin emulsion. Enzymatic degumming with PLC-Fe3O4@SiO2@p(GMA) under the conditions of the enzyme dosage of 110 mg/kg, reaction temperature of 65°C, pH of 7.5, and reaction time of 2.5 h resulted in residual phosphorus of 64.7 mg/kg, 1,2-diacylglycerol (1,2-DAG) contents of 1.07%, and oil yield of 98.1%. Moreover, PLC-Fe3O4@SiO2@p(GMA) still possessed more than 80% of its initial activity after 5 cycles.http://dx.doi.org/10.1155/2019/5951793
spellingShingle Yang Jiang
Jing Du
Honglin Tang
Xin Zhang
Wenbin Li
Liqi Wang
Lianzhou Jiang
Dianyu Yu
Synthesis and Application of Nanomagnetic Immobilized Phospholipase C
Journal of Chemistry
title Synthesis and Application of Nanomagnetic Immobilized Phospholipase C
title_full Synthesis and Application of Nanomagnetic Immobilized Phospholipase C
title_fullStr Synthesis and Application of Nanomagnetic Immobilized Phospholipase C
title_full_unstemmed Synthesis and Application of Nanomagnetic Immobilized Phospholipase C
title_short Synthesis and Application of Nanomagnetic Immobilized Phospholipase C
title_sort synthesis and application of nanomagnetic immobilized phospholipase c
url http://dx.doi.org/10.1155/2019/5951793
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