Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating

Abstract Switchable radiative cooling/heating holds great promise for mitigating the global energy and environmental crisis. Here, we reported a cost‐effective, high‐strength Janus film through surface optical engineering waste paper with one side decorated by a hydrophobic polymeric cooling coating...

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Main Authors: Zifan Song, Zipeng Zhang, Xueting Zhang, Jingyang Liu, Wanjie Wang, Jianfeng Wang, Xiuxiu Jin
Format: Article
Language:English
Published: Wiley 2025-01-01
Series:Carbon Energy
Subjects:
Online Access:https://doi.org/10.1002/cey2.676
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author Zifan Song
Zipeng Zhang
Xueting Zhang
Jingyang Liu
Wanjie Wang
Jianfeng Wang
Xiuxiu Jin
author_facet Zifan Song
Zipeng Zhang
Xueting Zhang
Jingyang Liu
Wanjie Wang
Jianfeng Wang
Xiuxiu Jin
author_sort Zifan Song
collection DOAJ
description Abstract Switchable radiative cooling/heating holds great promise for mitigating the global energy and environmental crisis. Here, we reported a cost‐effective, high‐strength Janus film through surface optical engineering waste paper with one side decorated by a hydrophobic polymeric cooling coating consisting of micro/nanopore/particle hierarchical structure and the other side coated with hydrophilic MXene nanosheets for heating. The cooling surface demonstrates high solar reflectivity (96.3%) and infrared emissivity (95.5%), resulting in daytime/nighttime sub‐ambient radiative cooling of 6°C/8°C with the theoretical cooling power of 100.6 and 138.5 W m−2, respectively. The heating surface exhibits high solar absorptivity (83.7%) and low infrared emissivity (15.2%), resulting in excellent radiative heating capacity for vehicle charging pile (~6.2°C) and solar heating performance. Impressively, the mechanical strength of Janus film increased greatly by 563% compared with that of pristine waste paper, which is helpful for its practical applications in various scenarios for switchable radiative thermal management through mechanical flipping. Energy‐saving simulation results reveal that significant total energy savings of up to 32.4 MJ m−2 can be achieved annually (corresponding to the 12.4% saving ratio), showing the immense importance of reducing carbon footprint and promoting carbon neutrality.
format Article
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institution Kabale University
issn 2637-9368
language English
publishDate 2025-01-01
publisher Wiley
record_format Article
series Carbon Energy
spelling doaj-art-45db7323e4534c7da9de45b13ce17f632025-01-24T13:35:41ZengWileyCarbon Energy2637-93682025-01-0171n/an/a10.1002/cey2.676Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heatingZifan Song0Zipeng Zhang1Xueting Zhang2Jingyang Liu3Wanjie Wang4Jianfeng Wang5Xiuxiu Jin6Henan Eye Hospital People's Hospital of Zhengzhou University, Henan Provincial People's Hospital Zhengzhou ChinaSchool of Materials Science and Engineering Zhengzhou ChinaSchool of Materials Science and Engineering Zhengzhou ChinaHenan Eye Hospital People's Hospital of Zhengzhou University, Henan Provincial People's Hospital Zhengzhou ChinaSchool of Materials Science and Engineering Zhengzhou ChinaSchool of Materials Science and Engineering Zhengzhou ChinaHenan Eye Hospital People's Hospital of Zhengzhou University, Henan Provincial People's Hospital Zhengzhou ChinaAbstract Switchable radiative cooling/heating holds great promise for mitigating the global energy and environmental crisis. Here, we reported a cost‐effective, high‐strength Janus film through surface optical engineering waste paper with one side decorated by a hydrophobic polymeric cooling coating consisting of micro/nanopore/particle hierarchical structure and the other side coated with hydrophilic MXene nanosheets for heating. The cooling surface demonstrates high solar reflectivity (96.3%) and infrared emissivity (95.5%), resulting in daytime/nighttime sub‐ambient radiative cooling of 6°C/8°C with the theoretical cooling power of 100.6 and 138.5 W m−2, respectively. The heating surface exhibits high solar absorptivity (83.7%) and low infrared emissivity (15.2%), resulting in excellent radiative heating capacity for vehicle charging pile (~6.2°C) and solar heating performance. Impressively, the mechanical strength of Janus film increased greatly by 563% compared with that of pristine waste paper, which is helpful for its practical applications in various scenarios for switchable radiative thermal management through mechanical flipping. Energy‐saving simulation results reveal that significant total energy savings of up to 32.4 MJ m−2 can be achieved annually (corresponding to the 12.4% saving ratio), showing the immense importance of reducing carbon footprint and promoting carbon neutrality.https://doi.org/10.1002/cey2.676hierarchical nano‐micro structurehigh strengthJanus optical nanoengineeringswitchable radiative cooling/heating
spellingShingle Zifan Song
Zipeng Zhang
Xueting Zhang
Jingyang Liu
Wanjie Wang
Jianfeng Wang
Xiuxiu Jin
Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating
Carbon Energy
hierarchical nano‐micro structure
high strength
Janus optical nanoengineering
switchable radiative cooling/heating
title Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating
title_full Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating
title_fullStr Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating
title_full_unstemmed Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating
title_short Hierarchically structured, Janus optical nanoengineered wastepaper for switchable radiative cooling/heating
title_sort hierarchically structured janus optical nanoengineered wastepaper for switchable radiative cooling heating
topic hierarchical nano‐micro structure
high strength
Janus optical nanoengineering
switchable radiative cooling/heating
url https://doi.org/10.1002/cey2.676
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AT jingyangliu hierarchicallystructuredjanusopticalnanoengineeredwastepaperforswitchableradiativecoolingheating
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