Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue

Abstract This study investigates the umami-related compounds, volatile components, and sensory attributes of Mekai (Pycnarrhena tumefacta miers) leaves based on maturity level and extraction solvent. The research examines free protein and free glutamate levels as umami indicators. Key metabolites, v...

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Main Authors: Nur Amaliah, Salengke Salengke, Zainal Zainal, Meta Mahendradatta
Format: Article
Language:English
Published: Springer 2025-07-01
Series:Discover Food
Subjects:
Online Access:https://doi.org/10.1007/s44187-025-00537-w
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author Nur Amaliah
Salengke Salengke
Zainal Zainal
Meta Mahendradatta
author_facet Nur Amaliah
Salengke Salengke
Zainal Zainal
Meta Mahendradatta
author_sort Nur Amaliah
collection DOAJ
description Abstract This study investigates the umami-related compounds, volatile components, and sensory attributes of Mekai (Pycnarrhena tumefacta miers) leaves based on maturity level and extraction solvent. The research examines free protein and free glutamate levels as umami indicators. Key metabolites, volatile chemicals, umami-related chemical changes, and intensity of taste were found utilizing liquid chromatography-high resolution mass spectrometry (LC-HRMS), gas chromatography-mass spectrometry (GC-MS), and an electronic tongue. The metabolite profiles varied between young and old leaves, as well as between water and methanolic extracts. Both leaf types exhibited low umami intensity, with 7 umami-related compounds detected in the water extract and 3 in the methanolic extract. Identified umami compounds included amino acids, peptides, nucleotides, and organic acids. Volatile analysis revealed aldehydes, particularly 4-hydroxy-3-methyl-butanal and butanal, as dominant components. Analysis showed the highest free protein (75.4 mg/mL) and free glutamate (10.3 µg/mL) concentrations in old leaves extracted with water. These findings provide insights into selecting Mekai leaves and extraction methods for umami enhancement. Further processing is necessary to enhance their umami intensity for potential application as a natural plant-based flavoring alternative.
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issn 2731-4286
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publishDate 2025-07-01
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series Discover Food
spelling doaj-art-4496443ee04c4b5b9a8839f097314d542025-08-20T04:03:01ZengSpringerDiscover Food2731-42862025-07-015111610.1007/s44187-025-00537-wCharacterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongueNur Amaliah0Salengke Salengke1Zainal Zainal2Meta Mahendradatta3Postgraduate School of Hasanuddin UniversityDepartment of Agricultural Technology, Hasanuddin UniversityDepartment of Agricultural Technology, Hasanuddin UniversityDepartment of Agricultural Technology, Hasanuddin UniversityAbstract This study investigates the umami-related compounds, volatile components, and sensory attributes of Mekai (Pycnarrhena tumefacta miers) leaves based on maturity level and extraction solvent. The research examines free protein and free glutamate levels as umami indicators. Key metabolites, volatile chemicals, umami-related chemical changes, and intensity of taste were found utilizing liquid chromatography-high resolution mass spectrometry (LC-HRMS), gas chromatography-mass spectrometry (GC-MS), and an electronic tongue. The metabolite profiles varied between young and old leaves, as well as between water and methanolic extracts. Both leaf types exhibited low umami intensity, with 7 umami-related compounds detected in the water extract and 3 in the methanolic extract. Identified umami compounds included amino acids, peptides, nucleotides, and organic acids. Volatile analysis revealed aldehydes, particularly 4-hydroxy-3-methyl-butanal and butanal, as dominant components. Analysis showed the highest free protein (75.4 mg/mL) and free glutamate (10.3 µg/mL) concentrations in old leaves extracted with water. These findings provide insights into selecting Mekai leaves and extraction methods for umami enhancement. Further processing is necessary to enhance their umami intensity for potential application as a natural plant-based flavoring alternative.https://doi.org/10.1007/s44187-025-00537-wMekai leavesUmamiMetaboliteVolatileLC-HRMS
spellingShingle Nur Amaliah
Salengke Salengke
Zainal Zainal
Meta Mahendradatta
Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue
Discover Food
Mekai leaves
Umami
Metabolite
Volatile
LC-HRMS
title Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue
title_full Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue
title_fullStr Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue
title_full_unstemmed Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue
title_short Characterization of umami-active and volatile compounds in Mekai (Pycnarrhena tumefacta miers) leaves from Kalimantan using LC-HRMS, GC-MS, and electronic tongue
title_sort characterization of umami active and volatile compounds in mekai pycnarrhena tumefacta miers leaves from kalimantan using lc hrms gc ms and electronic tongue
topic Mekai leaves
Umami
Metabolite
Volatile
LC-HRMS
url https://doi.org/10.1007/s44187-025-00537-w
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