Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries

Highlights A novel electrode design for high energy density all-solid-state batteries (ASSBs) is realized through the control of nano- and microstructures. An active materials@solid electrolyte composite with a half-covered “glitter-cake” morphology is adopted to optimize the transport of electrons...

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Main Authors: Min Ji Kim, Jin-Sung Park, Jin Woong Lee, Sung Eun Wang, Dowoong Yoon, Jong Deok Lee, Jung Hyun Kim, Taeseup Song, Ju Li, Yun Chan Kang, Dae Soo Jung
Format: Article
Language:English
Published: SpringerOpen 2025-01-01
Series:Nano-Micro Letters
Subjects:
Online Access:https://doi.org/10.1007/s40820-024-01644-6
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author Min Ji Kim
Jin-Sung Park
Jin Woong Lee
Sung Eun Wang
Dowoong Yoon
Jong Deok Lee
Jung Hyun Kim
Taeseup Song
Ju Li
Yun Chan Kang
Dae Soo Jung
author_facet Min Ji Kim
Jin-Sung Park
Jin Woong Lee
Sung Eun Wang
Dowoong Yoon
Jong Deok Lee
Jung Hyun Kim
Taeseup Song
Ju Li
Yun Chan Kang
Dae Soo Jung
author_sort Min Ji Kim
collection DOAJ
description Highlights A novel electrode design for high energy density all-solid-state batteries (ASSBs) is realized through the control of nano- and microstructures. An active materials@solid electrolyte composite with a half-covered “glitter-cake” morphology is adopted to optimize the transport of electrons and ions in the electrode. The optimized electrode design exhibited a volumetric energy density of 1258 Wh L−1 at an active material content of 85 wt%, exceeding the performance of the reported ASSB cells.
format Article
id doaj-art-423bc728e68e4eb98ff2b5a1bb2428e6
institution Kabale University
issn 2311-6706
2150-5551
language English
publishDate 2025-01-01
publisher SpringerOpen
record_format Article
series Nano-Micro Letters
spelling doaj-art-423bc728e68e4eb98ff2b5a1bb2428e62025-02-02T12:37:45ZengSpringerOpenNano-Micro Letters2311-67062150-55512025-01-0117111610.1007/s40820-024-01644-6Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State BatteriesMin Ji Kim0Jin-Sung Park1Jin Woong Lee2Sung Eun Wang3Dowoong Yoon4Jong Deok Lee5Jung Hyun Kim6Taeseup Song7Ju Li8Yun Chan Kang9Dae Soo Jung10Energy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyDepartment of Nuclear Science and Engineering, Massachusetts Institute of TechnologyEnergy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyEnergy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyEnergy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyEnergy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyEnergy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyDepartment of Energy Engineering, Hanyang UniversityDepartment of Nuclear Science and Engineering, Massachusetts Institute of TechnologyDepartment of Materials Science and Engineering, Korea UniversityEnergy and Environmental Division, Korea Institute of Ceramic Engineering and TechnologyHighlights A novel electrode design for high energy density all-solid-state batteries (ASSBs) is realized through the control of nano- and microstructures. An active materials@solid electrolyte composite with a half-covered “glitter-cake” morphology is adopted to optimize the transport of electrons and ions in the electrode. The optimized electrode design exhibited a volumetric energy density of 1258 Wh L−1 at an active material content of 85 wt%, exceeding the performance of the reported ASSB cells.https://doi.org/10.1007/s40820-024-01644-6All-solid-state batteriesCathodesSulfide-based solid electrolytesInterfacesMechanofusion
spellingShingle Min Ji Kim
Jin-Sung Park
Jin Woong Lee
Sung Eun Wang
Dowoong Yoon
Jong Deok Lee
Jung Hyun Kim
Taeseup Song
Ju Li
Yun Chan Kang
Dae Soo Jung
Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries
Nano-Micro Letters
All-solid-state batteries
Cathodes
Sulfide-based solid electrolytes
Interfaces
Mechanofusion
title Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries
title_full Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries
title_fullStr Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries
title_full_unstemmed Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries
title_short Half-Covered ‘Glitter-Cake’ AM@SE Composite: A Novel Electrode Design for High Energy Density All-Solid-State Batteries
title_sort half covered glitter cake am se composite a novel electrode design for high energy density all solid state batteries
topic All-solid-state batteries
Cathodes
Sulfide-based solid electrolytes
Interfaces
Mechanofusion
url https://doi.org/10.1007/s40820-024-01644-6
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