Agile cavity ringdown spectroscopy enabled by moderate optical feedback to a quantum cascade laser
Cavity ringdown spectroscopy (CRDS), relying on measuring the decay time of photons inside a high-finesse optical cavity, offers an important analytical tool for chemistry, physics, environmental science, and biology. Through the reflection of a slight amount of phase-coherent light back to the lase...
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| Main Authors: | , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Institue of Optics and Electronics, Chinese Academy of Sciences
2024-11-01
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| Series: | Opto-Electronic Advances |
| Subjects: | |
| Online Access: | https://www.oejournal.org/article/doi/10.29026/oea.2024.240077 |
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| Summary: | Cavity ringdown spectroscopy (CRDS), relying on measuring the decay time of photons inside a high-finesse optical cavity, offers an important analytical tool for chemistry, physics, environmental science, and biology. Through the reflection of a slight amount of phase-coherent light back to the laser source, the resonant optical feedback approach effectively couples the laser beam into the optical cavity and achieves a high signal-to-noise ratio. However, the need for active phase-locking mechanisms complicates the spectroscopic system, limiting its primarily laboratory-based use. Here, we report how passive optical feedback can be implemented in a quantum cascade laser (QCL) based CRDS system to address this issue. Without using any phase-locking loops, we reflect a moderate amount of light (–18.2 dB) to a continuous-wave QCL simply using a fixed flat mirror, narrowing the QCL linewidth from 1.2 MHz to 170 kHz and significantly increasing the laser-cavity coupling efficiency. To validate the method’s feasibility and effectiveness, we measured the absorption line (P(18e), 2207.62 cm−1) of N2O in a Fabry–Perot cavity with a high finesse of ~52000 and an inter-mirror distance of 33 cm. This agile approach paves the way for revolutionizing existing analytical tools by offering compact and high-fidelity mid-infrared CRDS systems. |
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| ISSN: | 2096-4579 |