Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate

The present study reports a novel Schiff base ‘Benzyl2-(4-(bis(2 chloroethyl)amino)benzylidene)hydrazinecarbodithioate’ and its characterization by infra red (IR), nuclear magnetic resonance (NMR), mass spectral methods with its density functional theory (DFT) quantum chemical studies. Tautomerism...

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Main Authors: Bhuvanendra Singh, Rajeev Singh, Bhoop Singh, Dilip Kumar
Format: Article
Language:English
Published: Elsevier 2017-11-01
Series:Kuwait Journal of Science
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Online Access:https://journalskuwait.org/kjs/index.php/KJS/article/view/2472
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author Bhuvanendra Singh
Rajeev Singh
Bhoop Singh
Dilip Kumar
author_facet Bhuvanendra Singh
Rajeev Singh
Bhoop Singh
Dilip Kumar
author_sort Bhuvanendra Singh
collection DOAJ
description The present study reports a novel Schiff base ‘Benzyl2-(4-(bis(2 chloroethyl)amino)benzylidene)hydrazinecarbodithioate’ and its characterization by infra red (IR), nuclear magnetic resonance (NMR), mass spectral methods with its density functional theory (DFT) quantum chemical studies. Tautomerism in this molecule was investigated theoretically by semi-empirical methods. The molecular geometry was calculated by DFT methods using split-valence triple-zeta 6311-G(2d,2p) Pople style basis set. The vibrational frequencies were calculated by DFT method at the same basis set level. The molecular parameters such as highest occupied molecular orbital energy, lowest unoccupied molecular orbital energy, frontier molecular orbital energy gap and dipole moment were calculated by DFT methods using 6311-G(2d,2p) basis set. Molecular electrostatic surface potential and electron localization function plots were also presented. The reactive sites in the molecule studied theoretically with electronic structure in sight.
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institution OA Journals
issn 2307-4108
2307-4116
language English
publishDate 2017-11-01
publisher Elsevier
record_format Article
series Kuwait Journal of Science
spelling doaj-art-406e3075bce042ca8a7daa5e7d19232b2025-08-20T02:03:38ZengElsevierKuwait Journal of Science2307-41082307-41162017-11-01444Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioateBhuvanendra Singh0Rajeev Singh1Bhoop Singh2Dilip Kumar3ITM University, GwaliorDepartment of Chemistry, Institute of Information Technology and Management,Gwalior, India.Institute of Information Technology and Management, GwaliorCenter of Research for Chemical Sciences, Post Graduate Department of Chemistry, SMS Govt. College, Gwalior The present study reports a novel Schiff base ‘Benzyl2-(4-(bis(2 chloroethyl)amino)benzylidene)hydrazinecarbodithioate’ and its characterization by infra red (IR), nuclear magnetic resonance (NMR), mass spectral methods with its density functional theory (DFT) quantum chemical studies. Tautomerism in this molecule was investigated theoretically by semi-empirical methods. The molecular geometry was calculated by DFT methods using split-valence triple-zeta 6311-G(2d,2p) Pople style basis set. The vibrational frequencies were calculated by DFT method at the same basis set level. The molecular parameters such as highest occupied molecular orbital energy, lowest unoccupied molecular orbital energy, frontier molecular orbital energy gap and dipole moment were calculated by DFT methods using 6311-G(2d,2p) basis set. Molecular electrostatic surface potential and electron localization function plots were also presented. The reactive sites in the molecule studied theoretically with electronic structure in sight. https://journalskuwait.org/kjs/index.php/KJS/article/view/2472DFTelectron localization functionHOMO-LUMOMESPquantum chemical calculations.
spellingShingle Bhuvanendra Singh
Rajeev Singh
Bhoop Singh
Dilip Kumar
Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate
Kuwait Journal of Science
DFT
electron localization function
HOMO-LUMO
MESP
quantum chemical calculations.
title Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate
title_full Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate
title_fullStr Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate
title_full_unstemmed Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate
title_short Computational study on molecular structure, vibrational and electronic properties of a novel Schiff base: Benzyl2-(4-(bis(2-chloroethyl)benzylidene) hydrazinecarbodithioate
title_sort computational study on molecular structure vibrational and electronic properties of a novel schiff base benzyl2 4 bis 2 chloroethyl benzylidene hydrazinecarbodithioate
topic DFT
electron localization function
HOMO-LUMO
MESP
quantum chemical calculations.
url https://journalskuwait.org/kjs/index.php/KJS/article/view/2472
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AT bhoopsingh computationalstudyonmolecularstructurevibrationalandelectronicpropertiesofanovelschiffbasebenzyl24bis2chloroethylbenzylidenehydrazinecarbodithioate
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