Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes

Poly-L-Lactic Acid (PLLA) is a bioabsorbable implant material due to its favorable biocompatibility and inherent degradability, while the insufficient mechanical strength hinders its further bone repair application. In present work, carbon nanotubes (CNTs) were introduced into PLLA scaffolds fabrica...

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Main Authors: Guoyong Wang, Fangwei Qi, Wenjing Yang, Youwen Yang, Chongxian He, Shuping Peng, Cijun Shuai
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:Advances in Polymer Technology
Online Access:http://dx.doi.org/10.1155/2019/8625325
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author Guoyong Wang
Fangwei Qi
Wenjing Yang
Youwen Yang
Chongxian He
Shuping Peng
Cijun Shuai
author_facet Guoyong Wang
Fangwei Qi
Wenjing Yang
Youwen Yang
Chongxian He
Shuping Peng
Cijun Shuai
author_sort Guoyong Wang
collection DOAJ
description Poly-L-Lactic Acid (PLLA) is a bioabsorbable implant material due to its favorable biocompatibility and inherent degradability, while the insufficient mechanical strength hinders its further bone repair application. In present work, carbon nanotubes (CNTs) were introduced into PLLA scaffolds fabricated via selective laser sintering. It was found that the crystallinity of PLLA increased considerably since CNTs could promote the orderly stacking of its molecular chains, thereby improving the mechanical strength of PLLA scaffold. Furthermore, the fracture surface analysis revealed that CNTs acted as a bridge across the cracks and hindered their further expansion. Moreover, CNTs pulled out from the matrix to consume a large amount of fracture energy, which enhanced the resistance to external forces. As a consequence, the compressive strength, Vickers hardness and tensile strength of the scaffold were enhanced by 22.7%, 58.8% and 17.6%, respectively. Besides, the cells exhibited good attachment, spreading and proliferation on the scaffold. This study demonstrated that PLLA/CNTs scaffold was a promising candidate as bone implant.
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language English
publishDate 2019-01-01
publisher Wiley
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series Advances in Polymer Technology
spelling doaj-art-3fffc8f4935248db99e44a9ed93175282025-08-20T03:55:36ZengWileyAdvances in Polymer Technology0730-66791098-23292019-01-01201910.1155/2019/86253258625325Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon NanotubesGuoyong Wang0Fangwei Qi1Wenjing Yang2Youwen Yang3Chongxian He4Shuping Peng5Cijun Shuai6Jiangxi University of Science and Technology, Ganzhou 341000, ChinaJiangxi University of Science and Technology, Ganzhou 341000, ChinaJiangxi University of Science and Technology, Ganzhou 341000, ChinaJiangxi University of Science and Technology, Ganzhou 341000, ChinaJiangxi University of Science and Technology, Ganzhou 341000, ChinaNHC Key Laboratory of Carcinogenesis and The Key Laboratory of Carcinogenesis and Cancer Invasion of the Chinese Ministry of Education, Xiangya Hospital, Central South University, Changsha, Hunan, ChinaJiangxi University of Science and Technology, Ganzhou 341000, ChinaPoly-L-Lactic Acid (PLLA) is a bioabsorbable implant material due to its favorable biocompatibility and inherent degradability, while the insufficient mechanical strength hinders its further bone repair application. In present work, carbon nanotubes (CNTs) were introduced into PLLA scaffolds fabricated via selective laser sintering. It was found that the crystallinity of PLLA increased considerably since CNTs could promote the orderly stacking of its molecular chains, thereby improving the mechanical strength of PLLA scaffold. Furthermore, the fracture surface analysis revealed that CNTs acted as a bridge across the cracks and hindered their further expansion. Moreover, CNTs pulled out from the matrix to consume a large amount of fracture energy, which enhanced the resistance to external forces. As a consequence, the compressive strength, Vickers hardness and tensile strength of the scaffold were enhanced by 22.7%, 58.8% and 17.6%, respectively. Besides, the cells exhibited good attachment, spreading and proliferation on the scaffold. This study demonstrated that PLLA/CNTs scaffold was a promising candidate as bone implant.http://dx.doi.org/10.1155/2019/8625325
spellingShingle Guoyong Wang
Fangwei Qi
Wenjing Yang
Youwen Yang
Chongxian He
Shuping Peng
Cijun Shuai
Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes
Advances in Polymer Technology
title Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes
title_full Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes
title_fullStr Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes
title_full_unstemmed Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes
title_short Crystallinity and Reinforcement in Poly-L-Lactic Acid Scaffold Induced by Carbon Nanotubes
title_sort crystallinity and reinforcement in poly l lactic acid scaffold induced by carbon nanotubes
url http://dx.doi.org/10.1155/2019/8625325
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