An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots
The use of nanostructures to enhance the emission of single-photon sources has attracted some attention in the last decade due to the development of quantum technologies. In particular, the use of metallic and high-refractive-index dielectric materials has been proposed. However, the utility of mode...
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MDPI AG
2024-11-01
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| author | Rafael Ramos Uña Braulio García Cámara Ángela I. Barreda |
| author_facet | Rafael Ramos Uña Braulio García Cámara Ángela I. Barreda |
| author_sort | Rafael Ramos Uña |
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| description | The use of nanostructures to enhance the emission of single-photon sources has attracted some attention in the last decade due to the development of quantum technologies. In particular, the use of metallic and high-refractive-index dielectric materials has been proposed. However, the utility of moderate-refractive-index dielectric nanostructures to achieve more efficient single-photon sources remains unexplored. Here, a systematic comparison of various metallic, high-refractive-index and moderate-refractive-index dielectric nanostructures was performed to optimize the excitation and emission of a CdSe/ZnS single quantum dot in the visible spectral region. Several geometries were evaluated in terms of electric field enhancement and Purcell factor, considering the combination of metallic, high-refractive-index and moderate-refractive-index dielectric materials conforming to homogeneous and hybrid nanoparticle dimers. Our results demonstrate that moderate-refractive-index dielectric nanoparticles can enhance the photoluminescence signal of quantum emitters due to their broader electric and magnetic dipolar resonances compared to high-refractive-index dielectric nanoparticles. However, hybrid combinations of metallic and high-refractive-index dielectric nanostructures offer the largest intensity enhancement and Purcell factors at the excitation and emission wavelengths of the quantum emitter, respectively. The results of this work may find applications in the development of single-photon sources. |
| format | Article |
| id | doaj-art-3ff07f12a4e34e39bcca822909ea1cde |
| institution | OA Journals |
| issn | 2079-4991 |
| language | English |
| publishDate | 2024-11-01 |
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| series | Nanomaterials |
| spelling | doaj-art-3ff07f12a4e34e39bcca822909ea1cde2025-08-20T02:05:07ZengMDPI AGNanomaterials2079-49912024-11-011422182210.3390/nano14221822An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum DotsRafael Ramos Uña0Braulio García Cámara1Ángela I. Barreda2Department of Electronic Engineering, University Carlos III of Madrid, Avda. de la Universidad, 30, 28911 Leganés, SpainDepartment of Electronic Engineering, University Carlos III of Madrid, Avda. de la Universidad, 30, 28911 Leganés, SpainDepartment of Electronic Engineering, University Carlos III of Madrid, Avda. de la Universidad, 30, 28911 Leganés, SpainThe use of nanostructures to enhance the emission of single-photon sources has attracted some attention in the last decade due to the development of quantum technologies. In particular, the use of metallic and high-refractive-index dielectric materials has been proposed. However, the utility of moderate-refractive-index dielectric nanostructures to achieve more efficient single-photon sources remains unexplored. Here, a systematic comparison of various metallic, high-refractive-index and moderate-refractive-index dielectric nanostructures was performed to optimize the excitation and emission of a CdSe/ZnS single quantum dot in the visible spectral region. Several geometries were evaluated in terms of electric field enhancement and Purcell factor, considering the combination of metallic, high-refractive-index and moderate-refractive-index dielectric materials conforming to homogeneous and hybrid nanoparticle dimers. Our results demonstrate that moderate-refractive-index dielectric nanoparticles can enhance the photoluminescence signal of quantum emitters due to their broader electric and magnetic dipolar resonances compared to high-refractive-index dielectric nanoparticles. However, hybrid combinations of metallic and high-refractive-index dielectric nanostructures offer the largest intensity enhancement and Purcell factors at the excitation and emission wavelengths of the quantum emitter, respectively. The results of this work may find applications in the development of single-photon sources.https://www.mdpi.com/2079-4991/14/22/1822plasmonicquantum dotsmoderate refractive indexhigh refractive indexsingle-photon sources |
| spellingShingle | Rafael Ramos Uña Braulio García Cámara Ángela I. Barreda An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots Nanomaterials plasmonic quantum dots moderate refractive index high refractive index single-photon sources |
| title | An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots |
| title_full | An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots |
| title_fullStr | An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots |
| title_full_unstemmed | An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots |
| title_short | An Evaluation of Moderate-Refractive-Index Nanoantennas for Enhancing the Photoluminescence Signal of Quantum Dots |
| title_sort | evaluation of moderate refractive index nanoantennas for enhancing the photoluminescence signal of quantum dots |
| topic | plasmonic quantum dots moderate refractive index high refractive index single-photon sources |
| url | https://www.mdpi.com/2079-4991/14/22/1822 |
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