Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects

Abstract Breast cancer is one of cancer’s most deadly varieties. Its variability makes the development of personalized therapies very difficult. Therefore, improvement of classic chemotherapy is still one of the important challenges of cancer research. We addressed this issue applying nanotechnology...

Full description

Saved in:
Bibliographic Details
Main Authors: Grzegorz Gołuński, Kinga Konkel, Barbara Galikowska-Bogut, Patrycja Bełdzińska, Katarzyna Bury, Marcin Zakrzewski, Kamila Butowska, Rafał Sądej, Jacek Piosik
Format: Article
Language:English
Published: Nature Portfolio 2024-08-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-024-69724-6
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850182339165945856
author Grzegorz Gołuński
Kinga Konkel
Barbara Galikowska-Bogut
Patrycja Bełdzińska
Katarzyna Bury
Marcin Zakrzewski
Kamila Butowska
Rafał Sądej
Jacek Piosik
author_facet Grzegorz Gołuński
Kinga Konkel
Barbara Galikowska-Bogut
Patrycja Bełdzińska
Katarzyna Bury
Marcin Zakrzewski
Kamila Butowska
Rafał Sądej
Jacek Piosik
author_sort Grzegorz Gołuński
collection DOAJ
description Abstract Breast cancer is one of cancer’s most deadly varieties. Its variability makes the development of personalized therapies very difficult. Therefore, improvement of classic chemotherapy is still one of the important challenges of cancer research. We addressed this issue applying nanotechnology to verify the influence of silver nanoparticles (AgNPs) on doxorubicin (DOX) anticancer activity and assess if the size of AgNPs affects their interactions with DOX. We employed a broad spectrum of biophysical methods, characterizing 5 and 50 nm AgNPs interactions with DOX using UV–Vis spectroscopy, dynamic light scattering, fluorescence spectroscopy, and atomic force microscopy imaging. Biological effects of observed AgNPs-DOX interactions were assessed utilizing MTT and 3D Matrigel assays on SKBR3 and MDA-MB-231 breast cancer cell lines. Obtained results indicate direct interactions between AgNPs and DOX. Furthermore, AgNPs size influences their interactions with DOX, as evidenced by differences in the heteroaggregates formation observed in biophysical experiments and further supported by in vitro biological assays. We detected reduction of tumor cell viability and/or colony sizes of the analyzed cancer cell lines, registering differences linked to the observed phenomenon. However, the effects may be limited to the outer borders of the tumor microenvironment as evidenced by the 3D model. Summing up, we observed diverse patterns of interactions and biological effects for different sizes of AgNPs with DOX providing insight how the nanoparticles’ size affects their interactions with other biologically active compounds. Moreover, obtained data can be further used in experiments on the reduction of tumor size i.e. before the surgical intervention.
format Article
id doaj-art-3f050aa6158e45989c82017dbcb08318
institution OA Journals
issn 2045-2322
language English
publishDate 2024-08-01
publisher Nature Portfolio
record_format Article
series Scientific Reports
spelling doaj-art-3f050aa6158e45989c82017dbcb083182025-08-20T02:17:39ZengNature PortfolioScientific Reports2045-23222024-08-0114111210.1038/s41598-024-69724-6Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effectsGrzegorz Gołuński0Kinga Konkel1Barbara Galikowska-Bogut2Patrycja Bełdzińska3Katarzyna Bury4Marcin Zakrzewski5Kamila Butowska6Rafał Sądej7Jacek Piosik8Laboratory of Biophysics, University of GdańskLaboratory of Biophysics, University of GdańskLaboratory of Molecular Enzymology and Oncology, Medical University of GdańskLaboratory of Biophysics, University of GdańskLaboratory of Molecular Biology, University of GdańskLaboratory of Biophysics, University of GdańskLaboratory of Biophysics, University of GdańskLaboratory of Molecular Enzymology and Oncology, Medical University of GdańskLaboratory of Biophysics, University of GdańskAbstract Breast cancer is one of cancer’s most deadly varieties. Its variability makes the development of personalized therapies very difficult. Therefore, improvement of classic chemotherapy is still one of the important challenges of cancer research. We addressed this issue applying nanotechnology to verify the influence of silver nanoparticles (AgNPs) on doxorubicin (DOX) anticancer activity and assess if the size of AgNPs affects their interactions with DOX. We employed a broad spectrum of biophysical methods, characterizing 5 and 50 nm AgNPs interactions with DOX using UV–Vis spectroscopy, dynamic light scattering, fluorescence spectroscopy, and atomic force microscopy imaging. Biological effects of observed AgNPs-DOX interactions were assessed utilizing MTT and 3D Matrigel assays on SKBR3 and MDA-MB-231 breast cancer cell lines. Obtained results indicate direct interactions between AgNPs and DOX. Furthermore, AgNPs size influences their interactions with DOX, as evidenced by differences in the heteroaggregates formation observed in biophysical experiments and further supported by in vitro biological assays. We detected reduction of tumor cell viability and/or colony sizes of the analyzed cancer cell lines, registering differences linked to the observed phenomenon. However, the effects may be limited to the outer borders of the tumor microenvironment as evidenced by the 3D model. Summing up, we observed diverse patterns of interactions and biological effects for different sizes of AgNPs with DOX providing insight how the nanoparticles’ size affects their interactions with other biologically active compounds. Moreover, obtained data can be further used in experiments on the reduction of tumor size i.e. before the surgical intervention.https://doi.org/10.1038/s41598-024-69724-6
spellingShingle Grzegorz Gołuński
Kinga Konkel
Barbara Galikowska-Bogut
Patrycja Bełdzińska
Katarzyna Bury
Marcin Zakrzewski
Kamila Butowska
Rafał Sądej
Jacek Piosik
Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects
Scientific Reports
title Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects
title_full Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects
title_fullStr Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects
title_full_unstemmed Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects
title_short Influence of silver nanoparticles’ size on their direct interactions with doxorubicin and its biological effects
title_sort influence of silver nanoparticles size on their direct interactions with doxorubicin and its biological effects
url https://doi.org/10.1038/s41598-024-69724-6
work_keys_str_mv AT grzegorzgołunski influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT kingakonkel influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT barbaragalikowskabogut influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT patrycjabełdzinska influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT katarzynabury influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT marcinzakrzewski influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT kamilabutowska influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT rafałsadej influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects
AT jacekpiosik influenceofsilvernanoparticlessizeontheirdirectinteractionswithdoxorubicinanditsbiologicaleffects