A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing

Abstract Given our poor understanding on mechanisms of stratospheric intrusions (SI) upon near‐surface ozone (O3) surges, predicting the SI‐induced O3 pollution pose inherent difficulties. Taking a wintertime O3 surge episode over the Sichuan Basin (SCB) as an example, we find SI contribute 47.8% to...

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Main Authors: Yuqing Zhang, Tianliang Zhao, Guicai Ning, Xiangde Xu, Zhixiong Chen, Mengwei Jia, Xiaoyun Sun, Zhuozhi Shu, Zhen Lu, Jane Liu, Xiushu Qie
Format: Article
Language:English
Published: Wiley 2025-05-01
Series:Geophysical Research Letters
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Online Access:https://doi.org/10.1029/2024GL114207
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author Yuqing Zhang
Tianliang Zhao
Guicai Ning
Xiangde Xu
Zhixiong Chen
Mengwei Jia
Xiaoyun Sun
Zhuozhi Shu
Zhen Lu
Jane Liu
Xiushu Qie
author_facet Yuqing Zhang
Tianliang Zhao
Guicai Ning
Xiangde Xu
Zhixiong Chen
Mengwei Jia
Xiaoyun Sun
Zhuozhi Shu
Zhen Lu
Jane Liu
Xiushu Qie
author_sort Yuqing Zhang
collection DOAJ
description Abstract Given our poor understanding on mechanisms of stratospheric intrusions (SI) upon near‐surface ozone (O3) surges, predicting the SI‐induced O3 pollution pose inherent difficulties. Taking a wintertime O3 surge episode over the Sichuan Basin (SCB) as an example, we find SI contribute 47.8% to near‐surface O3 levels and reveal the underlying mechanisms. Tropopause folding nearly extends to the deep atmospheric boundary layer over the Tibetan Plateau (TP) due to topographic forcing, driving stratospheric O3 penetration into the TP's near‐surface. The intruded O3 is subsequently transported into the downstream SCB by strong downdrafts along the TP's leeward slope. Interestingly, the mountain‐plains solenoid between the TP and the SCB strengthens the downward intrusions of O3 during both daytime and nighttime, further amplifying the contribution of SI to the SCB's near‐surface O3 levels. This unique mechanism of O3 surges could provide new insights for the forecast of unexpected nocturnal high‐O3 episodes.
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publishDate 2025-05-01
publisher Wiley
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series Geophysical Research Letters
spelling doaj-art-3ba1afadc9294fcd97919afc8dbb8e932025-08-20T02:05:13ZengWileyGeophysical Research Letters0094-82761944-80072025-05-015210n/an/a10.1029/2024GL114207A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic ForcingYuqing Zhang0Tianliang Zhao1Guicai Ning2Xiangde Xu3Zhixiong Chen4Mengwei Jia5Xiaoyun Sun6Zhuozhi Shu7Zhen Lu8Jane Liu9Xiushu Qie10Key Laboratory for Aerosol‐Cloud‐Precipitation of China Meteorological Administration Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science and Technology Nanjing ChinaKey Laboratory for Aerosol‐Cloud‐Precipitation of China Meteorological Administration Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science and Technology Nanjing ChinaKey Laboratory for Aerosol‐Cloud‐Precipitation of China Meteorological Administration Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science and Technology Nanjing ChinaState Key Laboratory of Severe Weather Chinese Academy of Meteorological Sciences China Meteorological Administration Beijing ChinaKey Laboratory for Humid Subtropical Eco‐Geographical Processes of the Ministry of Education School of Geographical Sciences Fujian Normal University Fuzhou ChinaJiangsu Provincial Key Laboratory of Geographic Information Science and Technology International Institute for Earth System Science Nanjing University Nanjing ChinaAnhui Province Key Laboratory of Atmospheric Science and Satellite Remote Sensing Anhui Institute of Meteorological Sciences Hefei ChinaChengdu Fluid Dynamics Innovation Center Chengdu ChinaKey Laboratory for Aerosol‐Cloud‐Precipitation of China Meteorological Administration Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science and Technology Nanjing ChinaKey Laboratory for Humid Subtropical Eco‐Geographical Processes of the Ministry of Education School of Geographical Sciences Fujian Normal University Fuzhou ChinaKey Laboratory of Middle Atmosphere and Global Environment Observation Institute of Atmospheric Physics Chinese Academy of Sciences Beijing ChinaAbstract Given our poor understanding on mechanisms of stratospheric intrusions (SI) upon near‐surface ozone (O3) surges, predicting the SI‐induced O3 pollution pose inherent difficulties. Taking a wintertime O3 surge episode over the Sichuan Basin (SCB) as an example, we find SI contribute 47.8% to near‐surface O3 levels and reveal the underlying mechanisms. Tropopause folding nearly extends to the deep atmospheric boundary layer over the Tibetan Plateau (TP) due to topographic forcing, driving stratospheric O3 penetration into the TP's near‐surface. The intruded O3 is subsequently transported into the downstream SCB by strong downdrafts along the TP's leeward slope. Interestingly, the mountain‐plains solenoid between the TP and the SCB strengthens the downward intrusions of O3 during both daytime and nighttime, further amplifying the contribution of SI to the SCB's near‐surface O3 levels. This unique mechanism of O3 surges could provide new insights for the forecast of unexpected nocturnal high‐O3 episodes.https://doi.org/10.1029/2024GL114207stratospheric ozone intrusiontopographic forcingmountain‐plains solenoidTibetan PlateauSichuan Basin
spellingShingle Yuqing Zhang
Tianliang Zhao
Guicai Ning
Xiangde Xu
Zhixiong Chen
Mengwei Jia
Xiaoyun Sun
Zhuozhi Shu
Zhen Lu
Jane Liu
Xiushu Qie
A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing
Geophysical Research Letters
stratospheric ozone intrusion
topographic forcing
mountain‐plains solenoid
Tibetan Plateau
Sichuan Basin
title A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing
title_full A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing
title_fullStr A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing
title_full_unstemmed A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing
title_short A Unique Mechanism of Ozone Surges Jointly Triggered by Deep Stratospheric Intrusions and the Tibetan Plateau Topographic Forcing
title_sort unique mechanism of ozone surges jointly triggered by deep stratospheric intrusions and the tibetan plateau topographic forcing
topic stratospheric ozone intrusion
topographic forcing
mountain‐plains solenoid
Tibetan Plateau
Sichuan Basin
url https://doi.org/10.1029/2024GL114207
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