Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions

We have used single molecule tracking to investigate dynamics of four penicillin-binding proteins (PBPs) in <i>Bacillus subtilis</i> to shed light on their possible modes of action. We show that Pbp2a, Pbp3, Pbp4, and Pbp4a, when expressed at very low levels, show at least two distinct s...

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Main Authors: Lisa Stuckenschneider, Peter L. Graumann
Format: Article
Language:English
Published: MDPI AG 2025-03-01
Series:Cells
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Online Access:https://www.mdpi.com/2073-4409/14/6/429
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author Lisa Stuckenschneider
Peter L. Graumann
author_facet Lisa Stuckenschneider
Peter L. Graumann
author_sort Lisa Stuckenschneider
collection DOAJ
description We have used single molecule tracking to investigate dynamics of four penicillin-binding proteins (PBPs) in <i>Bacillus subtilis</i> to shed light on their possible modes of action. We show that Pbp2a, Pbp3, Pbp4, and Pbp4a, when expressed at very low levels, show at least two distinct states of mobility: a state of slow motion, likely representing molecules involved in cell wall synthesis, and a mode of fast motion, likely representing freely diffusing molecules. Except for Pbp4, all other PBPs showed about 50% molecules in the slow mobility state, suggesting that roughly half of all molecules are engaged in a substrate-bound mode. We observed similar coefficients for the slow mobility state for Pbp4 and Pbp4a on the one hand, and for Pbp2a and Pbp3 on the other hand, indicating possible joint activities, respectively. Upon induction of osmotic stress, Pbp2a and Pbp4a changed from a pattern of localization mostly at the lateral cell membrane to also include localization at the septum, revealing that sites of preferred positioning for these two PBPs can be modified during stress conditions. While Pbp3 became more dynamic after induction of osmotic stress, Pbp4 became more static, showing that PBPs reacted markedly differently to envelope stress conditions. The data suggest that PBPs could take over functions in cell wall synthesis during different stress conditions, increasing the resilience of cell wall homeostasis in different environmental conditions. All PBPs lost their respective localization pattern after the addition of vancomycin or penicillin G, indicating that patterns largely depend on substrate availability. Our findings show that PBPs rapidly alter between non-targeted motion through the cell membrane and capture at sites of active cell wall synthesis, most likely guided by complex formation with other cell wall synthesis enzymes.
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spelling doaj-art-39c2d77bef3f41c380cf8922b1a467132025-08-20T02:11:22ZengMDPI AGCells2073-44092025-03-0114642910.3390/cells14060429Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress ConditionsLisa Stuckenschneider0Peter L. Graumann1SYNMIKRO, Zentrum für Synthetische Mikrobiologie, Hans-Meerwein-Straße, 35043 Marburg, GermanySYNMIKRO, Zentrum für Synthetische Mikrobiologie, Hans-Meerwein-Straße, 35043 Marburg, GermanyWe have used single molecule tracking to investigate dynamics of four penicillin-binding proteins (PBPs) in <i>Bacillus subtilis</i> to shed light on their possible modes of action. We show that Pbp2a, Pbp3, Pbp4, and Pbp4a, when expressed at very low levels, show at least two distinct states of mobility: a state of slow motion, likely representing molecules involved in cell wall synthesis, and a mode of fast motion, likely representing freely diffusing molecules. Except for Pbp4, all other PBPs showed about 50% molecules in the slow mobility state, suggesting that roughly half of all molecules are engaged in a substrate-bound mode. We observed similar coefficients for the slow mobility state for Pbp4 and Pbp4a on the one hand, and for Pbp2a and Pbp3 on the other hand, indicating possible joint activities, respectively. Upon induction of osmotic stress, Pbp2a and Pbp4a changed from a pattern of localization mostly at the lateral cell membrane to also include localization at the septum, revealing that sites of preferred positioning for these two PBPs can be modified during stress conditions. While Pbp3 became more dynamic after induction of osmotic stress, Pbp4 became more static, showing that PBPs reacted markedly differently to envelope stress conditions. The data suggest that PBPs could take over functions in cell wall synthesis during different stress conditions, increasing the resilience of cell wall homeostasis in different environmental conditions. All PBPs lost their respective localization pattern after the addition of vancomycin or penicillin G, indicating that patterns largely depend on substrate availability. Our findings show that PBPs rapidly alter between non-targeted motion through the cell membrane and capture at sites of active cell wall synthesis, most likely guided by complex formation with other cell wall synthesis enzymes.https://www.mdpi.com/2073-4409/14/6/429bacterial cell wall synthesispenicillin-binding proteins<i>Bacillus subtilis</i>single molecule dynamics
spellingShingle Lisa Stuckenschneider
Peter L. Graumann
Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions
Cells
bacterial cell wall synthesis
penicillin-binding proteins
<i>Bacillus subtilis</i>
single molecule dynamics
title Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions
title_full Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions
title_fullStr Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions
title_full_unstemmed Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions
title_short Localization and Single Molecule Dynamics of <i>Bacillus subtilis</i> Penicillin-Binding Proteins Depend on Substrate Availability and Are Affected by Stress Conditions
title_sort localization and single molecule dynamics of i bacillus subtilis i penicillin binding proteins depend on substrate availability and are affected by stress conditions
topic bacterial cell wall synthesis
penicillin-binding proteins
<i>Bacillus subtilis</i>
single molecule dynamics
url https://www.mdpi.com/2073-4409/14/6/429
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AT peterlgraumann localizationandsinglemoleculedynamicsofibacillussubtilisipenicillinbindingproteinsdependonsubstrateavailabilityandareaffectedbystressconditions