Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer

Abstract Introduction Ovarian cancer has only a 17% 5‐year survival rate in patients diagnosed with late stage disease. Tumor‐associated glycoprotein‐72 (TAG72), expressed in 88% of all stages of ovarian cancer, is an excellent candidate for antibody‐targeted therapy, as it is not expressed in norma...

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Main Authors: Megan Minnix, Lin Li, Paul Yazaki, Junie Chea, Erasmus Poku, David Colcher, John E. Shively
Format: Article
Language:English
Published: Wiley 2020-07-01
Series:Cancer Medicine
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Online Access:https://doi.org/10.1002/cam4.3078
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author Megan Minnix
Lin Li
Paul Yazaki
Junie Chea
Erasmus Poku
David Colcher
John E. Shively
author_facet Megan Minnix
Lin Li
Paul Yazaki
Junie Chea
Erasmus Poku
David Colcher
John E. Shively
author_sort Megan Minnix
collection DOAJ
description Abstract Introduction Ovarian cancer has only a 17% 5‐year survival rate in patients diagnosed with late stage disease. Tumor‐associated glycoprotein‐72 (TAG72), expressed in 88% of all stages of ovarian cancer, is an excellent candidate for antibody‐targeted therapy, as it is not expressed in normal human adult tissues, except in the secretory endometrium. Methods Using the clinically relevant anti‐TAG72 murine monoclonal antibody CC49, we evaluated antibody drug conjugates (ADCs) incorporating the highly potent, synthetic antimitotic agent monomethylauristatin E (MMAE). MMAE was conjugated to CC49 via reduced disulfides in the hinge region, using three different types of linker chemistry, vinylsulfone (VS‐MMAE), bromoacetamido (Br‐MMAE), and maleimido (mal‐MMAE). Results The drug antibody ratios (DARs) of the three ADCs were 2.3 for VS‐MMAE, 10 for Br‐MMAE, and 9.5 for mal‐MMAE. All three ADCs exhibited excellent tumor to blood ratios on PET imaging, but the absolute uptake of CC49‐mal‐MMAE (3.3%ID/g) was low compared to CC49‐Br‐MMAE (6.43%ID/g), at 142 hours. Blood clearance at 43 hours was 38% for intact CC49, about 24% for both CC49‐VS‐MMAE and CC49‐Br‐MMAE, and 7% for CC49‐mal‐MMAE. CC49‐VS‐MMAE was not further studied due to its low DAR, while CC49‐mal‐MMAE was ineffective in the OVCAR3 xenograft likely due to its rapid blood clearance. In contrast, CC49‐Br‐MMAE treated mice exhibited an average of a 15.6 day tumor growth delay and a 40% increase in survival vs controls with four doses of 7.5 or 15 mg/kg of CC49‐Br‐MMAE. Conclusion We conclude that CC49‐Br‐MMAE with a high DAR and stable linker performs well in a difficult to treat solid tumor model.
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spelling doaj-art-39c08780ebd94cffa6cfb8035f48bfb82024-12-20T13:05:46ZengWileyCancer Medicine2045-76342020-07-019134756476710.1002/cam4.3078Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancerMegan Minnix0Lin Li1Paul Yazaki2Junie Chea3Erasmus Poku4David Colcher5John E. Shively6Department of Molecular Imaging and Therapy Beckman Research Institute City of Hope Duarte CA USADepartment of Molecular Imaging and Therapy Beckman Research Institute City of Hope Duarte CA USADepartment of Molecular Imaging and Therapy Beckman Research Institute City of Hope Duarte CA USARadiopharmacy City of Hope Medical Center Duarte CA USARadiopharmacy City of Hope Medical Center Duarte CA USADepartment of Molecular Imaging and Therapy Beckman Research Institute City of Hope Duarte CA USADepartment of Molecular Imaging and Therapy Beckman Research Institute City of Hope Duarte CA USAAbstract Introduction Ovarian cancer has only a 17% 5‐year survival rate in patients diagnosed with late stage disease. Tumor‐associated glycoprotein‐72 (TAG72), expressed in 88% of all stages of ovarian cancer, is an excellent candidate for antibody‐targeted therapy, as it is not expressed in normal human adult tissues, except in the secretory endometrium. Methods Using the clinically relevant anti‐TAG72 murine monoclonal antibody CC49, we evaluated antibody drug conjugates (ADCs) incorporating the highly potent, synthetic antimitotic agent monomethylauristatin E (MMAE). MMAE was conjugated to CC49 via reduced disulfides in the hinge region, using three different types of linker chemistry, vinylsulfone (VS‐MMAE), bromoacetamido (Br‐MMAE), and maleimido (mal‐MMAE). Results The drug antibody ratios (DARs) of the three ADCs were 2.3 for VS‐MMAE, 10 for Br‐MMAE, and 9.5 for mal‐MMAE. All three ADCs exhibited excellent tumor to blood ratios on PET imaging, but the absolute uptake of CC49‐mal‐MMAE (3.3%ID/g) was low compared to CC49‐Br‐MMAE (6.43%ID/g), at 142 hours. Blood clearance at 43 hours was 38% for intact CC49, about 24% for both CC49‐VS‐MMAE and CC49‐Br‐MMAE, and 7% for CC49‐mal‐MMAE. CC49‐VS‐MMAE was not further studied due to its low DAR, while CC49‐mal‐MMAE was ineffective in the OVCAR3 xenograft likely due to its rapid blood clearance. In contrast, CC49‐Br‐MMAE treated mice exhibited an average of a 15.6 day tumor growth delay and a 40% increase in survival vs controls with four doses of 7.5 or 15 mg/kg of CC49‐Br‐MMAE. Conclusion We conclude that CC49‐Br‐MMAE with a high DAR and stable linker performs well in a difficult to treat solid tumor model.https://doi.org/10.1002/cam4.3078antibody drug conjugateovarian cancerTAG72
spellingShingle Megan Minnix
Lin Li
Paul Yazaki
Junie Chea
Erasmus Poku
David Colcher
John E. Shively
Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer
Cancer Medicine
antibody drug conjugate
ovarian cancer
TAG72
title Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer
title_full Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer
title_fullStr Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer
title_full_unstemmed Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer
title_short Improved targeting of an anti‐TAG‐72 antibody drug conjugate for the treatment of ovarian cancer
title_sort improved targeting of an anti tag 72 antibody drug conjugate for the treatment of ovarian cancer
topic antibody drug conjugate
ovarian cancer
TAG72
url https://doi.org/10.1002/cam4.3078
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AT juniechea improvedtargetingofanantitag72antibodydrugconjugateforthetreatmentofovariancancer
AT erasmuspoku improvedtargetingofanantitag72antibodydrugconjugateforthetreatmentofovariancancer
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