Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior

Polyurethane elastomers are widely utilized in various industrial applications due to their exceptional flexibility, energy absorption, and long-term pressure resistance. However, their mechanical stability under extremely low-frequency cyclic loading remains poorly understood, particularly in terms...

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Main Authors: Doyoung Kim, Gayoung Kim, Jinhyeok Jang, Jae-Hyuk Choi, Munkyu Lee, Woong-Ryeol Yu
Format: Article
Language:English
Published: Elsevier 2025-08-01
Series:Polymer Testing
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Online Access:http://www.sciencedirect.com/science/article/pii/S0142941825001783
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author Doyoung Kim
Gayoung Kim
Jinhyeok Jang
Jae-Hyuk Choi
Munkyu Lee
Woong-Ryeol Yu
author_facet Doyoung Kim
Gayoung Kim
Jinhyeok Jang
Jae-Hyuk Choi
Munkyu Lee
Woong-Ryeol Yu
author_sort Doyoung Kim
collection DOAJ
description Polyurethane elastomers are widely utilized in various industrial applications due to their exceptional flexibility, energy absorption, and long-term pressure resistance. However, their mechanical stability under extremely low-frequency cyclic loading remains poorly understood, particularly in terms of fatigue and creep behavior. This study investigates the failure mechanisms of thermoplastic polyurethane (TPU) and cross-linked TPU under long-term localized compressive stress under extremely low-frequency cyclic loading, simulating real-world conditions in the automotive sector. The experimental approach includes dynamic mechanical analysis, tensile, compression, shear, fatigue, and creep tests, complemented by finite element simulations using a visco-hyperelastic model. Our findings indicate that shear stress plays a more significant role in TPU failure compared to compressive stress, with fatigue behavior under extremely low-frequency conditions exhibiting characteristics similar to creep deformation. The time-temperature superposition method was employed to accelerate testing, validating predictive models for long-term elastomer durability. Furthermore, the introduction of SiO2-reinforced TPU nanocomposites demonstrated enhanced shear creep resistance, effectively extending failure time under equivalent stress conditions. These results provide valuable insights for improving the design and reliability of polyurethane elastomers in applications requiring prolonged mechanical stability.
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spelling doaj-art-397c246e039b4bedbf9dc6ed61abc5642025-08-20T02:37:46ZengElsevierPolymer Testing1873-23482025-08-0114910886410.1016/j.polymertesting.2025.108864Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behaviorDoyoung Kim0Gayoung Kim1Jinhyeok Jang2Jae-Hyuk Choi3Munkyu Lee4Woong-Ryeol Yu5Department of Materials Science and Engineering (MSE) and Research Institute of Advanced Materials (RIAM), Seoul National University, Seoul, 08826, Republic of KoreaDepartment of Materials Science and Engineering (MSE) and Research Institute of Advanced Materials (RIAM), Seoul National University, Seoul, 08826, Republic of KoreaDepartment of Materials Science and Engineering (MSE) and Research Institute of Advanced Materials (RIAM), Seoul National University, Seoul, 08826, Republic of KoreaDepartment of Materials Science and Engineering (MSE) and Research Institute of Advanced Materials (RIAM), Seoul National University, Seoul, 08826, Republic of KoreaVehicle Manufacturing Engineering Team 2, Hyundai Motor Group, 700 Yeompo-ro, Buk-Gu, Ulsan, 44259, Republic of KoreaDepartment of Materials Science and Engineering (MSE) and Research Institute of Advanced Materials (RIAM), Seoul National University, Seoul, 08826, Republic of Korea; Corresponding author.Polyurethane elastomers are widely utilized in various industrial applications due to their exceptional flexibility, energy absorption, and long-term pressure resistance. However, their mechanical stability under extremely low-frequency cyclic loading remains poorly understood, particularly in terms of fatigue and creep behavior. This study investigates the failure mechanisms of thermoplastic polyurethane (TPU) and cross-linked TPU under long-term localized compressive stress under extremely low-frequency cyclic loading, simulating real-world conditions in the automotive sector. The experimental approach includes dynamic mechanical analysis, tensile, compression, shear, fatigue, and creep tests, complemented by finite element simulations using a visco-hyperelastic model. Our findings indicate that shear stress plays a more significant role in TPU failure compared to compressive stress, with fatigue behavior under extremely low-frequency conditions exhibiting characteristics similar to creep deformation. The time-temperature superposition method was employed to accelerate testing, validating predictive models for long-term elastomer durability. Furthermore, the introduction of SiO2-reinforced TPU nanocomposites demonstrated enhanced shear creep resistance, effectively extending failure time under equivalent stress conditions. These results provide valuable insights for improving the design and reliability of polyurethane elastomers in applications requiring prolonged mechanical stability.http://www.sciencedirect.com/science/article/pii/S0142941825001783Thermoplastic polyurethaneExtremely low-frequencyFatigueCreepFailure
spellingShingle Doyoung Kim
Gayoung Kim
Jinhyeok Jang
Jae-Hyuk Choi
Munkyu Lee
Woong-Ryeol Yu
Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
Polymer Testing
Thermoplastic polyurethane
Extremely low-frequency
Fatigue
Creep
Failure
title Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
title_full Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
title_fullStr Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
title_full_unstemmed Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
title_short Analysis of low-frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
title_sort analysis of low frequency fatigue behavior of polyurethane elastomers under localized compressive loading using shear creep behavior
topic Thermoplastic polyurethane
Extremely low-frequency
Fatigue
Creep
Failure
url http://www.sciencedirect.com/science/article/pii/S0142941825001783
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