Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)

Rare Earth Elements (REEs) are critical raw materials essential for energy and digital transitions. In this study, original data are presented on the extraction of REEs from electrode powders of NiMH batteries pre-treated through physical methods in a cryo-mechanical pilot plant. The electrode powde...

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Main Authors: Francesca Pagnanelli, Pier Giorgio Schiavi, Marco Colasanti, Pietro Altimari
Format: Article
Language:English
Published: AIDIC Servizi S.r.l. 2025-07-01
Series:Chemical Engineering Transactions
Online Access:https://www.cetjournal.it/index.php/cet/article/view/15317
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author Francesca Pagnanelli
Pier Giorgio Schiavi
Marco Colasanti
Pietro Altimari
author_facet Francesca Pagnanelli
Pier Giorgio Schiavi
Marco Colasanti
Pietro Altimari
author_sort Francesca Pagnanelli
collection DOAJ
description Rare Earth Elements (REEs) are critical raw materials essential for energy and digital transitions. In this study, original data are presented on the extraction of REEs from electrode powders of NiMH batteries pre-treated through physical methods in a cryo-mechanical pilot plant. The electrode powder was characterized for its chemical composition and subsequently subjected to extraction using a DES based on choline chloride and lactic acid (with a molar ratio of 1:2). The performance of DES extraction was compared with leaching using sulfuric acid under varying temperatures. Empirical modeling of extraction with sulfuric acid revealed a significant negative effect of increasing temperature on the extraction of both Lanthanum and Cerium, which consequently reduced REE selectivity. Kinetic tests using DES showed a positive effect of time on REE extraction, while other metals (such as Nickel and Manganese) exhibited a non-monotonic effect of time, ultimately enhancing REE selectivity at longer durations.
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institution Kabale University
issn 2283-9216
language English
publishDate 2025-07-01
publisher AIDIC Servizi S.r.l.
record_format Article
series Chemical Engineering Transactions
spelling doaj-art-35fc9e27d62841fbb39cd2d47a5fff102025-08-20T03:58:37ZengAIDIC Servizi S.r.l.Chemical Engineering Transactions2283-92162025-07-01117Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)Francesca PagnanelliPier Giorgio SchiaviMarco ColasantiPietro AltimariRare Earth Elements (REEs) are critical raw materials essential for energy and digital transitions. In this study, original data are presented on the extraction of REEs from electrode powders of NiMH batteries pre-treated through physical methods in a cryo-mechanical pilot plant. The electrode powder was characterized for its chemical composition and subsequently subjected to extraction using a DES based on choline chloride and lactic acid (with a molar ratio of 1:2). The performance of DES extraction was compared with leaching using sulfuric acid under varying temperatures. Empirical modeling of extraction with sulfuric acid revealed a significant negative effect of increasing temperature on the extraction of both Lanthanum and Cerium, which consequently reduced REE selectivity. Kinetic tests using DES showed a positive effect of time on REE extraction, while other metals (such as Nickel and Manganese) exhibited a non-monotonic effect of time, ultimately enhancing REE selectivity at longer durations.https://www.cetjournal.it/index.php/cet/article/view/15317
spellingShingle Francesca Pagnanelli
Pier Giorgio Schiavi
Marco Colasanti
Pietro Altimari
Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)
Chemical Engineering Transactions
title Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)
title_full Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)
title_fullStr Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)
title_full_unstemmed Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)
title_short Extraction of Rare Earth Elements (REE) from End-of-Life NiMH Battery Electrode Powders Using Deep Eutectic Solvent (DES)
title_sort extraction of rare earth elements ree from end of life nimh battery electrode powders using deep eutectic solvent des
url https://www.cetjournal.it/index.php/cet/article/view/15317
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