Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury

Abstract Introduction Ischemic heart diseases are the leading cause of death worldwide due to the inability of regeneration of adult cardiomyocytes (CMs). Natural products from medical herbs are an important source of innovative drugs for many diseases including cardiovascular diseases. Objectives I...

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Main Authors: Kun Liu, Li Zheng, Qian-Yu Huang, Hong-Ji Li, Cheng Li, Hui Zhao, Ze-Bing Ye, Hao Wang, Xu-Feng Qi, Meng Wang
Format: Article
Language:English
Published: BMC 2025-06-01
Series:Chinese Medicine
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Online Access:https://doi.org/10.1186/s13020-025-01141-x
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author Kun Liu
Li Zheng
Qian-Yu Huang
Hong-Ji Li
Cheng Li
Hui Zhao
Ze-Bing Ye
Hao Wang
Xu-Feng Qi
Meng Wang
author_facet Kun Liu
Li Zheng
Qian-Yu Huang
Hong-Ji Li
Cheng Li
Hui Zhao
Ze-Bing Ye
Hao Wang
Xu-Feng Qi
Meng Wang
author_sort Kun Liu
collection DOAJ
description Abstract Introduction Ischemic heart diseases are the leading cause of death worldwide due to the inability of regeneration of adult cardiomyocytes (CMs). Natural products from medical herbs are an important source of innovative drugs for many diseases including cardiovascular diseases. Objectives In this study, we set out to screen novel small-molecule therapies from natural products to protect heart against ischemic injury. Methods High-throughput screening was performed using a natural product library to identify the potential small molecules which can promote survival of CMs under ischemic and ischemic/reperfusion conditions. In addition, myocardial infarction (MI) and ischemia/reperfusion (I/R) mice models were used to evaluate the in vivo effects of the screened candidate. We also applied various analysis including cell viability, qPCR, Western blot, immunofluorescent staining, echocardiography, Masson’s staining, TTC staining, and network pharmacology. Results High-throughput screening showed that the small molecule compound Darutigenol (Dar), derived from the Chinese traditional herb Herba Siegesbeckiae, could significantly promote CM survival and proliferation under ischemic conditions. Moreover, I/R-induced CM apoptosis and ROS generation could be significantly reduced by Dar treatment. In addition, in vivo administration of Dar was able to attenuate MI- and I/R-induced cardiac injury in adult mice by decreasing fibrosis and apoptosis, thereby improving cardiac function. Network pharmacology analysis and molecule docking assay showed that Dar has the highest binding affinity with AKT1 protein. Western blotting assay further revealed that AKT1 activation was significantly enhanced by Dar administration in the infarcted hearts. Conclusions Our data revealed that the small molecule compound Dar, screened from the natural product library in this study, is capable of protecting heart against MI and I/R injury by activating AKT1 pathway. These findings enrich the natural product candidates for cardiovascular disease treatment and provide new insights into potential therapeutic agents for MI and I/R injury.
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spelling doaj-art-35edfd677f964b0fa5d5f95e8689d5442025-08-20T03:47:16ZengBMCChinese Medicine1749-85462025-06-0120111510.1186/s13020-025-01141-xNatural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injuryKun Liu0Li Zheng1Qian-Yu Huang2Hong-Ji Li3Cheng Li4Hui Zhao5Ze-Bing Ye6Hao Wang7Xu-Feng Qi8Meng Wang9Department of Cardiology, Zhongshan Torch Development Zone People’s HospitalSchool of Environmental Science and Engineering, Guangdong University of TechnologyKey Laboratory of Regenerative Medicine of Ministry of Education, Institute of Aging and Regenerative Medicine, Department of Developmental & Regenerative Biology, and Department of Cardiology, The Affiliated Guangdong Second Provincial General Hospital, Jinan UniversityKey Laboratory of Regenerative Medicine of Ministry of Education, Institute of Aging and Regenerative Medicine, Department of Developmental & Regenerative Biology, and Department of Cardiology, The Affiliated Guangdong Second Provincial General Hospital, Jinan UniversityKey Laboratory of Regenerative Medicine of Ministry of Education, Institute of Aging and Regenerative Medicine, Department of Developmental & Regenerative Biology, and Department of Cardiology, The Affiliated Guangdong Second Provincial General Hospital, Jinan UniversityKey Laboratory of Regenerative Medicine of Ministry of Education, School of Biomedical Sciences, Faculty of Medicine, The Chinese University of Hong KongDepartment of Cardiology, The Affiliated Guangdong Second Provincial General Hospital, Jinan UniversityDepartment of Anesthesiology & Clinical Research Center, The First Affiliated Hospital, Jinan UniversityKey Laboratory of Regenerative Medicine of Ministry of Education, Institute of Aging and Regenerative Medicine, Department of Developmental & Regenerative Biology, and Department of Cardiology, The Affiliated Guangdong Second Provincial General Hospital, Jinan UniversityDepartment of Cardiology, Zhongshan Torch Development Zone People’s HospitalAbstract Introduction Ischemic heart diseases are the leading cause of death worldwide due to the inability of regeneration of adult cardiomyocytes (CMs). Natural products from medical herbs are an important source of innovative drugs for many diseases including cardiovascular diseases. Objectives In this study, we set out to screen novel small-molecule therapies from natural products to protect heart against ischemic injury. Methods High-throughput screening was performed using a natural product library to identify the potential small molecules which can promote survival of CMs under ischemic and ischemic/reperfusion conditions. In addition, myocardial infarction (MI) and ischemia/reperfusion (I/R) mice models were used to evaluate the in vivo effects of the screened candidate. We also applied various analysis including cell viability, qPCR, Western blot, immunofluorescent staining, echocardiography, Masson’s staining, TTC staining, and network pharmacology. Results High-throughput screening showed that the small molecule compound Darutigenol (Dar), derived from the Chinese traditional herb Herba Siegesbeckiae, could significantly promote CM survival and proliferation under ischemic conditions. Moreover, I/R-induced CM apoptosis and ROS generation could be significantly reduced by Dar treatment. In addition, in vivo administration of Dar was able to attenuate MI- and I/R-induced cardiac injury in adult mice by decreasing fibrosis and apoptosis, thereby improving cardiac function. Network pharmacology analysis and molecule docking assay showed that Dar has the highest binding affinity with AKT1 protein. Western blotting assay further revealed that AKT1 activation was significantly enhanced by Dar administration in the infarcted hearts. Conclusions Our data revealed that the small molecule compound Dar, screened from the natural product library in this study, is capable of protecting heart against MI and I/R injury by activating AKT1 pathway. These findings enrich the natural product candidates for cardiovascular disease treatment and provide new insights into potential therapeutic agents for MI and I/R injury.https://doi.org/10.1186/s13020-025-01141-xDrug screeningDarutigenolMyocardial infarctionIschemic/reperfusion injury
spellingShingle Kun Liu
Li Zheng
Qian-Yu Huang
Hong-Ji Li
Cheng Li
Hui Zhao
Ze-Bing Ye
Hao Wang
Xu-Feng Qi
Meng Wang
Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury
Chinese Medicine
Drug screening
Darutigenol
Myocardial infarction
Ischemic/reperfusion injury
title Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury
title_full Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury
title_fullStr Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury
title_full_unstemmed Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury
title_short Natural product library screening identifies Darutigenol for the treatment of myocardial infarction and ischemia/reperfusion injury
title_sort natural product library screening identifies darutigenol for the treatment of myocardial infarction and ischemia reperfusion injury
topic Drug screening
Darutigenol
Myocardial infarction
Ischemic/reperfusion injury
url https://doi.org/10.1186/s13020-025-01141-x
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