Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater

Abstract Sulfolane is a worldwide water-soluble pollutant, which typically migrates rapidly in impacted aquifers, with risks to water bodies and drinking water wells. Sulfolane migration may be delayed in sites co-polluted by hydrocarbons, which move more slowly and in which sulfolane partitions. Ho...

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Main Authors: Erica Pensini, Caitlyn Hsiung, Alejandro G. Marangoni
Format: Article
Language:English
Published: Springer 2025-05-01
Series:Discover Water
Subjects:
Online Access:https://doi.org/10.1007/s43832-025-00228-8
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author Erica Pensini
Caitlyn Hsiung
Alejandro G. Marangoni
author_facet Erica Pensini
Caitlyn Hsiung
Alejandro G. Marangoni
author_sort Erica Pensini
collection DOAJ
description Abstract Sulfolane is a worldwide water-soluble pollutant, which typically migrates rapidly in impacted aquifers, with risks to water bodies and drinking water wells. Sulfolane migration may be delayed in sites co-polluted by hydrocarbons, which move more slowly and in which sulfolane partitions. However, when bacteria such as Pseudomonas aeruginosa aerobically biodegrade hydrocarbons and sulfolane, they generate biosurfactants (such as rhamnolipids). These enclose sulfolane within micelles and droplets, as seen by optical microscopy, and hamper its partitioning into hydrocarbons, as shown by Fourier transform infrared spectroscopy. Therefore, biosurfactants have the potential to accelerate sulfolane migration in groundwater, compared to scenarios where biosurfactant-producing bacteria are absent. These findings will aid safe management of impacted sites, where aerobic bacterial bioremediation is used for pollutant clean-up. When aerobic bacterial activity is promoted to enable pollutant biodegradation, sulfolane migration may accelerate before clean-up is complete, begging for careful monitoring of pollutant plumes. Graphical Abstract
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issn 2730-647X
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spelling doaj-art-34ce0fca672440d6bb1befb0607348ad2025-08-20T03:08:44ZengSpringerDiscover Water2730-647X2025-05-015111410.1007/s43832-025-00228-8Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwaterErica Pensini0Caitlyn Hsiung1Alejandro G. Marangoni2School of Engineering, University of GuelphSchool of Engineering, University of GuelphBiophysics Interdepartmental Group (BIG), University of GuelphAbstract Sulfolane is a worldwide water-soluble pollutant, which typically migrates rapidly in impacted aquifers, with risks to water bodies and drinking water wells. Sulfolane migration may be delayed in sites co-polluted by hydrocarbons, which move more slowly and in which sulfolane partitions. However, when bacteria such as Pseudomonas aeruginosa aerobically biodegrade hydrocarbons and sulfolane, they generate biosurfactants (such as rhamnolipids). These enclose sulfolane within micelles and droplets, as seen by optical microscopy, and hamper its partitioning into hydrocarbons, as shown by Fourier transform infrared spectroscopy. Therefore, biosurfactants have the potential to accelerate sulfolane migration in groundwater, compared to scenarios where biosurfactant-producing bacteria are absent. These findings will aid safe management of impacted sites, where aerobic bacterial bioremediation is used for pollutant clean-up. When aerobic bacterial activity is promoted to enable pollutant biodegradation, sulfolane migration may accelerate before clean-up is complete, begging for careful monitoring of pollutant plumes. Graphical Abstracthttps://doi.org/10.1007/s43832-025-00228-8Bacterial biosurfactantsContaminant migrationSulfolaneCo-contaminants
spellingShingle Erica Pensini
Caitlyn Hsiung
Alejandro G. Marangoni
Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater
Discover Water
Bacterial biosurfactants
Contaminant migration
Sulfolane
Co-contaminants
title Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater
title_full Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater
title_fullStr Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater
title_full_unstemmed Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater
title_short Biosurfactant-producing bacteria counteract hydrocarbon-driven delay of sulfolane migration in groundwater
title_sort biosurfactant producing bacteria counteract hydrocarbon driven delay of sulfolane migration in groundwater
topic Bacterial biosurfactants
Contaminant migration
Sulfolane
Co-contaminants
url https://doi.org/10.1007/s43832-025-00228-8
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AT caitlynhsiung biosurfactantproducingbacteriacounteracthydrocarbondrivendelayofsulfolanemigrationingroundwater
AT alejandrogmarangoni biosurfactantproducingbacteriacounteracthydrocarbondrivendelayofsulfolanemigrationingroundwater