Textile waste pre-treatments for enhanced chemical recycling

Abstract Textile waste recycling faces significant challenges due to contaminants that remain on the fibers, interfering with recovery processes regardless of the method used. In chemical recycling, the original finishing additives present in textiles can disrupt secondary reactions, making a pre-tr...

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Main Authors: Cecília Ribeiro, Diana Sofia Pinto, Ana Francisca Miranda, João Seixas, Marcelo Oliveira, Catarina Costa
Format: Article
Language:English
Published: Springer 2025-05-01
Series:Discover Applied Sciences
Subjects:
Online Access:https://doi.org/10.1007/s42452-025-07091-1
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author Cecília Ribeiro
Diana Sofia Pinto
Ana Francisca Miranda
João Seixas
Marcelo Oliveira
Catarina Costa
author_facet Cecília Ribeiro
Diana Sofia Pinto
Ana Francisca Miranda
João Seixas
Marcelo Oliveira
Catarina Costa
author_sort Cecília Ribeiro
collection DOAJ
description Abstract Textile waste recycling faces significant challenges due to contaminants that remain on the fibers, interfering with recovery processes regardless of the method used. In chemical recycling, the original finishing additives present in textiles can disrupt secondary reactions, making a pre-treatment step essential for impurity removal and chemical recycling process optimization. This study explores effective pre-treatment methods for the chemical recycling of cotton (CO) and polyester-cotton blends (PES-CO/CO-PES), focusing on approaches that balance efficiency and sustainability. An alkaline pre-treatment was used for decolorizing the samples, with ISO brightness measured, showing PES-CO achieving the best result (80.6%). As an innovation, process optimization was carried out by introducing an additive that allowed a 50% reduction in the amount of Na2S2O4 required while maintaining decolorization efficiency. This modification enhances process sustainability by reducing the consumption of chemical reagents. Additionally, an acid treatment with nitric acid was applied after the alkaline treatment to remove residual metals that could interfere with chemical recycling. This step proved highly beneficial, not only improving the purity of recycled materials but also increasing ISO brightness in all analyzed samples. Another crucial factor assessed was the degree of polymerization (DPv), which determines the material’s suitability for further recycling processes. Results showed a slight decrease in DPv throughout the treatments, indicating that despite the effective removal of dyes and contaminants, the structural integrity of the fibers was preserved, ensuring high-quality recycled material.
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spelling doaj-art-346fcf0884f144cb9a40a1efb4d82e502025-08-20T01:53:19ZengSpringerDiscover Applied Sciences3004-92612025-05-017611210.1007/s42452-025-07091-1Textile waste pre-treatments for enhanced chemical recyclingCecília Ribeiro0Diana Sofia Pinto1Ana Francisca Miranda2João Seixas3Marcelo Oliveira4Catarina Costa5CeNTI-Centre for Nanotechnology and Advanced MaterialsCeNTI-Centre for Nanotechnology and Advanced MaterialsCeNTI-Centre for Nanotechnology and Advanced MaterialsCeNTI-Centre for Nanotechnology and Advanced MaterialsCeNTI-Centre for Nanotechnology and Advanced MaterialsCeNTI-Centre for Nanotechnology and Advanced MaterialsAbstract Textile waste recycling faces significant challenges due to contaminants that remain on the fibers, interfering with recovery processes regardless of the method used. In chemical recycling, the original finishing additives present in textiles can disrupt secondary reactions, making a pre-treatment step essential for impurity removal and chemical recycling process optimization. This study explores effective pre-treatment methods for the chemical recycling of cotton (CO) and polyester-cotton blends (PES-CO/CO-PES), focusing on approaches that balance efficiency and sustainability. An alkaline pre-treatment was used for decolorizing the samples, with ISO brightness measured, showing PES-CO achieving the best result (80.6%). As an innovation, process optimization was carried out by introducing an additive that allowed a 50% reduction in the amount of Na2S2O4 required while maintaining decolorization efficiency. This modification enhances process sustainability by reducing the consumption of chemical reagents. Additionally, an acid treatment with nitric acid was applied after the alkaline treatment to remove residual metals that could interfere with chemical recycling. This step proved highly beneficial, not only improving the purity of recycled materials but also increasing ISO brightness in all analyzed samples. Another crucial factor assessed was the degree of polymerization (DPv), which determines the material’s suitability for further recycling processes. Results showed a slight decrease in DPv throughout the treatments, indicating that despite the effective removal of dyes and contaminants, the structural integrity of the fibers was preserved, ensuring high-quality recycled material.https://doi.org/10.1007/s42452-025-07091-1DecolorizationTextile wasteAcid treatmentTextile recycling
spellingShingle Cecília Ribeiro
Diana Sofia Pinto
Ana Francisca Miranda
João Seixas
Marcelo Oliveira
Catarina Costa
Textile waste pre-treatments for enhanced chemical recycling
Discover Applied Sciences
Decolorization
Textile waste
Acid treatment
Textile recycling
title Textile waste pre-treatments for enhanced chemical recycling
title_full Textile waste pre-treatments for enhanced chemical recycling
title_fullStr Textile waste pre-treatments for enhanced chemical recycling
title_full_unstemmed Textile waste pre-treatments for enhanced chemical recycling
title_short Textile waste pre-treatments for enhanced chemical recycling
title_sort textile waste pre treatments for enhanced chemical recycling
topic Decolorization
Textile waste
Acid treatment
Textile recycling
url https://doi.org/10.1007/s42452-025-07091-1
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AT dianasofiapinto textilewastepretreatmentsforenhancedchemicalrecycling
AT anafranciscamiranda textilewastepretreatmentsforenhancedchemicalrecycling
AT joaoseixas textilewastepretreatmentsforenhancedchemicalrecycling
AT marcelooliveira textilewastepretreatmentsforenhancedchemicalrecycling
AT catarinacosta textilewastepretreatmentsforenhancedchemicalrecycling