Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window

Excitation at the 1700-nm window is an effective means for extending imaging depth and imaging modalities in multiphoton microscopy (MPM). To enhance multiphoton signal levels and enable deep-tissue penetration, water immersion has to be replaced by deuterium dioxide (D<sub>2</sub>O) imm...

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Main Authors: Hongji Liu, Yu Du, Xiao Peng, Xuechang Zhou, Ping Qiu, Ke Wang
Format: Article
Language:English
Published: IEEE 2017-01-01
Series:IEEE Photonics Journal
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Online Access:https://ieeexplore.ieee.org/document/8013790/
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author Hongji Liu
Yu Du
Xiao Peng
Xuechang Zhou
Ping Qiu
Ke Wang
author_facet Hongji Liu
Yu Du
Xiao Peng
Xuechang Zhou
Ping Qiu
Ke Wang
author_sort Hongji Liu
collection DOAJ
description Excitation at the 1700-nm window is an effective means for extending imaging depth and imaging modalities in multiphoton microscopy (MPM). To enhance multiphoton signal levels and enable deep-tissue penetration, water immersion has to be replaced by deuterium dioxide (D<sub>2</sub>O) immersion to boost transmittance at the 1700-nm window. The key problem facing this D<sub>2</sub>O immersion technique is the hygroscopic nature of D<sub>2</sub>O, which leads to decrease of MPM signals as time lapses. Here, we demonstrate a simple, yet very effective technique to isolate D<sub>2 </sub>O from the ambient environment, by sealing it with the paraffin liquid. We demonstrate the application of this technique to MPM signal maintenance in both three-photon fluorescence generation in a fluorescent dye and third-harmonic generation (THG) imaging of biological tissue, excited at the 1700-nm window. <italic>Ex-vivo</italic> imaging results show that during an imaging session of 5 h, multiphoton signals of both modalities can be maintained with no deterioration due to absorption of water vapor from the environment. Furthermore, we demonstrate <italic> in-vivo</italic> deep-tissue mouse brain imaging using this technique, in which THG signals can be maintained for at least 5 h. This justifies the applicability and effectiveness of our D<sub>2</sub>O sealing technique for long-span <italic>in-vivo</italic> imaging.
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spelling doaj-art-3302a07925404ac6b705630ebb2a362a2025-08-20T03:14:51ZengIEEEIEEE Photonics Journal1943-06552017-01-01951810.1109/JPHOT.2017.27370128013790Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm WindowHongji Liu0Yu Du1Xiao Peng2Xuechang Zhou3Ping Qiu4Ke Wang5Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, College of Optoelectronic Engineering, Shenzhen University, Shenzhen, ChinaKey Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, College of Optoelectronic Engineering, Shenzhen University, Shenzhen, ChinaKey Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, College of Optoelectronic Engineering, Shenzhen University, Shenzhen, ChinaCollege of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, ChinaCollege of Physics and Energy, Shenzhen University, Shenzhen, ChinaKey Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, College of Optoelectronic Engineering, Shenzhen University, Shenzhen, ChinaExcitation at the 1700-nm window is an effective means for extending imaging depth and imaging modalities in multiphoton microscopy (MPM). To enhance multiphoton signal levels and enable deep-tissue penetration, water immersion has to be replaced by deuterium dioxide (D<sub>2</sub>O) immersion to boost transmittance at the 1700-nm window. The key problem facing this D<sub>2</sub>O immersion technique is the hygroscopic nature of D<sub>2</sub>O, which leads to decrease of MPM signals as time lapses. Here, we demonstrate a simple, yet very effective technique to isolate D<sub>2 </sub>O from the ambient environment, by sealing it with the paraffin liquid. We demonstrate the application of this technique to MPM signal maintenance in both three-photon fluorescence generation in a fluorescent dye and third-harmonic generation (THG) imaging of biological tissue, excited at the 1700-nm window. <italic>Ex-vivo</italic> imaging results show that during an imaging session of 5 h, multiphoton signals of both modalities can be maintained with no deterioration due to absorption of water vapor from the environment. Furthermore, we demonstrate <italic> in-vivo</italic> deep-tissue mouse brain imaging using this technique, in which THG signals can be maintained for at least 5 h. This justifies the applicability and effectiveness of our D<sub>2</sub>O sealing technique for long-span <italic>in-vivo</italic> imaging.https://ieeexplore.ieee.org/document/8013790/Fluorescence microscopynon-linear microscopyoptical properties of photonic materials.
spellingShingle Hongji Liu
Yu Du
Xiao Peng
Xuechang Zhou
Ping Qiu
Ke Wang
Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window
IEEE Photonics Journal
Fluorescence microscopy
non-linear microscopy
optical properties of photonic materials.
title Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window
title_full Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window
title_fullStr Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window
title_full_unstemmed Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window
title_short Sealing of Immersion Deuterium Dioxide and Its Application to Signal Maintenance for Ex-Vivo and In-Vivo Multiphoton Microscopy Excited at the 1700-nm Window
title_sort sealing of immersion deuterium dioxide and its application to signal maintenance for ex vivo and in vivo multiphoton microscopy excited at the 1700 nm window
topic Fluorescence microscopy
non-linear microscopy
optical properties of photonic materials.
url https://ieeexplore.ieee.org/document/8013790/
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